Unraveling quantum pathways using optical 3D Fourier-transform spectroscopy

Nature Communications

Volumn 4, Issue , 2013, Pages

  Li, Hebin ^a   Bristow, Alan D ^a,b   Siemens, Mark E ^a,c   Moody, Galan ^a   Cundiff, Steven T ^a  

^a UNIVERSITY OF COLORADO   (United States)

^b WEST VIRGINIA UNIVERSITY   (United States)

^c UNIVERSITY OF DENVER   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

POTASSIUM;

EXPERIMENTAL STUDY; FTIR SPECTROSCOPY; NONLINEARITY; PARTICULATE MATTER; QUANTUM MECHANICS; THREE-DIMENSIONAL MODELING;

ABSORPTION SPECTROSCOPY; ARTICLE; ATOM; DIPOLE; INFRARED SPECTROSCOPY; LASER; QUANTUM CHEMISTRY;

EID: 84873027206     PISSN: None     EISSN: 20411723     Source Type: Journal    
DOI: 10.1038/ncomms2405     Document Type: Article

References (45)

1. Brumer, P. & Shapiro, M. Control of unimolecular reactions using coherent-light. Chem. Phys. Lett. 126, 541-546 (1986).
2. Warren, W. S., Rabitz, H. & Dahleh, M. Coherent control of quantum dynamics-the dream is alive. Science 259, 1581-1589 (1993).
3. Potter, E. D., Herek, J. L., Pedersen, S., Liu, Q. & Zewail, A. H. Femtosecond laser control of a chemical reaction. Nature 355, 66-68 (1992).
4. Zhu, L. C. et al. Coherent laser control of the product distribution obtained in the photoexcitation of HI. Science 270, 77-80 (1995).
5. Assion, A. et al. Control of chemical reactions by feedback-optimized phase-shaped femtosecond laser pulses. Science 282, 919-922 (1998). (Pubitemid 28507518)
6. Meshulach, D. & Silberberg, Y. Coherent quantum control of two-photon transitions by a femtosecond laser pulse. Nature 396, 239-242 (1998). (Pubitemid 28541382)
7. Weinacht, T. C., Ahn, J. & Bucksbaum, P. H. Controlling the shape of a quantum wavefunction. Nature 397, 233-235 (1999).
8. Bartels, R. et al. Shaped-pulse optimization of coherent emission of high-harmonic soft X-rays. Nature 406, 164-166 (2000). (Pubitemid 30468992)
9. Herek, J. L., Wohlleben, W., Cogdell, R. J., Zeidler, D. & Motzkus, M. Quantum control of energy flow in light harvesting. Nature 417, 533-535 (2002). (Pubitemid 34595916)
10. Costa, L., Betz, M., Spasenovic, M., Bristow, A. D. & Van Driel, H. M. All-optical injection of ballistic electrical currents in unbiased silicon. Nat. Phys. 3, 632-635 (2007).
11. Voss, T., Rückmann, I., Gutowski, J., Axt, V. M. & Kuhn, T. Coherent control of the exciton and exciton-biexciton transitions in the generation of nonlinear wave-mixing signals in a semiconductor quantum well. Phys. Rev. B 73, 115311 (2006).
12. Bonadeo, N. H. et al. Coherent optical control of the quantum state of a single quantum dot. Science 282, 1473-1476 (1998). (Pubitemid 28538605)
13. Judson, R. S. & Rabitz, H. Teaching lasers to control molecules. Phys. Rev. Lett. 68, 1500-1503 (1992).
14. Rabitz, H., de Vivie-Riedle, R., Motzkus, M. & Kompa, K. Chemistry-whither the future of controlling quantum phenomena? Science 288, 824-828 (2000). (Pubitemid 30257723)
15. Zeidler, D., Frey, S., Kompa, K.-L. & Motzkus, M. Evolutionary algorithms and their application to optimal control studies. Phys. Rev. A 64, 023420 (2001).
16. Scully, M. O. & Zubairy, M. S. Quantum Optics (Cambridge University Press, 1997).
17. Rydberg, R. Graphische Darstellung einiger Bandenspektroskopischer Ergebnisse. Z. Phys. 73, 376-385 (1932).
18. Klein, O. Zur Berechnung von Potentialkurven für zweiatomige Moleküle mit hilfe von Spektraltermen. Z. Phys. 76, 226-235 (1932).
19. Rees, A. The calculation of potential-energy curves from band-spectroscopic data. Proc. Phys. Soc. London 59, 998-1008 (1947).
20. Geremia, J. M. & Rabitz, H. Optimal identification of Hamiltonian information by closed-loop laser control of quantum systems. Phys. Rev. Lett. 89, 263902 (2002).
21. Branderhorst, M. P. A. et al. Coherent control of decoherence. Science 320, 638-643 (2008). (Pubitemid 351934118)
22. Brixner, T. et al. Two-dimensional spectroscopy of electronic couplings in photosynthesis. Nature 434, 625-628 (2005). (Pubitemid 40488551)
23. Cundiff, S. T., Zhang, T. H., Bristow, A. D., Karaiskaj, D. & Dai, X. C. Optical two-dimensional Fourier transform spectroscopy of semiconductor quantum wells. Acc. Chem. Res. 42, 1423-1432 (2009).
24. Moody, G. et al. Exciton-exciton and exciton-phonon interactions in an interfacial GaAs quantum dot ensemble. Phys. Rev. B 83, 115324 (2011).
25. xAs quantum well and quantum dot ensemble. Phys. Rev. B 83, 245316 (2011).
26. Ernst, R., Bodenhausen, G. & Wokaun, A. Principles of Nuclear Magnetic Resonance in One and Two Dimensions (Oxford Science Publications, 1987).
27. Clore, G. M. & Gronenborn, A. M. Structures for larger proteins in solution: three-and four-dimensional heteronuclear NMR spectroscopy. Science 252, 1390-1399 (1991). (Pubitemid 21917051)
28. Siemens, M. E., Moody, G., Li, H., Bristow, A. D. & Cundiff, S. T. Resonance lineshapes in two-dimensional Fourier transform spectroscopy. Opt. Express 18, 17699-17708 (2010).
29. Khalil, M., Demirdoven, N. & Tokmakoff, A. Vibrational coherence transfer characterized with Fourier-transform 2D IR spectroscopy. J. Chem. Phys. 121, 362-373 (2004).
30. Engel, G. S. et al. Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems. Nature 446, 782-786 (2007). (Pubitemid 46582029)
31. Collini, E. et al. Coherently wired light-harvesting in photosynthetic marine algae at ambient temperature. Nature 463, 644-647 (2010).
32. Turner, D. B., Stone, K. W., Gundogdu, K. & Nelson, K. A. Three-dimensional electronic spectroscopy of excitons in GaAs quantum wells. J. Chem. Phys. 131, 144510 (2009).
33. Ding, F. & Zanni, M. T. Heterodyned 3D IR spectroscopy. Chem. Phys. 341, 95-105 (2007).
34. Garrett-Roe, S. & Hamm, P. Purely absorptive three-dimensional infrared spectroscopy. J. Chem. Phys. 130, 164510 (2009).
35. Fidler, A. F., Harel, E. & Engel, G. S. Dissecting hidden couplings using fifth-order three-dimensional electronic spectroscopy. J. Phys. Chem. Lett. 1, 2876-2880 (2010).
36. Garrett-Roe, S., Perakis, F., Rao, F. & Hamm, P. Three-dimensional infrared spectroscopy of isotope-substituted liquid water reveals heterogeneous dynamics. J. Phys. Chem. B 115, 6976-6984 (2011).
37. Yang, L., Zhang, T., Bristow, A. D., Cundif, S. T. & Mukamel, S. Isolating excitonic Raman coherence in semiconductors using two-dimensional correlation spectroscopy. J. Chem. Phys. 129, 234711 (2008).
38. Dai, X., Bristow, A. D., Karaiskaj, D. & Cundiff, S. T. Two-dimensional Fourier-transform spectroscopy of potassium vapor. Phys. Rev. A 82, 052503 (2010).
39. Li, X., Zhang, T., Borca, C. N. & Cundiff, S. T. Many-body interactions in semiconductors probed by optical two-dimensional Fourier transform spectroscopy. Phys. Rev. Lett. 96, 057406 (2006).
40. Chemla, D. S. & Shah, J. Many-body and correlation effects in semiconductors. Nature 411, 549-557 (2001). (Pubitemid 32531394)
41. Bloch, I., Dalibard, J. & Zwerger, W. Many-body physics with ultracold gases. Rev. Mod. Phys. 80, 885-964 (2008).
42. Bristow, A. D. et al. A versatile ultrastable platform for optical multidimensional Fourier-transform spectroscopy. Rev. Sci. Inst. 80, 073108 (2009).
43. DeCamp, M. F. & Tokmakoff, A. Single-shot two-dimensional spectrometer. Opt. Lett. 31, 113-115 (2006). (Pubitemid 43133298)
44. Seber, G. A. F. & Wild, C. J. Nonlinear Regression (John Wiley & Sons, Inc., 2003).
45. Nesmeyanov, A. N. Vapour Pressure of the Chemical Elements (Elsevier, 1963).