Understanding the solvent effect on the catalytic oxidation of 1,4-butanediol in methanol over Au/TiO 2 catalyst: NMR diffusion and relaxation studies

Chemistry - A European Journal

Volumn 18, Issue 45, 2012, Pages 14426-14433

  D'Agostino, Carmine ^a   Brett, Gemma L ^b   Miedziak, Peter J ^b   Knight, David W ^b   Hutchings, Graham J ^b   Gladden, Lynn F ^a   Mantle, Mick D ^a  

^a UNIVERSITY OF CAMBRIDGE   (United Kingdom)

^b CARDIFF UNIVERSITY   (United Kingdom)

Author keywords

adsorption; diffusion; heterogeneous catalysis; NMR spectroscopy; solvent effects

Indexed keywords

1 ,4-BUTANEDIOL; ADSORPTION STRENGTH; CATALYST SURFACES; CATALYTIC REACTIONS; CATALYTIC SITES; CATALYTIC SYSTEM; DIFFUSION RATE; DIMETHYL SUCCINATE; EFFECT OF WATER; EFFECTIVE DIFFUSION; NMR DIFFUSION; NMR RELAXATION; PFG-NMR; PRESENCE OF WATER; PULSED-FIELD GRADIENTS; REACTANT MOLECULES; RELAXATION MEASUREMENTS; RELAXATION STUDIES; SELF-DIFFUSIVITY; SOLVENT EFFECTS; SURFACE INTERACTIONS; WATER ADDITION;

ADSORPTION; CATALYSIS; CATALYTIC OXIDATION; DIFFUSION; METHANOL; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; ORGANIC SOLVENTS; REACTION RATES;

CATALYSTS;

EID: 84868014788     PISSN: 09476539     EISSN: 15213765     Source Type: Journal    
DOI: 10.1002/chem.201201922     Document Type: Article

References (40)

1. G. J. Hutchings, J. Catal. 1985, 96, 292-295.
2. M. Haruta, T. Kobayashi, H. Sano, N. Yamada, Chem. Lett. 1987, 405-408.
3. L. McEwan, M. Julius, S. Roberts, J. C. Q. Fletcher, Gold Bull. 2010, 43, 298-306.
4. G. J. Hutchings, M. Haruta, Appl. Catal. A 2005, 291, 2-5.
5. A. I. Kozlov, A. P. Kozlova, H. C. Liu, Y. Iwasawa, Appl. Catal. A 1999, 182, 9-28.
6. D. I. Enache, J. K. Edwards, P. Landon, B. Solsona-Espriu, A. F. Carley, A. A. Herzing, M. Watanabe, C. J. Kiely, D. W. Knight, G. J. Hutchings, Science 2006, 311, 362-365.
7. T. Hayashi, T. Inagaki, N. Itayama, H. Baba, Catal. Today 2006, 117, 210-213.
8. I. S. Nielsen, E. Taarning, K. Egeblad, R. Madsen, C. H. Christensen, Catal. Lett. 2007, 116, 35-40.
9. E. Taarning, A. T. Madsen, J. M. Marchetti, K. Egeblad, C. H. Christensen, Green Chem. 2008, 10, 408-414.
10. N. Dimitratos, J. A. Lopez-Sanchez, S. Meenakshisundaram, J. M. Anthonykutty, G. Brett, A. F. Carley, S. H. Taylor, D. W. Knight, G. J. Hutchings, Green Chem. 2009, 11, 1209-1216.
11. C. Bianchi, F. Porta, L. Prati, M. Rossi, Top. Catal. 2000, 13, 231-236.
12. S. De Rossi, G. Ferraris, S. Fremiotti, A. Cimino, V. Indovina, Appl. Catal. A 1992, 81, 113-132.
13. H. G. Manyar, D. Weber, H. Daly, J. M. Thompson, D. W. Rooney, L. F. Gladden, E. H. Stitt, J. J. Delgado, S. Bernal, C. Hardacre, J. Catal. 2009, 265, 80-88.
14. H. Takagi, T. Isoda, K. Kusakabe, S. Morooka, Energy Fuels 1999, 13, 1191-1196.
15. S. Mukherjee, M. A. Vannice, J. Catal. 2006, 243, 108-130.
16. P. Lignier, S. Mangematin, F. Morfin, J. L. Rousset, V. Caps, Catal. Today 2008, 138, 50-54.
17. L. F. Gladden, J. Mitchell, New J. Phys. 2011, 13, 035001.
18. P. T. Callaghan, Principles of Nuclear Magnetic Resonance Microscopy, Oxford University Press, Oxford, 1993.
19. D. Weber, J. Mitchell, J. McGregor, L. F. Gladden, J. Phys. Chem. C 2009, 113, 6610-6615.
20. J. Mitchell, S. C. Stark, J. H. Strange, J. Phys. D 2005, 38, 1950-1958.
21. M. D. Mantle, D. I. Enache, E. Nowicka, S. P. Davies, J. K. Edwards, C. D'Agostino, D. P. Mascarenhas, L. Durham, M. Sankar, D. W. Knight, L. F. Gladden, S. H. Taylor, G. J. Hutchings, J. Phys. Chem. C 2011, 115, 1073-1079.
22. M. Dvoyashkin, R. Valiullin, J. Kärger, Phys. Rev. 2007, 75, 041202.
23. J. Rouquerol, D. Avnir, C. W. Fairbridge, D. H. Everett, J. M. Haynes, N. Pernicone, J. D. F. Ramsay, K. S. W. Sing, K. K. Unger, Pure Appl. Chem. 1994, 66, 1739-1758.
24. S. Dixit, W. C. K. Poon, J. Crain, J. Phys. Condens. Matter 2000, 12, L323-L328.
25. Z. J. Derlacki, A. J. Easteal, A. V. J. Edge, L. A. Woolf, Z. Roksandic, J. Phys. Chem. 1985, 89, 5318-5322.
26. S. Dixit, J. Crain, W. C. K. Poon, J. L. Finney, A. K. Soper, Nature 2002, 416, 829-832.
27. A. Wakisaka, S. Komatsu, Y. Usui, 26th International Conference on Solution Chemistry (26 ICSC) 1999, 175-184.
28. R. Li, C. D'Agostino, J. McGregor, J. H. P. Collins, E. P. J. Parrot, M. D. Mantle, A. Zeitler, L. F. Gladden, 35th International Conference on Infrared, Millimeter and THz Waves 2010.
29. A. Menjoge, J. Dixon, J. F. Brennecke, E. J. Maginn, S. Vasenkov, J. Phys. Chem. B 2009, 113, 6353-6359.
30. D. Xu, C. J. Tsai, R. Nussinov, Protein Eng. 1997, 10, 999-1012.
31. C. D'Agostino, J. Mitchell, L. F. Gladden, M. D. Mantle, J. Phys. Chem. C 2012, 116, 8975-8982.
32. T. Mallat, A. Baiker, Chem. Rev. 2004, 104, 3037-3058.
33. M. Besson, P. Gallezot, Catal. Today 2000, 57, 127-141.
34. K. M. Song, J. Mitchell, H. Jaffel, L. F. Gladden, J. Mater. Sci. 2010, 45, 5282-5290.
35. N. Bloembergen, E. M. Purcell, R. V. Pound, Phys. Rev. 1948, 73, 679-746.
36. S. N. Lanin, E. V. Vlasenko, N. V. Kovaleva, F. M. Zung, Russ. J. Phys. Chem. A 2008, 82, 2152-2155.
37. E. O. Stejskal, J. E. Tanner, J. Chem. Phys. 1965, 42, 288-292.
38. R. M. Cotts, M. J. R. Hoch, T. Sun, J. T. Markert, J. Magn. Reson. 1989, 83, 252-266.
39. E. Fukushima, S. W. Roeder, Experimental Pulse NMR, Addison-Wesley, Reading, 1981.
40. H. Y. Carr, E. M. Purcell, Phys. Rev. 1954, 94, 630-638.