Ion-pair or ion-cloud relaxation? on the origin of small-amplitude low-frequency relaxations of weakly associating aqueous electrolytes

Journal of Molecular Liquids

Volumn 176, Issue , 2012, Pages 52-59

  Eiberweiser, Andreas ^a   Buchner, Richard ^a  

^a UNIVERSITY OF REGENSBURG   (Germany)

Author keywords

Dielectric relaxation; Ion association; Ion hydration; Ion cloud relaxation; Sodium chloride

Indexed keywords

AQUEOUS ELECTROLYTE; ASSOCIATION CONSTANT; ELECTROLYTE SOLUTIONS; INFINITE DILUTION; ION ASSOCIATION; ION HYDRATION; ION PAIRS; ION-CLOUD RELAXATION; LOW CONCENTRATIONS; LOW-FREQUENCY RELAXATION; NACL SOLUTION; SALT CONCENTRATION; WATER DYNAMICS; WATER MOLECULE; WIDE FREQUENCY RANGE;

DIELECTRIC RELAXATION; ELECTROLYTES; SODIUM CHLORIDE;

IONS;

EID: 84870513660     PISSN: 01677322     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.molliq.2012.03.025     Document Type: Conference Paper

References (66)

1. P. Debye, and E. Hückel Physikalische Zeitschrift 24 1923 185
2. Y. Marcus, and G. Hefter Chemical Reviews 106 2006 4585
3. J.S. Fritz, and D.T. Gjerde Ion chromatography 2009 Wiley-VCH Weinheim
4. S. Zugmann, M. Fleischmann, M. Amereller, R.M. Gschwind, M. Winter, and H.J. Gores Journal of Chemical and Engineering Data 56 2011 4786
5. M. Makosza Pure and Applied Chemistry 72 2000 1399
6. K. Iti, E.-M. Schön, J. Bachl, D. Kühbeck, C. Cativiela, S. Saha, R. Banerjee, S. Roelens, J.J. Marrero-Tellado, and D. Díaz Díaz Soft Matter 8 2012 3446
7. K.J. Powell, P.L. Brown, R.H. Byrne, T. Gajda, G. Hefter, A.-K. Leuz, S. Sjöberg, and H. Wanner Pure and Applied Chemistry 83 2011 1163
8. C.J. Fennell, A. Bizjak, V. Vlachy, and K.A. Dill The Journal of Physical Chemistry. B 113 2009 6782
9. R. Buchner, and G. Hefter Physical Chemistry Chemical Physics 11 2009 8984
10. K.D. Collins Biophysical Chemistry 119 2006 271
11. B. Jagoda-Cwiklik, R. Vácha, M. Lund, M. Srebro, and P. Jungwirth The Journal of Physical Chemistry. B 111 2007 14077
12. P. Ganguly, P. Schravendijk, B. Hess, and N.F.A. van der Vegt The Journal of Physical Chemistry. B 115 2011 3734
13. M. Eigen, and K. Tamm Zeitschrift für Elektrochemie 66 1962 93 & 107
14. A. Płaczek, G. Hefter, H.M.A. Rahman, and R. Buchner The Journal of Physical Chemistry. B 115 2011 2234
15. F. Kremer, and A. Schönhals Broadband dielectric spectroscopy 2003 Springer Berlin
16. C. Böttcher, and P. Bordewijk Theory of electrical polarization vol. 2 1978 Elsevier Amsterdam
17. T. Chen, G. Hefter, and R. Buchner The Journal of Physical Chemistry A 107 2003 4025
18. W. Wachter, W. Kunz, R. Buchner, and G. Hefter The Journal of Physical Chemistry A 109 2005 8675
19. M.V. Fedotova, S.E. Kruchinin, H.M.A. Rahman, and R. Buchner Journal of Molecular Liquids 159 2011 9
20. H.M.A. Rahman, G. Hefter, and R. Buchner The Journal of Physical Chemistry. B 116 2012 314
21. R.H. Cole Annual Review of Physical Chemistry 40 1989 1
22. P. Debye, and H. Falkenhagen Physikalische Zeitschrift 29 1928 121
23. F. Carrique, E. Ruiz-Reina, F.J. Arroyo, and A.V. Delgado The Journal of Physical Chemistry. B 114 2010 6134
24. F. Bordi, C. Cametti, and R.H. Colby Journal of Physics. Condensed Matter 16 2004 R1423
25. R. Buchner, C. Baar, P. Fernandez, S. Schrödle, and W. Kunz Journal of Molecular Liquids 118 2005 179
26. J.E. Anderson Journal of Non-Crystalline Solids 172-174 1994 1190
27. T. Yamaguchi, T. Matsuoka, and S. Koda The Journal of Chemical Physics 130 2009 094506
28. R. Buchner, G.T. Hefter, and P.M. May The Journal of Physical Chemistry A 103 1999 1
29. S. Schrödle, G. Hefter, W. Kunz, and R. Buchner Langmuir 22 2006 924
30. J. Barthel, R. Buchner, P.N. Eberspächer, M. Münsterer, J. Stauber, and B. Wurm Journal of Molecular Liquids 78 1998 82
31. ELectrolyte DAta Regensburg is a subset of the database DETHERM(distributor: STN, Karlsruhe, Germany).
32. A.P. Gregory, and R.N. Clarke Measurement Science and Technology 18 2007 1372
33. P.R. Bevington Data reduction and error analysis for the physical sciences 1969 McGraw-Hill New York
34. A.Y. Zasetsky, and R. Buchner Journal of Physics. Condensed Matter 23 2011 025903
35. T. Fukasawa, T. Sato, J. Watanabe, Y. Hama, W. Kunz, and R. Buchner Physical Review Letters 95 2005 197802
36. S. Schrödle, Ph.D. thesis, Regensburg, 2005.
37. W. Wachter, R. Buchner, and G. Hefter The Journal of Physical Chemistry. B 110 2006 5147
38. W. Wachter, S. Fernandez, R. Buchner, and G. Hefter The Journal of Physical Chemistry. B 111 2007 9010
39. U. Kaatze Chemical Physics Letters 203 1993 1
40. J. Barthel, R. Buchner, C.G. Hölzl, and M. Münsterer Zeitschrift für Physikalische Chemie 214 2000 1213
41. J.L. Dote, and D. Kivelson The Journal of Physical Chemistry 87 1983 3889
42. S.H. Glarum The Journal of Chemical Physics 33 1960 1371
43. J. Barthel, H. Hetzenauer, and R. Buchner Berichte der Bunsengesellschaft für Physikalische Chemie 96 1992 1424
44. J.H. Gibbs, C. Cohen, P.D. Fleming III, and H. Porosoff The physical chemistry of aqueous systems 1973 Plenum New York
45. Y. Marcus Ion properties 1997 Marcel Dekker New York
46. L. Korson, W. Drost-Hansen, and F.J. Millero The Journal of Physical Chemistry 73 1969 34
47. R. Buchner Pure and Applied Chemistry 80 2008 1239
48. J.B. Hasted, and F. Franks Water, a comprehensive treatise Vol. 1 1972 Plenun New York
49. J.F. Zemaitis Jr., D.M. Clark, M. Rafal, and N.C. Scrivner Handbook of aqueous electrolyte thermodynamics: theory and application 1986 American Institute of Chemical Engineers New York
50. R.M. Fuoss Proceedings of the National Academy of Sciences of the United States of America 77 1980 34
51. M. Bešter-Rogač, R. Neueder, and J. Barthel Journal of Solution Chemistry 28 1999 1071
52. D. Laage, and J.T. Hynes Proceedings of the National Academy of Sciences of the United States of America 104 2007 11167
53. K. Yui, M. Sakuma, and T. Funazukuri Fluid Phase Equilibria 297 2010 227
54. B. Hess, and N.F.A. van der Vegt Proceedings of the National Academy of Sciences of the United States of America 106 2009 13296
55. J. Hunger, A. Stoppa, R. Buchner, and G. Hefter The Journal of Physical Chemistry. B 112 2008 12913
56. J. Sangoro, C. Iacob, A. Serghei, S. Naumov, P. Galvosas, J. Kärger, C. Wespe, F. Bordusa, A. Stoppa, J. Hunger, R. Buchner, and F. Kremer The Journal of Chemical Physics 128 2008 214509
57. T. Yamaguchi, Personal communication.
58. R. Mancinelli, A. Botti, F. Bruni, and M.A. Ricci The Journal of Physical Chemistry. B 111 2007 13570
59. H. Falkenhagen, and W. Ebeling Theorie der Elektrolyte 1971 S. Hirzel Leipzig
60. T. Yamaguchi, T. Matsuoka, and S. Koda The Journal of Chemical Physics 127 2007 234501
61. R. Leonard Technical report 1, Office of Naval Research Contract N6-onr-27507 1950 University of California Los Angeles
62. K.G. Breitschwerdt, and H. Kistenmacher The Journal of Chemical Physics 56 1972 4800
63. I.A. Heisler, K. Mazur, and S.R. Meech The Journal of Physical Chemistry. B 115 2011 1863
64. A. Tongraar, and B.M. Rode Chemical Physics Letters 385 2004 378
65. J.A. White, E. Schwegler, G. Galli, and F. Gygi The Journal of Chemical Physics 113 2000 4668
66. A. Tongraar, K.R. Liedl, and B.M. Rode The Journal of Physical Chemistry A 102 1998 10340