Measurement of an electronic resonance in a ground-state, gas-phase acetophenone cation via strong-field mass spectrometry

Journal of Physical Chemistry Letters

Volumn 4, Issue 10, 2013, Pages 1587-1591

  Bohinski, Timothy ^a   Moore Tibbetts, Katharine ^a   Tarazkar, Maryam ^a   Romanov, Dmitri ^a   Matsika, Spiridoula ^a   Levis, Robert J ^a  

^a Temple University   (United States)

Author keywords

electronic spectroscopy; femtosecond mass spectrometry; ionic resonance; tunnel ionization

Indexed keywords

ELECTRONIC SPECTROSCOPY; EQUATION OF MOTION COUPLED CLUSTERS; EXCITATION WAVELENGTH; FEMTOSECONDS; FORBIDDEN TRANSITIONS; NON-PLANAR STRUCTURES; RESONANT WAVELENGTHS; TUNNEL IONIZATION;

EQUATIONS OF MOTION; EXCITED STATES; IONIZATION OF GASES; KETONES; MASS SPECTROMETERS; PHOTONS; RESONANCE;

MASS SPECTROMETRY;

EID: 84878038669     PISSN: None     EISSN: 19487185     Source Type: Journal    
DOI: 10.1021/jz400516h     Document Type: Article

References (21)

1. Becker, K. H.; Tarnovsky, V. Electron-Impact Ionization of Atoms, Molecules, Ions and Transient Species Plasma Sources Sci. Technol. 1995, 4, 307
2. Krylov, A. I. Equation-of-Motion Coupled-Cluster Methods for Open-Shell and Electronically Excited Species: The Hitchhiker'S Guide to Fock Space. Annual Review of Physical Chemistry; Annual Reviews: Palo Alto, CA, 2008; Vol. 59, pp 433-462. (Pubitemid 351703394)
3. Matsika, S.; Krause, P. Nonadiabatic Events and Conical Intersections. In Annual Review of Physical Chemistry; Leone, S. R.; Cremer, P. S.; Groves, J. T.; Johnson, M. A., Eds.; Annual Reviews: Palo Alto, CA, 2011; Vol. 62, pp 621-643.
4. Lezius, M.; Blanchet, V.; Ivanov, M. Y.; Stolow, A. Polyatomic Molecules in Strong Laser Fields: Nonadiabatic Multielectron Dynamics J. Chem. Phys. 2002, 117, 1575-1588 (Pubitemid 34923907)
5. Harada, H.; Shimizu, S.; Yatsuhashi, T.; Sakabe, S.; Izawa, Y.; Nakashima, N. A Key Factor in Parent and Fragment Ion Formation on Irradiation with an Intense Femtosecond Laser Pulse Chem. Phys. Lett. 2001, 342, 563-570 (Pubitemid 33628336)
6. Kotur, M.; Weinacht, T.; Pearson, B. J.; Matsika, S. Closed-Loop Learning Control of Isomerization Using Shaped Ultrafast Laser Pulses in the Deep Ultraviolet J. Chem. Phys. 2009, 130, 134311
7. Yatsuhashi, T.; Nakashima, N. Effects of Polarization of 1.4 μm Femtosecond Laser Pulses on the Formation and Fragmentation of Naphthalene Molecular Ions Compared at the Same Effective Ionization Intensity J. Phys. Chem. A 2005, 109, 9414-9418 (Pubitemid 41598525)
8. Markevitch, A. N.; Nakashima, N.; Smith, S. M.; Romanov, D. A.; Schlegel, H. B.; Ivanov, M. Y.; Levis, R. J. Nonadiabatic Dynamics of Polyatomic Molecules and Ions in Strong Laser Fields Phys. Rev. A 2003, 68, 011402
9. Trushin, S. A.; Fuss, W.; Schmid, W. E. Dissociative Ionization at High Laser Intensities: Importance of Resonances and Relaxation for Fragmentation J. Phys. B: At., Mol. Opt. Phys. 2004, 37, 3987-4011
10. Amarie, S.; Arefe, K.; Starcke, J. H.; Dreuw, A.; Wachtveitl, J. Identification of an Additional Low-Lying Excited State of Carotenoid Radical Cations J. Phys. Chem. B 2008, 112, 14011-14017
11. Grilj, J.; Buchgraber, P.; Vauthey, E. Excited-State Dynamics of Wurster's Salts J. Phys. Chem. A 2012, 116, 7516-7522
12. Pearson, B. J.; Nichols, S. R.; Weinacht, T. Molecular Fragmentation Driven by Ultrafast Dynamic Ionic Resonances J. Chem. Phys. 2007, 127, 131101
13. Nichols, S. R.; Weinacht, T. C.; Rozgonyi, T.; Pearson, B. J. Strong-Field Phase-Dependent Molecular Dissociation Phys. Rev. A 2009, 79, 043407
14. Trallero, C.; Pearson, B. J.; Weinacht, T.; Gilliard, K.; Matsika, S. Interpreting Ultrafast Molecular Fragmentation Dynamics with Ab Initio Electronic Structure Calculations J. Chem. Phys. 2008, 128, 124107
15. X Molecules in the Strong Field Regime J. Phys. Chem. A 2004, 108, 3162-3165
16. Centineo, G.; Fragala, I.; Bruno, G.; Spampinato, S. Photoelectron Spectroscopy of Benzophenone, Acetophenone and Their Ortho-Alkyl Derivatives J. Mol. Struct. 1978, 44, 203-210
17. Kobayashi, T.; Nagakura, S. Photoelectron Spectra of Substituted Benzenes Bull. Chem. Soc. Jpn. 1974, 47, 2563-2572
18. Wilson, K.; Yakovlev, V. Ultrafast Rainbow: Tunable Ultrashort Pulses from a Solid-State Kilohertz System J. Opt. Soc. Am. B 1997, 14, 444-448
19. Hankin, S. M.; Villeneuve, D. M.; Corkum, P. B.; Rayner, D. M. Intense-Field Laser Ionization Rates in Atoms and Molecules Phys. Rev. A 2001, 64, 013405
20. Shao, Y.; Molnar, L. F.; Jung, Y.; Kussmann, J.; Ochsenfeld, C.; Brown, S. T.; Gilbert, A. T. B.; Slipchenko, L. V.; Levchenko, S. V.; O'Neill, D. P. Advances in Methods and Algorithms in a Modern Quantum Chemistry Program Package Phys. Chem. Chem. Phys. 2006, 8, 3172-3191
21. Frisch, M. J.; Trucks, G. W.; Schlegel, H. B. GAUSSIAN 03; Gaussian, Inc.: Pittsburgh, PA, 2003.