The surface science approach for understanding reactions on oxide powders: The importance of IR spectroscopy

Angewandte Chemie - International Edition

Volumn 51, Issue 19, 2012, Pages 4731-4734

  Xu, Mingchun ^a   Noei, Heshmat ^a   Fink, Karin ^b   Muhler, Martin ^a   Wang, Yuemin ^a   Wöll, Christof ^b  

^a RUHR UNIVERSITY BOCHUM   (Germany)

^b KARLSRUHE INSTITUTE OF TECHNOLOGY   (Germany)

Author keywords

defect sites; heterogeneous catalysis; oxides; surface chemistry; vibrational spectroscopy

Indexed keywords

DEFECT SITES; OXIDE POWDER; POWDER PARTICLES; PROBE MOLECULES; REDUCTIVE COUPLINGS; RUTILE TIO; SURFACE SCIENCE;

CATALYSIS; ETHYLENE; OXIDE MINERALS; OXIDES; SURFACE CHEMISTRY; TITANIUM DIOXIDE; VIBRATIONAL SPECTROSCOPY;

FOURIER TRANSFORM INFRARED SPECTROSCOPY;

EID: 84860764193     PISSN: 14337851     EISSN: 15213773     Source Type: Journal    
DOI: 10.1002/anie.201200585     Document Type: Article

References (28)

1. R. Schaub, P. Thostrup, N. Lopez, E. Laegsgaard, I. Stensgaard, J. K. Norskov, F. Besenbacher, Phys. Rev. Lett. 2001, 87, 266104
2. Z. Zhang, O. Bondarchuk, B. D. Kay, J. M. White, Z. Dohnalek, J. Phys. Chem. B 2006, 110, 21840
3. A. C. Papageorgiou, N. S. Beglitis, C. L. Pang, G. Teobaldi, G. Cabailh, Q. Chen, A. J. Fisher, W. A. Hofer, G. Thornton, Proc. Natl. Acad. Sci. USA 2010, 107, 2391.
4. S. Wendt, R. Schaub, J. Matthiesen, E. K. Vestergaard, E. Wahlstrom, M. D. Rasmussen, P. Thostrup, L. M. Molina, E. Laegsgaard, I. Stensgaard, B. Hammer, F. Besenbacher, Surf. Sci. 2005, 598, 226.
5. S. Wendt, P. T. Sprunger, E. Lira, G. K. H. Madsen, Z. S. Li, J. O. Hansen, J. Matthiesen, A. Blekinge-Rasmussen, E. Laegsgaard, B. Hammer, F. Besenbacher, Science 2008, 320, 1755
6. O. Bikondoa, C. L. Pang, R. Ithnin, C. A. Muryn, H. Onishi, G. Thornton, Nat. Mater. 2006, 5, 189.
7. P. Scheiber, A. Riss, M. Schmid, P. Varga, U. Diebold, Phys. Rev. Lett. 2010, 105, 216101.
8. S. C. Li, U. Diebold, J. Am. Chem. Soc. 2010, 132, 64.
9. E. Asari, R. Souda, Surf. Sci. 2001, 486, 203
10. B. A. Kwetkus, K. Sattler, Ultramicroscopy 1992, 42, 749.
11. C. Lamberti, A. Zecchina, E. Groppo, S. Bordiga, Chem. Soc. Rev. 2010, 39, 4951.
12. G. Ertl, H. J. Freund, Phys. Today 1999, 52, 32.
13. M. Kunat, F. Traeger, D. Silber, H. Qiu, Y. Wang, A. C. van Veen, C. Wöll, P. M. Kowalski, B. Meyer, C. Hattig, D. Marx, J. Chem. Phys. 2009, 130, 144703.
14. Y. Zhao, Z. Wang, X. F. Cui, T. Huang, B. Wang, Y. Luo, J. L. Yang, J. G. Hou, J. Am. Chem. Soc. 2009, 131, 7958.
15. C. N. Rusu, J. T. Yates, Langmuir 1997, 13, 4311
16. M. A. Henderson, W. S. Epling, C. L. Perkins, C. H. F. Peden, U. Diebold, J. Phys. Chem. B 1999, 103, 5328.
17. M. T. Green, J. Am. Chem. Soc. 2006, 128, 1902
18. K. R. Asmis, G. Meijer, M. Brummer, C. Kaposta, G. Santambrogio, L. Woste, J. Sauer, J. Chem. Phys. 2004, 120, 6461.
19. G. Kresse, J. Furthmuller, Phys. Rev. B 1996, 54, 11169
20. G. Kresse, D. Joubert, Phys. Rev. B 1999, 59, 1758.
21. C. Di Valentin, G. Pacchioni, A. Selloni, Phys. Rev. Lett. 2006, 97, 166803.
22. B. J. Morgan, G. W. Watson, Surf. Sci. 2007, 601, 5034.
23. H. Qiu, H. Idriss, Y. M. Wang, C. Wöll, J. Phys. Chem. C 2008, 112, 9828.
24. M. C. Xu, Y. K. Gao, E. M. Moreno, M. Kunst, M. Muhler, Y. M. Wang, H. Idriss, C. Wöll, Phys. Rev. Lett. 2011, 106, 0.
25. H. Noei, C. Wöll, M. Muhler, Y. M. Wang, J. Phys. Chem. C 2011, 115, 908
26. Y. Wang, A. Glenz, M. Muhler, C. Wöll, Rev. Sci. Instrum. 2009, 80, 113108.
27. J. P. Perdew, K. Burke, M. Ernzerhof, Phys. Rev. Lett. 1997, 78, 1396.
28. P. E. Blöchl, Phys. Rev. B 1994, 50, 17953.