Real-time observation of surface bond breaking with an X-ray laser

Science

Volumn 339, Issue 6125, 2013, Pages 1302-1305

  Dell'Angela, M ^a   Anniyev, T ^b   Beye, M ^b,c   Coffee, R ^b   Fohlisch A ^c,d   Gladh, J ^e   Katayama, T ^b   Kaya, S ^b   Krupin, O ^b,f   LaRue, J ^b   Mogelhoj A ^g,h   Nordlund, D ⁱ   Norskov J K ^g,j   Oberg H ^e   Ogasawara, H ⁱ   Ostrom H ^e   Pettersson, L G M ^e   Schlotter, W F ^b   Sellberg, J A ^b,e   Sorgenfrei, F ^a   Turner, J J ^b   Wolf, M ^k   Wurth, W ^a   Nilsson, A ^b,e,g,i   more..

^a UNIVERSITY OF HAMBURG   (Germany)

^b SLAC NATIONAL ACCELERATOR LABORATORY   (United States)

^c HAHN MEITNER INSTITUT   (Germany)

^d UNIVERSITY OF POTSDAM   (Germany)

^e ALBANOVA UNIVERSITY CENTER   (Sweden)

^f EUROPEAN XFEL GMBH   (Germany)

^g European X Ray Free Electron Laser ^*  (United States)

^h TECHNICAL UNIVERSITY OF DENMARK   (Denmark)

ⁱ SLAC NATIONAL ACCELERATOR LABORATORY   (United States)

^j Stanford University   (United States)

^k FRITZ HABER INSTITUT DER MAX PLANCK GESELLSCHAFT   (Germany)

more..

Author keywords

[No Author keywords available]

Indexed keywords

CARBON MONOXIDE;

ADSORPTION; CARBON MONOXIDE; CHEMICAL BONDING; DESORPTION; ENTROPY; LASER; METAL; OBSERVATIONAL METHOD; REAL TIME; X-RAY SPECTROSCOPY;

ADSORPTION; ARTICLE; DENSITY FUNCTIONAL THEORY; DESORPTION; ENTROPY; FEMTOSECOND LASER; FLUORESCENCE SPECTROSCOPY; LASER; PRIORITY JOURNAL; SPECTROSCOPY; X RAY; X RAY ABSORPTION SPECTROSCOPY; X RAY EMISSION SPECTROSCOPY;

EID: 84874983375     PISSN: 00368075     EISSN: 10959203     Source Type: Journal    
DOI: 10.1126/science.1231711     Document Type: Article

References (27)

1. A. Cassuto, D. A. King, Surf. Sci. 102, 388 (1981).
2. D. J. Doren, J. C. Tully, Langmuir 4, 256 (1988).
3. P. Kisliuk, J. Phys. Chem. Solids 3, 95 (1957).
4. J. B. Taylor, I. Langmuir, Phys. Rev. 44, 423 (1933).
5. C. Frischkorn, M. Wolf, Chem. Rev. 106, 4207 (2006).
6. H. Arnolds, M. Bonn, Surf. Sci. Rep. 65, 45 (2010).
7. E. H. G. Backus, A. Eichler, A. W. Kleyn, M. Bonn, Science 310, 1790 (2005).
8. M. Bonn et al ., Phys. Rev. Lett. 84, 4653 (2000).
9. F. Fournier, W. Zheng, S. Carrez, H. Dubost, B. Bourguignon, J. Chem. Phys. 121, 4839 (2004).
10. I. M. Lane, D. A. King, Z. P. Liu, H. Arnolds, Phys. Rev. Lett. 97, 186105 (2006).
11. K. Inoue, K. Watanabe, Y. Matsumoto, J. Chem. Phys. 137, 024704 (2012).
12. Materials and methods, and supporting analysis of the experimental and theoretical data, are available as supplementary materials on Science Online
13. A. Föhlisch, W. Wurth, M. Stichler, C. Keller, A. Nilsson, J. Chem. Phys. 121, 4848 (2004).
14. A. Nilsson, L. G. M. Pettersson, Surf. Sci. Rep. 55, 49 (2004).
15. A. Nilsson et al ., Phys. Rev. Lett. 78, 2847 (1997).
16. A. Föhlisch et al., J. Chem. Phys. 112, 1946 (2000).
17. O. Björneholm et al., Phys. Rev. B 46, 10353 (1992).
18. L. Bartels, F. Wang, D. Möller, E. Knoesel, T. F. Heinz, Science 305, 648 (2004).
19. J. Wellendorff et al., Phys. Rev. B 85, 235149 (2012).
20. M. Dion, H. Rydberg, E. Schröder, D. C. Langreth, B. I. Lundqvist, Phys. Rev. Lett. 92, 246401 (2004).
21. H. Pfnür, P. Feulner, D. Menzel, J. Chem. Phys. 79, 4613 (1983).
22. D. J. Doren, J. C. Tully, J. Chem. Phys. 94, 8428 (1991).
23. C. Keller et al., Phys. Rev. Lett. 80, 1774 (1998).
24. P. Skytt et al ., Phys. Rev. A 55, 134 (1997).
25. Y. R. Shen, Principles of Non-Linear Optics (Wiley-Interscience, New York, 2003)
26. J. H. Hunt, P. Guyot-Sionnest, Y. R. Shen, Chem. Phys. Lett. 133, 189 (1987).
27. I. Chorkendorf, H. Niemantsverdriet, Concepts of Modern Catalysis and Kinetics (Wiley-VCH, Weinheim, Germany, 2003).