Arsenic(III) and iron(II) co-oxidation by oxygen and hydrogen peroxide: Divergent reactions in the presence of organic ligands

Chemosphere

Volumn 93, Issue 9, 2013, Pages 1936-1941

  Wang, Zhaohui ^a,b   Bush, Richard T ^a   Liu, Jianshe ^b  

^a SOUTHERN CROSS UNIVERSITY   (Australia)

^b DONGHUA UNIVERSITY   (China)

Author keywords

Arsenic; EDTA; Fe(II) oxidation; Fenton reaction; Radical scavenger

Indexed keywords

ARSENIC; CATALYSIS; ETHYLENEDIAMINETETRAACETIC ACID; LIGANDS; OXIDATION; REMEDIATION;

ARSENIC REMEDIATIONS; ENGINEERED SYSTEMS; FENTON REACTIONS; HYDROXYL RADICALS; IRON-CATALYZED OXIDATIONS; NATURALLY OCCURRING; PARTIAL OXIDATIONS; RADICAL SCAVENGERS;

IRON COMPOUNDS;

2 PROPANOL; ARSENIC; EDETIC ACID; FERROUS ION; HYDROGEN PEROXIDE; IRON; LIGAND; METHANOL; OXYGEN; SCAVENGER;

ARSENIC; CONCENTRATION (COMPOSITION); IRON; LIGAND; OPTIMIZATION; OXIDATION; PH; REMOVAL EXPERIMENT; SPECIATION (CHEMISTRY);

AQUATIC ENVIRONMENT; ARTICLE; CATALYST; CHEMICAL ANALYSIS; CHEMICAL REACTION; CONCENTRATION (PARAMETERS); CONTROLLED STUDY; CROSS COUPLING REACTION; FENTON REACTION; OXIDATION; OXIDATION REDUCTION STATE; PH; PROCESS OPTIMIZATION; SYNTHESIS;

ARSENIC; EDTA; FE(II) OXIDATION; FENTON REACTION; RADICAL SCAVENGER;

ARSENIC; EDETIC ACID; ENVIRONMENTAL REMEDIATION; GROUNDWATER; HYDROGEN PEROXIDE; IRON; LIGANDS; OXIDATION-REDUCTION; OXYGEN; WATER POLLUTANTS, CHEMICAL;

EID: 84886429016     PISSN: 00456535     EISSN: 18791298     Source Type: Journal    
DOI: 10.1016/j.chemosphere.2013.06.076     Document Type: Article

References (31)

1. Burton E.D., Bush R.T., Johnston S.G., Watling K., Hocking R.K., Sullivan L.A., Heber G.K. Sorption of arsenic(V) and arsenic(III) to schwertmannite. Environ. Sci. Technol. 2009, 43:9202-9207.
2. Bussan A.L., Strathmann T.J. Influence of organic ligands on the reduction of polyhalogenated alkanes by iron(II). Environ. Sci. Technol. 2007, 41:6740-6747.
3. Buxton G.V., Greenstock C.L., Helman W.P., Ross A.B. Critical review of rate constants for reactions of hydrated electrons, hydrogen atoms and hydroxyl radicals in aqueous solutions. J. Phys. Chem. Ref. Data. 1988, 17:513-886.
4. Cullen W.R., Reimer K.J. Arsenic speciation in the environment. Chem. Rev. 1989, 89:713-764.
5. Dhar R.K., Zheng Y., Rubenstone J., van Geen A. A rapid colorimetric method of measuring arsenic concentrations in groundwater. Anal. Chim. Acta 2004, 526:203-209.
6. Engelmann M.D., Bobier R.T., Hiatt T., Cheng I.F. Variability of the Fenton reaction characteristics of the EDTA, DTPA, and citrate complexes of iron. BioMetals 2003, 16:519-527.
7. Gustafsson, J.P., 2010. Visual MINTEQ ver. 3.0. http://www2.lwr.kth.se/English/OurSoftware/vminteq/index.htm.
8. Hersey M. Oxidation of arsenite via chelator mediated Fenton systems, Master Thesis 2006, The University of Maine, Orono, ME.
9. Hug S.J., Leupin O. Iron-catalyzed oxidation of arsenic(III) by oxygen and by hydrogen peroxide: pH-dependent formation of oxidants in the Fenton reaction. Environ. Sci. Technol. 2003, 37:2734-2742.
10. Jacobsen F., Holcman J., Sehested K. Reactions of the ferryl ion with some compounds found in cloud water. Int. J. Chem. Kinet. 1998, 30:215-221.
11. Katsoyiannis I.A., Ruettimann T., Hug S.J. PH dependence of Fenton reagent generation and As(III) oxidation and removal by corrosion of zero valent iron in aerated water. Environ. Sci. Technol. 2008, 42:7424-7430.
12. Keenan C.R., Sedlak D.L. Factors affecting the yield of oxidants from the reaction of nanoparticulate zero-valent iron and oxygen. Environ. Sci. Technol. 2008, 42:1262-1267.
13. Kurimura Y., Ochiai R., Matsuura N. Oxygen oxidation of ferrous ions induced by chelation. Bull. Chem. Soc. Jpn. 1968, 41:2234-2239.
14. Meng X.G., Bang S., Korfiatis G.P. Effect of silicate, sulfate and carbonate on arsenic removal by ferric hydroxide. Water Res. 2000, 34:1255-1261.
15. Mohan D., Pittman C.U. Arsenic removal from water/wastewater using adsorbents - a critical review. J. Hazard. Mater. 2007, 142:1-53.
16. Monod A., Chebbi A., Durand-Jolibois R., Carlier P. Oxidation of methanol by hydroxyl radicals in aqueous solution under simulated cloud droplet conditions. Atmos. Environ. 2000, 34:5283-5294.
17. Noradoun C.E., Cheng I.F. EDTA degradation induced by oxygen activation in a zero-valent iron/air/water system. Environ. Sci. Technol. 2005, 39:7158-7163.
18. Pang S.Y., Jiang J., Ma J., Pang S.Y., Ouyang F. New insight into the oxidation of arsenite by the reaction of zerovalent iron and oxygen. Comment on "pH dependence of Fenton reagent generation and As(III) oxidation and removal by corrosion of zero valent iron in aerated water. Environ. Sci. Technol. 2009, 43:3978-3979.
19. Pang S.Y., Jiang J., Ma J. Oxidation of sulfoxides and arsenic(III) in corrosion of nanoscale zero valent iron by oxygen: evidence against ferryl ions (Fe(IV)) as active intermediates in Fenton reaction. Environ. Sci. Technol. 2011, 45:307-312.
20. Pignatello J.J., Oliveros E., MacKay A. Advanced oxidation processes for organic contaminant destruction based on the Fenton reaction and related chemistry. Crit. Rev. Environ. Sci. Technol. 2006, 36:1-84.
21. Rastogi A., Al-Abed S.R., Dionysiou D.D. Effect of inorganic, synthetic and naturally occurring chelating agents on Fe(II) mediated advanced oxidation of chlorophenols. Water Res. 2009, 43:684-694.
22. 2. Mar. Chem. 2006, 99:70-82.
23. Sedlak D.L., Hoigné J. The role of copper and oxalate in the redox cycling of iron in atmospheric waters. Atmos. Environ. 1993, 27A:2173-2185.
24. II(edta)] oxidation by molecular oxygen revisited. New evidence for a multistep mechanism. Inorg. Chem. 1997, 36:4115-4120.
25. Smedley P.L., Kinniburgh D.G. A review of the source, behaviour and distribution of arsenic in natural waters. Appl. Geochem. 2002, 17:517-568.
26. Sun Y., Pignatello J.J. Chemical treatment of pesticide wastes. Evaluation of Fe(III) chelates for catalytic hydrogen peroxide oxidation of 2,4-D at circumneutral pH. J. Agric. Food. Chem. 1992, 40:322-327.
27. Viollier E., Inglett P.W., Hunter K., Roychoudhury A.N., Van Cappellen P. The ferrozine method revisited: Fe(II)/Fe(III) determination in natural waters. Appl. Geochem. 2000, 15:785-790.
28. Wang Z.H., Ma W.H., Chen C.C., Zhao J.C. Photochemical coupling reactions between Fe(III)/Fe(II), Cr(VI)/Cr(III) and polycarboxylates: inhibitory effect of Cr species. Environ. Sci. Technol. 2008, 42:7260-7266.
29. Wang Z.H., Chen X., Ma W.H., Chen C.C., Zhao J.C. Photochemical cycling of iron mediated by dicarboxylates: special effect of malonate. Environ. Sci. Technol. 2010, 44:263-268.
30. Wang Z.H., Ma W.H., Chen C.C., Ji H.W., Zhao J.C. Photochemical coupling of iron redox reactions and transformation of low-molecular-weight organic matter. J. Phys. Chem. Lett. 2012, 3:2044-2051.
31. Woods R., Kolthoff I.M., Meehan E.J. Arsenic (IV) as an intermediate in the induced oxidation of Arsenic(III) by the iron (II)-hydrogen peroxide reaction. J. Am. Chem. Soc. 1964, 86:1670-1698.