Chemical reduction of actinides probed by resonant inelastic x-ray scattering

Analytical Chemistry

Volumn 85, Issue 23, 2013, Pages 11196-11200

  Butorin, Sergei M ^a   Shuh, David K ^b   Kvashnina, Kristina O ^a,c   Guo, Jinghua ^b   Werme, Lars ^a   Nordgren, Joseph ^a  

^a UPPSALA UNIVERSITY   (Sweden)

^b LAWRENCE BERKELEY NATIONAL LABORATORY   (United States)

^c EUROPEAN SYNCHROTRON RADIATION FACILITY   (France)

Author keywords

[No Author keywords available]

Indexed keywords

CHARACTERISTIC FLUORESCENCE; CHEMICAL REDUCTION; IRON SURFACE; METALLIC IRON; MOBILE SPECIES; REDUCTION RATE; RESONANT INELASTIC X-RAY SCATTERING; WASTE CANISTERS;

GROUNDWATER; NEPTUNIUM; RADIOACTIVE WASTES; URANIUM; URANIUM COMPOUNDS;

X RAY SCATTERING;

EID: 84889077136     PISSN: 00032700     EISSN: 15206882     Source Type: Journal    
DOI: 10.1021/ac4020534     Document Type: Article

References (13)

1. Suzuki, Y.; Kelly, S. D.; Kemner, K. M.; Banfield, J. F. Nature 2002, 419, 134
2. Lovely, D. R.; Phillips, E. J. P.; Gorby, Y. A.; Landa, E. R. Nature 1991, 350, 413
3. Wiell, T.; Tillborg, H.; Nilsson, A.; Wassdahl, N.; MaÌŠ rtensson, N.; Nordgren, J. Local probing of adsorbate electronic structure using soft X-ray emission; atomic nitrogen on Ni(100) and Cu(100) Surf. Sci. Lett. 1994, 304, L451-L455
4. Nilsson, P. O.; Kanski, J.; Thordson, J. V.; Andersson, T. G.; Nordgren, J.; Guo, J.; Magnusson, M. Electronic structure of buried Si layers in GaAs(001) as studied by soft X-ray emission Phys. Rev. B 1995, 52, R8643-R8645
5. Fanghänel, Th.; Neck, V. Aquatic chemistry and solubility phenomena of actinide oxides/hydrooxides Pure Appl. Chem. 2002, 74, 1895-1907 and references therein.
6. Grenthe, I.; Fuger, J.; Konings, R. J. M.; Lemire, R. J.; Muller, A. B.; Nguyen-Trung, C.; Wanner, H., Eds. Organisation for Economic Co-operation and Development (OECD), Nuclear Energy Agency (NEA). Chemical Thermodynamics of Uranium; Elsevier/North-Holland: Amsterdam/Oxford, U.K., 1992.
7. Lemire, R. J.; Fuger, J.; Nitsche, H.; Potter, P.; Rand, M. H.; Rydberg, J.; Spahiu, K.; Sullivan, J. C.; Ullman, W. J.; Vitorge, P.; Wanner, H., Eds. Organisation for Economic Co-operation and Development (OECD), Nuclear Energy Agency (NEA). Chemical Thermodynamics of Neptunium and Plutonium; Elsevier/North-Holland: Amsterdam/Oxford, U.K., 2001.
8. Butorin, S. M. Resonant inelastic X-ray scattering as a probe of optical scale excitations in strongly electron-correlated systems: quasi-localized view J. Electr. Spectros. Relat. Phenomena 2000, 110-111, 213-233
9. Kalkowski, G.; Kaindl, G.; Brewer, W. D.; Krone, W. Near-edge X-ray absorption fine structure in uranium compounds Phys. Rev. 1987, B35, 2667-2677
10. Warwick, T.; Heimann, P.; Mossessian, D.; McKinney, W.; Padmore, H. Performance of a high resolution, high flux density SGM undulator beamline at the ALS Rev. Sci. Instrum. 1995, 66, 2037-2040
11. Nordgren, J.; Bray, G.; Cramm, S.; Nyholm, R.; Rubensson, J.-E.; Wassdahl, N. Soft X-ray emission spectroscopy using monochromatized synchrotron radiation Rev. Sci. Instrum. 1989, 60, 1690-1696
12. Butorin, S.; Ollila, K.; Albinsson, Y.; Nordgren, J.; Werme, L. Reduction of uranyl carbonate and hydroxyl complexes and neptunyl carbonate complexes studied with chemical-electrochemical methods and RIXS spectroscopy, Posiva Report 2004-1, May 2004, (ISBN 951-652-127-4).
13. Kvashnina, K. O.; Butorin, S. M.; Shuh, D. K.; Guo, J.-H.; Werme, L.; Nordgren, J. Resonant Inelastic X-ray Scattering of Curium Oxide Phys. Rev. B 2007, 75, 115107