PEMFC cathode catalyst contamination evaluation with a RRDE-acetylene

Electrochimica Acta

Volumn 133, Issue , 2014, Pages 65-72

  Ge, Junjie ^a   St Pierre, Jean ^a   Zhai, Yunfeng ^a  

^a UNIVERSITY OF HAWAII   (United States)

Author keywords

Acetylene; Airborne Contaminant; ORR; PEMFC; RRDE

Indexed keywords

ACETYLENE; CATALYSTS; CATHODES; CYCLIC VOLTAMMETRY; ELECTROLYTIC REDUCTION; LIGHTING; PLATINUM; PROTON EXCHANGE MEMBRANE FUEL CELLS (PEMFC);

ADSORPTION ENERGIES; AIRBORNE CONTAMINANTS; ELECTROCHEMICAL SURFACE AREA; ORR; OXYGEN REDUCTION REACTION; RATE DETERMINING STEP; ROTATING RING-DISK ELECTRODE TECHNIQUES; RRDE;

ADSORPTION;

EID: 84899554883     PISSN: 00134686     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.electacta.2014.04.005     Document Type: Article

References (24)

1. D. van der Vliet, D.S. Strmcnik, C. Wang, V.R. Stamenkovic, N.M. Markovic, and M.T.M. Koper On the importance of correcting for the uncompensated Ohmic resistance in model experiments of the Oxygen Reduction Reaction J. Electroanal. Chem. 647 2010 29 34
2. Y. Zhai, G. Bender, S. Dorn, and R. Rocheleau The Multiprocess Degradation of PEMFC Performance Due to Sulfur Dioxide Contamination and Its Recovery J. Electrochem. Soc. 157 2010 B20 B26
3. M.R. Rahman, M.I. Awad, F. Kitamura, T. Okajima, and T. Ohsaka A comparative study of ORR at the Pt electrode in ammonium ion-contaminated H2SO4 and HClO4 solutions J. Power Sources 220 2012 65 73
4. M.S. El-Deab, F. Kitamura, and T. Ohsaka Impact of acrylonitrile poisoning on oxygen reduction reaction at Pt/C catalysts J. Power Sources 229 2013 65 71
5. J. St-Pierre, M. Angelo, and Y. Zhai Focusing Research by Developing Performance Related Selection Criteria for PEMFC Contaminants ECS Transactions 41 2011 279 286
6. O.A. Baturina, B.D. Gould, Y. Garsany, and K.E. Swider-Lyons Insights on the SO2 poisoning of Pt3Co/VC and Pt/VC fuel cell catalysts Electrochimica Acta 55 2010 6676 6686
7. B.D. Gould, O.A. Baturina, and K.E. Swider-Lyons Deactivation of Pt/VC proton exchange membrane fuel cell cathodes by SO2, H2S and CO J. Power Sources 188 2009 89 95
8. Y. Nagahara, S. Sugawara, and K. Shinohara The impact of air contaminants on PEMFC performance and durability J. Power Sources 182 2008 422 428
9. Y. Garsany, S. Dutta, and K.E. Swider-Lyons Effect of glycol-based coolants on the suppression and recovery of platinum fuel cell electrocatalysts J. Power Sources 216 2012 515 525
10. J. St-Pierre, Y.F. Zhai, and M. Angelo Quantitative ranking criteria for PEMFC contaminants International Journal of Hydrogen Energy 37 2012 6784 6789
11. D.J. Burnett, A.M. Gabelnick, D.A. Fischer, A.L. Marsh, and J.L. Gland Mechanism of acetylene oxidation on the Pt(111) surface using in situ fluorescence yield near-edge spectroscopy Journal of Catalysis 230 2005 282 290
12. X.Q. Lu, L. Liu, Y. Li, W.Y. Guo, L.M. Zhao, and H.H. Shan Theoretical analysis of the conversion mechanism of acetylene to ethylidyne on Pt(111) Phys. Chem. Chem. Phys. 14 2012 5642 5650
13. A.B. Delgado, A.M.C. Luna, W.E. Triaca, and A.J. Arvia The Adsorption and the Potentiodynamic Electrooxidation of Acetylene on Platinized Platinum J. Electrochem. Soc. 129 1982 1493 1498 (Pubitemid 12532461)
14. S.P. Mehandru, and A.B. Anderson Dependence of carbon-carbon and carbon-hydrogen bond activation on d band position: acetylene on platinum(111) and iron(100). An electrochemical model J. Am. Chem. Soc. 107 1985 844 849
15. E.L. Muetterties, M.C. Tsai, and S.R. Kelemen Chemistry of Acetylene on Platinum (111) And (100) Surfaces Proceedings of the National Academy of Sciences of the United States of America-Physical Sciences 78 1981 6571 6575
16. J.W. Johnson, H. Wroblowa, and J.O.M. Bockris The Mechanism of the Electro-Oxidation of Acetylene on Platinum J. Electrochem. Soc. 111 1964 863 870
17. Y. Garsany, I.L. Singer, and K.E. Swider-Lyons Impact of film drying procedures on RDE characterization of Pt/VC electrocatalysts Journal of Electroanalytical Chemistry 662 2011 396 406
18. K.J.J. Mayrhofer, D. Strmcnik, B.B. Blizanac, V. Stamenkovic, M. Arenz, and N.M. Markovic Measurement of oxygen reduction activities via the rotating disc electrode method: From Pt model surfaces to carbon-supported high surface area catalysts Electrochimica Acta 53 2008 3181 3188
19. V. Stamenkovic, T.J. Schmidt, P.N. Ross, and N.M. Markovic Surface composition effects in electrocatalysis: Kinetics of oxygen reduction on well-defined Pt3Ni and Pt3Co alloy surfaces J. Phys. Chem. B 106 2002 11970 11979 (Pubitemid 35433950)
20. J. Lipkowski, P.N., Ross, Electrocatalysis, Wiley, 1998.
21. A.W.E. Chan, R. Hoffmann, and W. Ho Theoretical aspects of photoinitiated chemisorption, dissociation, and desorption of oxygen on platinum(111) Langmuir 8 1992 1111 1119 (Pubitemid 23572920)
22. N.M. Markovic, H.A. Gasteiger, B.N. Grgur, and P.N. Ross Oxygen reduction reaction on Pt(111): effects of bromide Journal of Electroanalytical Chemistry 467 1999 157 163
23. H.A. Gasteiger, S.S. Kocha, B. Sompalli, and F.T. Wagner Activity benchmarks and requirements for Pt, Pt-alloy, and non-Pt oxygen reduction catalysts for PEMFCs Appl. Catal. B-Environ 56 2005 9 35
24. J. St-Pierre, Y. Zhai, and M.S. Angelo Effect of selected airborne contaminants on PEMFC performance J Electrochem. Soc. 161 2014 F280 F290