AROMATIZATION OF PROPYLENE OVER HZSM-5: A DESIGN OF EXPERIMENTS (DOE) APPROACH

Chemical Engineering Communications

Volumn 200, Issue 8, 2013, Pages 1039-1056

  Fegade, Swapnil L ^a   Tande, Brian M ^a   Cho, Hyunwook ^a   Seames, Wayne S ^a   Sakodynskaya, Inna ^a   Muggli, Darrin S ^b   Kozliak, Evguenii I ^c  

^a University of North Dakota   (United States)

^b BENEDICTINE COLLEGE   (United States)

^c UNIVERSITY OF NORTH DAKOTA   (United States)

Author keywords

Aromatics; Aromatization; BTX; Design of experiments (DOE); Zeolite

Indexed keywords

AROMATICS; BENZENE AND TOLUENE; BTX; CATALYST CONCENTRATION; CONTINUOUS REACTORS; EFFECTS OF TEMPERATURE; EXPERIMENTAL STRATEGY; INTERACTION EFFECT;

ALUMINUM; AROMATIZATION; BENZENE; CATALYSTS; DESIGN OF EXPERIMENTS; SILICON; TOLUENE; XYLENE; ZEOLITES;

PROPYLENE;

EID: 84876112679     PISSN: 00986445     EISSN: 15635201     Source Type: Journal    
DOI: 10.1080/00986445.2012.737385     Document Type: Article

References (34)

1. Ancheyta-Juárez, J., and Villafuerte-Macías, E. (2000). Kinetic modeling of naphtha catalytic reforming reactions, Energy Fuels, 14 (5), 1032-1037.
2. Arzumanov, S. S., Gabrienko, A. A., Freude, D., and Stepanov, A. G. (2009). In situ high temperature MAS NMR study of the mechanisms of catalysis. Ethane aromatization on Zn-modified zeolite BEA, Solid State Nucl. Magn. Reson., 35 (2), 113-119.
3. Bhan, A., and Delgass, W. N. (2008). Propane aromatization over HZSM-5 and Ga/HZSM-5 catalysts, Catal. Rev.- Sci. Eng., 50 (1), 19-151.
4. Bhan, A., Joshi, Y. V., Delgass, W. N., and Thomson, K. T. (2003). DFT investigation of alkoxide formation from olefins in H-ZSM-5, J. Phys. Chem. B, 107 (38), 10476-10487.
5. Choudhary, T. V., Kinage, A., Banerjee, S., and Choudhary, V. R. (2006). Influence of Si/Ga and Si/Al ratios on propane aromatization over highly active H-GaAlMFI, Catal. Commun., 7 (3), 166-169.
6. Choudhary, V. R., and Devadas, P. (1997). Influence of space velocity on product selectivity and distribution of aromatics and xylenes in propane aromatization over H-GaMFI zeolite, J. Catal., 172 (2), 475-478.
7. 2 pretreated Ga-modified ZSM-5 type zeolite catalysts in propane aromatization, J. Catal., 158(1), 23-33.
8. Choudhary, V. R., Panjala, D., and Banerjee, S. (2002). Aromatization of propene and n-butene over H-galloaluminosilicate (ZSM-5 type) zeolite, Appl. Catal. A: Gen., 231 (1-2), 243-251.
9. 3, Stud. Surf. Sci. Catal., 46, 153-162.
10. Gonzales, N. O., Chakraborty, A. K., and Bell, A. T. (1998). A density functional theory study of the effects of metal cations on the Brønsted acidity of H-ZSM-5, Catal. Lett., 50 (3-4), 135-139.
11. Haw, J. F., Richardson, B. R., Oshiro, I. S., Lazo, N. D., and Speed, J. A. (1989). Reactions of propene on zeolite HY catalyst studied by in situ variable-temperature solid-state nuclear magnetic resonance spectroscopy, J. Am. Chem. Soc., 111 (6), 2052-2058.
12. Huang, M., and Kaliaguine, S. (1993). Propene aromatization over alkali-exchanged ZSM-5 zeolites, J. Molec. Catal., 81 (1), 37-49.
13. Krishnamurthy, G., Bhan, A., and Delgass, W. N. (2010). Identity and chemical function of gallium species inferred from microkinetic modeling studies of propane aromatization over Ga/HZSM-5 catalysts, J. Catal., 271 (2), 370-385.
14. Kwak, B. S., and Sachtler, W. M. H. (1996). Aromatization of propane over Zn/HZSM-5 catalysts prepared by chemical vapor deposition, Korean J. Chem. Eng., 13 (4), 356-363.
15. Kwak, B. S., Sachtler, W. M. H., and Haag, W. O. (1994). Catalytic conversion of propane to aromatics: Effects of adding Ga and/or Pt to HZSM-5, J. Catal., 149 (2), 465-473.
16. Lawson, J., and Erjavec, J. (2001). Modern Statistics for Engineering and Quality Improvement, Duxbury/Thomson Learning, Pacific Grove, Calif.
17. Lechert, H., Bezouhanova, C., Dimitrov, C., and Nenova, V. (1989). Intermediates in the formation of aromatics from propene and 2-propanol on H-ZSM-5 zeolites, Stud. Surf. Sci. Catal., 46, 91-98.
18. Lenth, R. V. (1989). Quick and easy analysis of unreplicated factorials, Technometrics, 31 (4), 469-473.
19. Liu, B., Yang, Y., and Sayari, A. (2001). Non-oxidative dehydroaromatization of methane over Ga-promoted Mo/HZSM-5-based catalysts, Appl. Catal. A: Gen., 214 (1), 95-102.
20. Lukyanov, D. B., Gnep, N. S., and Guisnet, M. R. (1994). Kinetic modeling of ethene and propene aromatization over HZSM-5 and GaHZSM-5, Ind. Eng. Chem. Res., 33 (2), 223-234.
21. Olah, G. A., and Molnár, Á. (2003). Hydrocarbon Chemistry, 2nd ed., Wiley-Interscience, Hoboken, NJ.
22. Rice, M. J., Chakraborty, A. K., and Bell, A. T. (1999). Al next nearest neighbor, ring occupation, and proximity statistics in ZSM-5, J. Catal., 186 (1), 222-227.
23. Rodrigues, M., Barre, M., Magnoux, P., Choudhary, V. R., and Guisnet, M. (1996). Coking, aging and regeneration of zeolites. XVIII Coking and deactivation of HZSM-5 and Ga/HZSM-5 catalysts during propene aromatization, J. Chim. Phys. Phys.-Chim. Biol., 93 (2), 317-330.
24. 27Al (multiquantum) magic angle spinning NMR study, J. Phys. Chem., 100 (50), 19223-19226.
25. Shen, X. C., Lou, H., Hu, K., and Zheng, X. M. (2007). Non-oxidative aromatization of C1 to C3 hydrocarbons over Pd-promoted Ga/HZSM-5 catalyst under mild conditions, Chin. Chem. Lett., 18 (4), 479-482.
26. Sillar, K., and Burk, P. (2004a). Computational study of vibrational frequencies of bridging hydroxyl groups in zeolite ZSM-5, Chem. Phys. Lett., 393 (4-6), 285-289.
27. Sillar, K., and Burk, P. (2004b). Hybrid quantum chemical and density functional theory (ONIOM) study of the acid sites in zeolite ZSM-5, J. Phys. Chem. B, 108(28), 9893-9899.
28. Smiešková, A., Rojasová, E., Hudec, P., and Šabo, L. (2004). Study of the role of Zn in aromatization of light alkanes with probe molecules, React. Kinet. Catal. Lett., 82 (2), 227-234.
29. Sun, Y., and Brown, T. C. (2002). Catalytic cracking, dehydrogenation, and aromatization of isobutane over Ga/HZSM-5 and Zn/HZSM-5 at low pressures, Int. J. Chem. Kinet., 34 (8), 467-480.
30. Tamunaidu, P., and Bhatia, S. (2007). Catalytic cracking of palm oil for the production of biofuels: Optimization studies, Bioresour. Technol., 98 (18), 3593-3601.
31. Van Bokhoven, J. A., Lee, T.-L., Drakopoulos, M., Lamberti, C., Thieß, S., and Zegenhagen, J. (2008). Determining the aluminium occupancy on the active T-sites in zeolites using X-ray standing waves, Nat. Mater., 7 (7), 551-555.
32. Viswanadham, N., Pradhan, A. R., Ray, N., Vishnoi, S. C., Shanker, U., and Prasada Rao, T. S. R. (1996). Reaction pathways for the aromatization of paraffins in the presence of H-ZSM-5 and Zn/H-ZSM-5, Appl. Catal. A: Gen., 137 (2), 225-233.
33. You, H. (2006). Influence of aromatization reaction conditions in the presence of HZSM-5 catalyst, Pet. Sci. Technol., 24 (6), 707-716.
34. Zhu, X., Liu, S., Song, Y., Xie, S., and Xu, L. (2005). Catalytic cracking of 1-butene to propene and ethene on MCM-22 zeolite, Appl. Catal. A: Gen., 290 (1-2), 191-199.