Sorption of U(VI) at the TiO2-water interface: An in situ vibrational spectroscopic study

Geochimica et Cosmochimica Acta

Volumn 76, Issue , 2012, Pages 191-205

  Müller, Katharina ^a   Foerstendorf, Harald ^a   Meusel, Tilmann ^a   Brendler, Vinzenz ^a   Lefèvre, Grégory ^b   Comarmond, M Josick ^c   Payne, Timothy E ^c  

^a INSTITUTE OF ION BEAM PHYSICS AND MATERIALS RESEARCH   (Germany)

^b CNRS   (France)

^c AUSTRALIAN NUCLEAR SCIENCE AND TECHNOLOGY ORGANISATION   (Australia)

Author keywords

[No Author keywords available]

Indexed keywords

CARBONATE; CONCENTRATION (COMPOSITION); FORMATION MECHANISM; FTIR SPECTROSCOPY; IN SITU MEASUREMENT; MOLECULAR ANALYSIS; PARTICLE SIZE; PH; SIZE DISTRIBUTION; THERMODYNAMICS; TITANIUM; URANIUM; VIBRATION;

EID: 84855886900     PISSN: 00167037     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.gca.2011.10.004     Document Type: Article

References (57)

1. Arai Y., McBeath M., Bargar J. R., Joye J. and Davis J. A. (2006) Uranyl adsorption and surface speciation at the imogolite-water interface: self-consistent spectroscopic and surface complexation models. Geochim. Cosmochim. Acta 70, 2492-2509.
2. Bargar J. R., Reitmeyer R., Lenhart J. J. and Davis J. A. (2000) Characterization of U(VI)-carbonato ternary complexes on hematite: EXAFS and electrophoretic mobility measurements. Geochim. Cosmochim. Acta 64, 2737-2749.
3. Bargar J. R., Kubicki J. D., Reitmeyer R. and Davis J. A. (2005) ATR-FTIR spectroscopic characterization of coexisting carbonate surface complexes on hematite. Geochim. Cosmochim. Acta 69, 1527-1542.
4. Blesa M. A., Weisz A. D., Morando P. J., Salfity J. A., Magaz G. E. and Regazzoni A. E. (2000) The interaction of metal oxide surfaces with complexing agents dissolved in water. Coord. Chem. Rev. 196, 31-63.
5. Brown, G. E., 1990. Spectroscopic Studies of Chemisorption Reaction Mechanisms at Oxide-Water Interfaces, Mineralogical Society of America, Washington D.C., USA.
6. Carp O., Huisman C. L. and Reller A. (2004) Photoinduced reactivity of titanium dioxide. Prog. Solid State Chem. 32, 33-177.
7. 3 (11 02) surfaces. Geochim. Cosmochim. Acta 69, 3555-3572.
8. Chardon E. S., Bosbach D., Bryan N. D., Lyon I. C., Marquardt C., Romer J., Schild D., Vaughan D. J., Wincott P. L., Wogelius R. A. and Livens F. R. (2008) Reactions of the feldspar surface with metal ions: sorption of Pb(II), U(VI) and Np(V), and surface analytical studies of reaction with Pb(II) and U(VI). Geochim. Cosmochim. Acta 72, 288-297.
9. Chisholm-Brause C., Conradson S. D., Buscher C. T., Eller P. G. and Morris D. E. (1994) Speciation of uranyl sorbed at multiple binding sites on montmorillonite. Geochim. Cosmochim. Acta 58, 3625-3631.
10. Choppin G. R. and Stout B. E. (1989) Actinide behavior in natural waters. Sci. Total Environ. 83, 203-216.
11. Comarmond M. J., Payne T. E., Harrison J. J., Thiruvoth S., Wong H. K., Aughterson R. D., Lumpkin G. R., Muller K. and Foerstendorf H. (2011) Uranium sorption on various forms of titanium dioxide -influence of surface area, surface charge, and impurities. Environ. Sci. Technol. 45, 5536-5542.
12. Den Auwer C., Drot R., Simoni E., Conradson S. D., Gailhanou M. and de Leon J. M. (2003) Grazing incidence XAFS spectroscopy of uranyl sorbed onto TiO2 rutile surfaces. New J. Chem. 27, 648-655.
13. Dixon J. B. and Weed S. B. (1989) Minerals in Soil Environments. Soil Science Society of America, Madison.
14. Drot R., Roques J. and Simoni E. (2007) Molecular approach of the uranyl/mineral interfacial phenomena. C.R. Chim. 10, 1078-1091.
15. Duff M. C., Coughlin J. U. and Hunter D. B. (2002) Uranium coprecipitation with iron oxide minerals. Geochim. Cosmochim. Acta 66, 3533-3547.
16. Elzinga E. J. and Sparks D. L. (2007) Phosphate adsorption onto hematite: an in situ ATR-FTIR investigation of the effects of pH and loading level on the mode of phosphate surface complexation. J. Colloid Interface Sci. 308, 53-70.
17. Grenthe I., Fuger J., Lemire R. J., Muller A. B., Nguyen-Trung C. and Wanner H. (1992) Chemical Thermodynamics of Uranium. Elsevier Science Publishers B.V., Amsterdam.
18. Guillaumont R., Fanghänel T., Fuger J., Grenthe I., Neck V., Palmer D. A. and Rand M. H. (2003) Update on the Chemical Thermodynamics of U, Np, Pu, Am and Tc. Elsevier, Amsterdam.
19. 2: effects of contact time, ionic strength, concentration and humic substance. J. Radioanal. Nucl. Chem. 261, 157-162.
20. Hattori T., Saito T., Ishida K., Scheinost A. C., Tsuneda T., Nagasaki S. and Tanaka S. (2009) The structure of monomeric and dimeric uranyl adsorption complexes on gibbsite: a combined DFT and EXAFS study. Geochim. Cosmochim. Acta 73, 5975-5988.
21. Hippel A. v., Breckenridge R. G., Chesley F. G. and Tisza L. (1946) High dielectric constant ceramics. Ind. Eng. Chem. 38, 1097-1109.
22. 2. Radiochim. Acta 82, 257-262.
23. Jones L. H. and Penneman R. A. (1953) Infrared spectra and structure of uranyl and transuranium(V) and(VI) ions in aqueous perchloric acid solution. J. Chem. Phys. 21, 542-544.
24. 2) in mixed solvents. Colloids Surf. 64, 57-65.
25. Lefèvre G. (2004) In situ fourier-transform infrared spectroscopy studies of inorganic ions adsorption on metal oxides and hydroxides. Adv. Colloid Interface Sci. 107, 109-123.
26. Lefèvre G., Duc M., and Fédoroff M. (2006a) Accuracy in the determination of acid-base properties of metal oxide surfaces, Surface Complexation Modeling. Elsevier, Amsterdam.
27. Lefèvre G., Kneppers J. and Fédoroff M. (2008) Sorption of uranyl ions on titanium oxide studied by ATR-IR spectroscopy. J. Colloid Interface Sci. 327, 15-20.
28. Lefèvre G., Noinville S. and Fédoroff M. (2006b) Study of uranyl sorption onto hematite by in situ attenuated total reflectioninfrared spectroscopy. J. Colloid Interface Sci. 296, 608-613.
29. Maya L. (1982) Sorbed uranium(VI) species on hydrous titania, zirconia, and silica gel. Radiochim. Acta 31, 147-151.
30. Milnes, A. R. and Fitzpatrick, R. W., 1989. Titanium and zirconium minerals, Soil Science Soc. of America, Madison, Wisconsin, USA.
31. Müller K., Brendler V. and Foerstendorf H. (2008) Aqueous uranium(VI) hydrolysis species characterized by attenuated total reflection fourier-transform infrared spectroscopy. Inorg. Chem. 47, 10127-10134.
32. 2, and ZnO: an in situ ATR FT-IR spectroscopic study. Environ. Sci. Technol. 43, 7665-7670.
33. Müller K., Foerstendorf H., Tsushima S., Brendler V. and Bernhard G. (2009b) Direct spectroscopic characterization of aqueous actinyl(VI) species: a comparative study of Np and U. J. Phys. Chem. A 113, 6626-6632.
34. O'Day P. A. (1999) Molecular environmental geochemistry. Rev. Geophys. 37, 249-274.
35. 2 surface from aqueous solution. Oxid. Commun. 29, 698-707.
36. Parks, G. A., 1990. Surface energy and adsorption at mineral-water interfaces: An introduction, Mineralogical Society of America, Washington D.C., USA.
37. 3. Geochim. Cosmochim. Acta 72, 277-287.
38. Payne T. E., Davis J. A., Lumpkin G. R., Chisari R. and Waite T. D. (2004) Surface complexation model of uranyl sorption on Georgia kaolinite. Appl. Clay Sci. 26, 151-162.
39. 2 rutile (1 1 0) face. Inorg. Chem. 45, 6568-6570.
40. Prikryl J. D., Pabalan R. T., Turner D. R. and Leslie B. W. (1994) Uranium sorption on a-alumina -effects of pH and surface area/solution-volume ratio. Radiochim. Acta 66(67), 291-296.
41. Quilès F. and Burneau A. (2000) Infrared and Raman spectra of uranyl(VI) oxo-hydroxo complexes in acid aqueous solutions: a chemometric study. Vib. Spectrosc. 23, 231-241.
42. Rossberg A., Ulrich K. U., Weiss S., Tsushima S., Hiemstra T. and Scheinostt A. C. (2009) Identification of uranyl surface complexes an ferrihydrite: advanced EXAFS data analysis and CDMUSIC modeling. Environ. Sci. Technol. 43, 1400-1406.
43. Sherman D. M., Peacock C. L. and Hubbard C. G. (2008) Surface complexation of U(VI) on goethite (a-FeOOH). Geochim. Cosmochim. Acta 72, 298-310.
44. Silva R. J. and Nitsche H. (1995) Actinide environmental chemistry. Radiochim. Acta 70-1, 377-396.
45. Su C. M. and Suarez D. L. (1997) In situ infrared speciation of absorbed carbonate on aluminum and iron oxide. Clay Clay Min. 45, 814-825.
46. Sylwester E. R., Hudson E. A. and Allen P. G. (2000) The structure of uranium(VI) sorption complexes on silica, alumina, and montmorillonite. Geochim. Cosmochim. Acta 64, 2431-2438.
47. Thakur P., Moore R. C. and Choppin G. R. (2005) Sorption of U(VI) species on hydroxyapatite. Radiochim. Acta 93, 385-391.
48. Tochiyama O., Yamazaki H. and Mikami T. (1996) Sorption of neptunium(V) on various aluminum oxides and hydrous aluminum oxides. Radiochim. Acta 73, 191-198.
49. Tsushima S. (2011) On the "yl" bond weakening in uranyl(VI) coordination complexes. Dalton Trans. 40, 6732-6737.
50. Tsushima S., Nagasaki S., Tanaka S. and Suzuki A. (1998) A Raman spectroscopic study of uranyl species adsorbed onto colloidal particles. J. Phys. Chem. B 102, 9029-9032.
51. Ulrich K. U., Rossberg A., Foerstendorf H., Zänker H. and Scheinost A. C. (2006) Molecular characterization of uranium(VI) sorption complexes on iron(III)-rich acid mine water colloids. Geochim. Cosmochim. Acta 70, 5469-5487.
52. Vandenborre J., Drot R. and Simoni E. (2007) Interaction mechanisms between uranium(VI) and rutile titanium dioxide: from single crystal to powder. Inorg. Chem. 46, 1291-1296.
53. Waite T. D., Davis J. A., Payne T. E., Waychunas G. A. and Xu N. (1994) Uranium(VI) adsorption to ferrihydrite -application of a surface complexation model. Geochim. Cosmochim. Acta 58, 5465-5478.
54. Walter M., Arnold T., Geipel G., Scheinost A. and Bernhard G. (2005) An EXAFS and TRLFS investigation on uranium(VI) sorption to pristine and leached albite surfaces. J. Colloid Interface Sci. 282, 293-305.
55. Wazne M., Korfiatis G. P. and Meng X. G. (2003) Carbonate effects on hexavalent uranium adsorption by iron oxyhydroxide. Environ. Sci. Technol. 37, 3619-3624.
56. Wijnja H. and Schulthess C. P. (2001) Carbonate adsorption mechanism on goethite studied with ATR-FTIR, DRIFT, and proton coadsorption measurements. Soil Sci. Soc. Am. J. 65, 324-330.
57. Yamaguchi T., Nakayama S. and Yoshida T. (2004) Interactions between anionic complex species of actinides and negatively charged mineral surfaces. Radiochim. Acta 92, 677-682.