How does deposition of gas phase species affect pH at frozen salty interfaces?

Atmospheric Chemistry and Physics

Volumn 12, Issue 21, 2012, Pages 10065-10073

  Wren, S N ^a   Donaldson, D J ^a  

^a UNIVERSITY OF TORONTO   (Canada)

Author keywords

[No Author keywords available]

Indexed keywords

AIR-ICE INTERACTION; ATMOSPHERIC CHEMISTRY; ATMOSPHERIC DEPOSITION; ATMOSPHERIC GAS; BROMINE; PH; SALT WATER; SEA ICE;

EID: 84868674205     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-12-10065-2012     Document Type: Article

References (52)

1. Abbatt, J. P. D., Thomas, J. L., Abrahamsson, K., Boxe, C., Gran-fors, A., Jones, A. E., King, M. D., Saiz-Lopez, A., Shep-son, P. B., Sodeau, J., Toohey, D. W., Toubin, C., von Glasow, R., Wren, S. N., and Yang, X.: Halogen activation via interactions with environmental ice and snow in the polar lower troposphere and other regions, Atmos. Chem. Phys., 12, 6237-6271, doi:10.5194/acp-12-6237-2012, 2012.
2. Adams, J. W., Holmes, N. S., and Crowley, J. N.: Uptake and reaction of HOBr on frozen and dry NaCl/NaBr surfaces between 253 and 233K, Atmos. Chem. Phys., 2, 79-91, doi:10.5194/acp-2-79-2002, 2002.
3. Alvarez-Aviles, L., Simpson, W. R., Douglas, T. A., Sturm, M., Perovich, D., and Domine, F.: Frost flower chemical composition during growth and its implications for aerosol production and bromine activation, J. Geophys. Res. Atmos., 113, 21304, doi:10.1029/2008JD010277, 2008.
4. Balon, M., Hidalgo, J., Guardado, P., Munoz, M. A., and Car-mona, C.: Acid-base and spectral properties of beta-carbolines-1. Tetrahydro-beta- carbolines, J. Chem. Soc. Perkin Trans. 2, 91-97, 1993.
5. Bock, J. and Jacobi, H. W.: Development of a mechanism for nitrate photochemistry in snow, J. Phys. Chem. A, 114, 1790-1796, 2010.
6. Cho, H., Shepson, P. B., Barrie, L. A., Cowin, J. P., and Zaveri, R.: NMR investigation of the quasi-brine layer in ice/brine mixtures, J. Phys. Chem. B, 106, 11226-11232, 2002. (Pubitemid 35313761)
7. Clegg, S. L. and Brimblecombe, P.: Solubility of ammonia in pure aqueous and multicomponent solutions, J. Phys. Chem., 93, 7237-7248, 1989.
8. Clifford, D. and Donaldson, D. J.: Direct experimental evidence for a heterogeneous reaction of ozone with bromide at the air-aqueous interface, J. Phys. Chem. A, 111, 9809-9814, 2007. (Pubitemid 47598287)
9. Clifford, D., Bartels-Rausch, T., and Donaldson, D. J.: Suppression of aqueous surface hydrolysis by monolayers of short chain organic amphiphiles, Phys. Chem. Chem. Phys., 9, 1363-1369, 2007.
10. Delzeit, L., Rowland, B., and Devlin, J. P.: Infrared-spectra of HCl complexed ionized in amorphous hydrates and at ice surfaces in the 15-90-K range, J. Phys. Chem., 97, 10312-10318, 1993.
11. Dias, A., Varela, A. P., Miguel, M. D., Becker, R. S., Burrows, H. D., and Macanita, A. L.: Beta-carbolines-2. Rate constants of proton transfer from multiexponential decays in the lowest singlet excited state of harmine in water as a function of pH, J. Phys. Chem., 100, 17970-17977, 1996. (Pubitemid 126790078)
12. Dibb, J. E., Arsenault, M., Peterson, M. C., and Honrath, R. E.: Fast nitrogen oxide photochemistry in summit, greenland snow, Atmos. Environ., 36, 2501-2511, 2002. (Pubitemid 34628345)
13. Dieckmann, G. S., Nehrke, G., Papadimitriou, S., Goettlicher, J., Steininger, R., Kennedy, H., Wolf-Gladrow, D., and Thomas, D. N.: Calcium carbonate as ikaite crystals in antarctic sea ice, Geophys. Res. Lett., 35, 08501, doi:10.1029/2008GL033540, 2008.
14. 2O) discovered in arctic sea ice, Cryosphere, 4, 227-230, doi:10.5194/tc-4-227-2010, 2010.
15. Domine, F. and Shepson, P. B.: Air-snow interactions and atmospheric chemistry, Science, 297, 1506-1510, 2002. (Pubitemid 34970989)
16. Doppenschmidt, A., and Butt, H. J.: Measuring the thickness of the liquid-like layer on ice surfaces with atomic force microscopy, Langmuir, 16, 6709-6714, 2000.
17. Fan, S. M. and Jacob, D. J.: Surface ozone depletion in arctic spring sustained by bromine reactions on aerosols, Nature, 359, 522-524, 1992. (Pubitemid 23374550)
18. Fickert, S., Adams, J. W., and Crowley, J. N.: Activation of Br-2 and BrCl via uptake of HOBr onto aqueous salt solutions, J. Geophys. Res. Atmos., 104, 23719-23727, 1999.
19. Grannas, A. M., Jones, A. E., Dibb, J., Ammann, M., Anastasio, C., Beine, H. J., Bergin, M., Bottenheim, J., Boxe, C. S., Carver, G., Chen, G., Crawford, J. H., Domine, F., Frey, M. M., Guzman, M. I., Heard, D. E., Helmig, D., Hoffmann, M. R., Honrath, R. E., Huey, L. G., Hutterli, M., Jacobi, H. W., Klan, P., Lefer, B., McConnell, J., Plane, J., Sander, R., Savarino, J., Shepson, P. B., Simpson, W. R., Sodeau, J. R., von Glasow, R., Weller, R., Wolff, E. W., and Zhu, T.: An overview of snow photochemistry: Evidence, mechanisms and impacts, Atmos. Chem. Phys., 7, 4329-4373, doi:10.5194/acp-7-4329-2007, 2007. (Pubitemid 47325999)
20. 2O solid-phase vapor-pressures and HCl solubility in ice, J. Phys. Chem., 94, 4700-4705, 1990.
21. Heger, D., Jirkovsky, J., and Klan, P.: Aggregation of methylene blue in frozen aqueous solutions studied by absorption spec-troscopy, J. Phys. Chem. A, 109, 6702-6709, 2005. (Pubitemid 41156862)
22. 3 above the snowpack at Summit, Greenland, Atmos. Environ., 36, 2629-2640, 2002. (Pubitemid 34628356)
23. Kahan, T. F. and Donaldson, D. J.: Photolysis of polycyclic aromatic hydrocarbons on water and ice surfaces, J. Phys. Chem. A, 111, 1277-1285, 2007. (Pubitemid 46384223)
24. Kahan, T. F. and Donaldson, D. J.: Benzene photolysis on ice: Implications for the fate of organic contaminants in the winter, Environ. Sci.Technol., 44, 3819-3824, 2010.
25. Kahan, T. F., Reid, J. P., and Donaldson, D. J.: Spectroscopic probes of the quasi-liquid layer on ice, J. Phys. Chem. A, 111, 11006-11012, 2007. (Pubitemid 350097557)
26. Kahan, T. F., Kwamena, N. O. A., and Donaldson, D. J.: Different photolysis kinetics at the surface of frozen freshwater vs. frozen salt solutions, Atmos. Chem. Phys., 10, 10917-10922, doi:10.5194/acp-10-10917-2010, 2010a.
27. Kahan, T. F., Zhao, R., and Donaldson, D. J.: Hydroxyl radical reactivity at the air-ice interface, Atmos. Chem. Phys., 10, 843-854, doi:10.5194/acp-7- 10-843-2007, 2010b.
28. Kahan, T. F., Zhao, R., Jumaa, K. B., and Donaldson, D. J.: Anthracene photolysis in aqueous solution and ice: Photon flux dependence and comparison of kinetics in bulk ice and at the air-ice interface, Environ. Sci. Tech., 44, 1302-1306, 2010c.
29. Kang, H., Shin, T. H., Park, S. C., Kim, I. K., and Han, S. J.: Acidity of hydrogen chloride on ice, J. Am. Chem. Soc., 122, 9842-9843, 2000.
30. Koop, T., Kapilashrami, A., Molina, L. T., and Molina, M. J.: Phase transitions of sea-salt/water mixtures at low temperatures: Implications for ozone chemistry in the polar marine boundary layer, J. Geophys. Res. Atmos., 105, 26393-26402, 2000. (Pubitemid 32109127)
31. Kuo, M. H., Moussa, S. G., and McNeill, V. F.: Modeling interfa-cial liquid layers on environmental ices, Atmos. Chem. Phys, 11, 9971-9982, doi:10.5194/acp-11-9971-2011, 2011.
32. 2: A key role for hydrates in the kinetics and mechanism, J. Phys. Chem. A, 101, 1277-1286, 1997. (Pubitemid 127585149)
33. Li, Y. and Somorjai, G. A.: Surface premelting of ice, J. Phys. Chem. C, 111, 9631-9637, 2007. (Pubitemid 47155143)
34. Liyana-Arachchi, T. P., Valsaraj, K. T., and Hung, F. R.: Molecular simulation study of the adsorption of naphthalene and ozone on atmospheric air/ice interfaces, J. Phys. Chem. A, 115, 9226-9236, 2011.
35. McNeill, V. F., Loerting, T., Geiger, F. M., Trout, B. L., and Molina, M. J.: Hydrogen chloride-induced surface disordering on ice, Proc. Natl. Acad. Sci., 103, 9422-9427, 2006. (Pubitemid 43955841)
36. Mmereki, B. T. and Donaldson, D. J.: Laser induced fluorescence of pyrene at an organic coated air-water interface, Phys. Chem. Chem. Phys., 4, 4186-4191, 2002.
37. Molina, M. J., Tso, T. L., Molina, L. T., and Wang, F. C. Y.: Antarctic stratospheric chemistry of chlorine nitrate, hydrogen-chloride and ice-release of active chlorine, Science, 238, 1253-1257, 1987.
38. Molina, M. J. The Chemistry of the Atmosphere: The Impact of Global Change, Blackwell Scientific Publications: Boston, Chapter 3, 27-38, 1994
39. Morin, S., Marion, G. M., von Glasow, R., Voisin, D., Bouchez, J., and Savarino, J.: Precipitation of salts in freezing seawater and ozone depletion events: A status report, Atmos. Chem. Phys, 8, 7317-7324, doi:10.5194/acp-8- 7317-2008, 2008.
40. Oldridge, N. W. and Abbatt, J. P. D.: Formation of gas-phase bromine from interaction of ozone with frozen and liquid NaCl/NaBr solutions: Quantitative separation of surficial chemistry from bulk-phase reaction, J. Phys. Chem. A, 115, 2590-2598, 2011.
41. 3 with seawa-ter ice, Geophys. Res. Lett., 25, 3923-3926, 1998. (Pubitemid 29094473)
42. Parent, P. and Laffon, C.: Adsorption of HCl on the water ice surface studied by X-ray absorption spectroscopy, J. Phys. Chem. B, 109, 1547-1553, 2005. (Pubitemid 40219541)
43. Park, S. C. and Kang, H.: Adsorption, ionization, and migration of hydrogen chloride on ice films at temperatures between 100 and 140K, J. Phys. Chem. B, 109, 5124-5132, 2005. (Pubitemid 40407734)
44. Sander, R., Burrows, J., and Kaleschke, L.: Carbonate precipitation in brine-a potential trigger for tropospheric ozone depletion events, Atmos. Chem. Phys., 6, 4653-4658, doi:10.5194/acp-6-4653-2006, 2006. (Pubitemid 44600870)
45. Simpson, W. R., von Glasow, R., Riedel, K., Anderson, P., Ariya, P., Bottenheim, J., Burrows, J., Carpenter, L. J., Friess, U., Good-site, M. E., Heard, D., Hutterli, M., Jacobi, H. W., Kaleschke, L., Neff, B., Plane, J., Platt, U., Richter, A., Roscoe, H., Sander, R., Shepson, P., Sodeau, J., Steffen, A., Wagner, T., and Wolff, E.: Halogens and their role in polar boundary-layer ozone depletion, Atmos. Chem. Phys., 7, 4375-4418, doi:10.5194/acp-7-4375-2007, 2007. (Pubitemid 47325998)
46. Sjostedt, S. J. and Abbatt, J. P. D.: Release of gas-phase halogens from sodium halide substrates: Heterogeneous oxidation of frozen solutions and desiccated salts by hydroxyl radicals, Environ. Res. Lett., 3, 045007, doi:10.1088/1748-9326/3/4/045007, 2008.
47. Thibert, E. and Domine, F.: Thermodynamics and kinetics of the solid solution of hcl in ice, J. Phys. Chem. B, 101, 3554-3565, 1997. (Pubitemid 127611910)
48. Wei, X., Miranda, P. B., Zhang, C., and Shen, Y. R.: Sum-frequency spectroscopic studies of ice interfaces, Phys. Rev. B, 66, 085401, doi:10.1103/PhysRevB.66.085401, 2002.
49. Wolff, E. W., Mulvaney, R., and Oates, K.: Diffusion and location of hydrochloric-acid in ice-implications for polar stratospheric clouds and ozone depletion, Geophys. Res. Lett., 16, 487-490, 1989. (Pubitemid 19207963)
50. Wren, S. N. and Donaldson, D. J.: Laboratory study of ph at the air-ice interface, J. Phys. Chem. C, 116, 10171-10180, 2012.
51. 3(g) and halides at the surface of frozen salt solutions, J. Geophys. Res. Atmos., 115, 16309, doi:10.1029/2010JD013929, 2010.
52. Zhou, X. L., Beine, H. J., Honrath, R. E., Fuentes, J. D., Simpson, W., Shepson, P. B., and Bottenheim, J. W.: Snowpack photochemical production of HONO: A major source of OH in the arctic boundary layer in springtime, Geophys. Res. Lett., 28, 4087-4090, 2001. (Pubitemid 33124728)