Analysis of ozone and nitric acid in spring and summer Arctic pollution using aircraft, ground-based, satellite observations and MOZART-4 model: Source attribution and partitioning

Atmospheric Chemistry and Physics

Volumn 12, Issue 1, 2012, Pages 237-259

  Wespes, C ^a   Emmons, L ^a   Edwards, D P ^a   Hannigan, J ^a   Hurtmans, D ^b   Saunois, M ^a   Coheur, P F ^b   Clerbaux, C ^b,c   Coffey, M T ^a   Batchelor, R L ^a   Lindenmaier, R ^d   Strong, K ^d   Weinheimer, A J ^a   Nowak, J B ^e,f   Ryerson, T B ^e   Crounse, J D ^g   Wennberg, P O ^g  

^a NATIONAL CENTER FOR ATMOSPHERIC RESEARCH   (United States)

^b UNIVERSITÉ LIBRE DE BRUXELLES   (Belgium)

^c SORBONNE UNIVERSITÉ   (France)

^d UNIVERSITY OF TORONTO   (Canada)

^e EARTH SYSTEM RESEARCH LABORATORY   (United States)

^f UNIVERSITY OF COLORADO   (United States)

^g CALIFORNIA INSTITUTE OF TECHNOLOGY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

AIR MASS; ANTHROPOGENIC SOURCE; ATMOSPHERIC POLLUTION; ATMOSPHERIC TRANSPORT; CORRELATION; NITRIC ACID; NUMERICAL MODEL; OZONE; REMOTE SENSING; TROPOSPHERE;

EID: 84855512617     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-12-237-2012     Document Type: Article

References (79)

1. Alvarado, M. J., Logan, J. A., Mao, J., Apel, E., Riemer, D., Blake, D., Cohen, R. C., Min, K.-E., Perring, A. E., Browne, E. C., Wooldridge, P. J., Diskin, G. S., Sachse, G. W., Fuelberg, H., Sessions, W. R., Harrigan, D. L., Huey, G., Liao, J., Case-Hanks, A., Jimenez, J. L., Cubison, M. J., Vay, S. A., Weinheimer, A. J., Knapp, D. J., Montzka, D. D., Flocke, F. M., Pollack, I. B., Wennberg, P. O., Kurten, A., Crounse, J., Clair, J. M. St., Wisthaler, A., Mikoviny, T., Yantosca, R. M., Carouge, C. C., and Le Sager, P.: Nitrogen oxides and PAN in plumes from boreal fires during ARCTAS-B and their impact on ozone: an integrated analysis of aircraft and satellite observations, Atmos. Chem. Phys., 10, 9739-9760, doi:10.5194/acp-10-9739-2010, 2010.
2. Antón, M., Loyola, D., Clerbaux, C., López, M., Vilaplana, J. M., Bañón, M., Hadji-Lazaro, J., Valks, P., Hao, N., Zimmer, W., Co-heur, P. F., Hurtmans, D., and Alados-Arboledas, L.: Validation of the Metop-A total ozone data from GOME-2 and IASI using reference ground-based measurements at the Iberian Peninsula, Remote Sens. Environ., 115, 1380-1386, 2011.
3. Batchelor, R. L., Strong, K., Lindenmaier, R., Mittermeier, R. L., Fast, H., Drummond, J. R., and Fogal, P. F.: A new Bruker IFS 125HR FTIR spectrometer for the Polar Environment Atmospheric Research Laboratory at Eureka, Canada: measurements and comparison with the existing BomemDA8 spectrometer, J. Atmos. Ocean. Tech., 26, 1328-1340, doi:10.1175/2009JTECHA1215.1, 2009.
4. Bey, I., Jacob, D. J., Logan, J. A., and Yantosca, R. M.: Asian chemical out now to the Paciec in spring: Origins, pathways, and budgets, J. Geophys. Res., 106, 23097-23113, 2001.
5. Bouwman, A. F., Boumans, L. J. M., and Batjes, N. H.: Modeling global annual N2O and NO emissions from fertilized fields, Global Biogeochem. Cy., 16, 1080, doi:10.1029/2001GB001812, 2002.
6. Boynard, A., Clerbaux, C., Coheur, P.-F., Hurtmans, D., Tur-quety, S., George, M., Hadji-Lazaro, J., Keim, C., and Meyer-Arnek, J.: Measurements of total and tropospheric ozone from IASI: comparison with correlative satellite, ground-based and ozonesonde observations, Atmos. Chem. Phys., 9, 6255-6271, doi:10.5194/acp-9-6255-2009, 2009.
7. Bregman, A., van Velthoven, P. F. J., Wienhold, F. G., Fischer, H., Zenker, T., Waibel, A., Frenzel, A., Arnold, F., Harris, G. W., Bolder, M. J. A., and Lelieveld, J.: Aircraft measurements of O3, HNO3, and N2O in the winter Arctic lower stratosphere during the Stratosphere-Troposphere Experiment by Aircraft Measurements (STREAM) 1, J. Geophys. Res., 100, 11245-11260, 1995.
8. Brock, C. A., Cozic, J., Bahreini, R., Froyd, K. D., Middlebrook, A. M., McComiskey, A., Brioude, J., Cooper, O. R., Stohl, A., Aikin, K. C., de Gouw, J. A., Fahey, D. W., Ferrare, R. A., Gao, R.-S., Gore, W., Holloway, J. S., Hübler, G., Jefferson, A., Lack, D. A., Lance, S., Moore, R. H., Murphy, D. M., Nenes, A., Novelli, P. C., Nowak, J. B., Ogren, J. A., Peischl, J., Pierce, R. B., Pilewskie, P., Quinn, P. K., Ryerson, T. B., Schmidt, K. S., Schwarz, J. P., Sodemann, H., Spackman, J. R., Stark, H., Thomson, D. S., Thornberry, T., Veres, P., Watts, L. A., Warneke, C., and Wollny, A. G.: Characteristics, sources, and transport of aerosols measured in spring 2008 during the aerosol, radiation, and cloud processes affecting Arctic Climate (ARCPAC) Project, Atmos. Chem. Phys., 11, 2423-2453, doi:10.5194/acp-11-2423-2011, 2011.
9. Clerbaux, C., Boynard, A., Clarisse, L., George, M., Hadji-Lazaro, J., Herbin, H., Hurtmans, D., Pommier, M., Razavi, A., Turquety, S., Wespes, C., and Coheur, P.-F.: Monitoring of atmospheric composition using the thermal infrared IASI/MetOp sounder, At-mos. Chem. Phys., 9, 6041-6054, doi:10.5194/acp-9-6041- 2009, 2009.
10. Coheur, P.-F., Clarisse, L., Turquety, S., Hurtmans, D., and Cler-baux, C.: IASI measurements of reactive trace species in biomass burning plumes, Atmos. Chem. Phys., 9, 5655-5667, doi:10.5194/acp-9-5655-2009, 2009.
11. Cooper, O. R., Moody, J. L., Parrish, D. D., Trainer, M., Holloway, J. S., Hubler, G., Fehsenfeld, F. C., and Stohl, A.: Trace gas composition of midlatitude cyclones over the western North Atlantic Ocean: A seasonal comparison of O3 and CO, J. Geophys. Res., 107, 4057, doi:10.1029/2001JD000902, 2002.
12. Cooper, M., Martin, R. V., Sauvage, B., Boone, C. D., Walker, K. A., Bernath, P. F., McLinden, C. A., Degenstein, D. A., Volz-Thomas, A., and Wespes, C.: Evaluation of ACE-FTS and OSIRIS satellite retrievals of ozone and nitric acid in the tropical upper troposphere: Application to ozone production efficiency, J. Geophys. Res., 116, D12306, doi:10.1029/2010JD015056, 2011.
13. Crounse, J. D., McKinney, K. A., Kwan, A. J., and Wennberg, P. O.: Measurement of gas-phase hydroperoxides by chemical ioniza-tion mass spectrometry, Anal. Chem., 78, 6726-6732, 20 2006. (Pubitemid 44522521)
14. Crounse, J. D., DeCarlo, P. F., Blake, D. R., Emmons, L. K., Campos, T. L., Apel, E. C., Clarke, A. D., Weinheimer, A. J., Mc-Cabe, D. C., Yokelson, R. J., Jimenez, J. L., and Wennberg, P. O.: Biomass burning and urban air pollution over the Central Mexican Plateau, Atmos. Chem. Phys., 9, 4929-4944, doi:10.5194/acp-9-4929-2009, 2009.
15. Dufour, G., Eremenko, M., Griesfeller, A., Barret, B., LeFlochmoën, E., Clerbaux, C., Hadji-Lazaro, J., Coheur, P.-F., and Hurtmans, D.: Validation of three different scientific ozone products retrieved from IASI spectra using ozonesondes, Atmos. Meas. Tech. Discuss., 4, 5425-5479, doi:10.5194/amtd-4-5425- 2011, 2011.
16. Emmons, L. K., Hauglustaine, D. A., Müller, J.-F., Carroll, M. A., Brasseur, G. P., Brunner, D., Stahelin, J., Thouret, V., and Marenco, A.: Data composites of airborne observations of tropo-spheric ozone and its precursors, J. Geophys. Res., 105, 20497-20538, 2000. (Pubitemid 32036295)
17. Emmons, L. K., Walters, S., Hess, P. G., Lamarque, J.-F., Pfister, G. G., Fillmore, D., Granier, C., Guenther, A., Kinnison, D., Laepple, T., Orlando, J., Tie, X., Tyndall, G., Wiedinmyer, C., Baughcum, S. L., and Kloster, S.: Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4), Geosci. Model Dev., 3, 43-67, doi:10.5194/gmd-3-43-2010, 2010a.
18. Emmons, L. K., Apel, E. C., Lamarque, J.-F., Hess, P. G., Avery, M., Blake, D., Brune, W., Campos, T., Crawford, J., DeCarlo, P. F., Hall, S., Heikes, B., Holloway, J., Jimenez, J. L., Knapp, D. J., Kok, G., Mena-Carrasco, M., Olson, J., O'Sullivan, D., Sachse, G., Walega, J., Weibring, P., Weinheimer, A., and Wiedinmyer, C.: Impact of Mexico City emissions on regional air quality from MOZART-4 simulations, Atmos. Chem. Phys., 10, 6195-6212, doi:10.5194/acp-10-6195-2010, 2010b.
19. Fisher, H., Wienhold, F. G., Hoor, P., Bujok, O., Schiller, C., Sieg-mund, P., Ambaum, M., Scheeren, H. A., and Lelieveld, J.: Tracer correlations in the northern high latitude lowermost stratosphere: Influence of cross-tropopause mass exchange, Geophys. Res. Lett., 27, 97-100, 2000.
20. Fisher, J. A., Jacob, D. J., Purdy, M. T., Kopacz, M., Le Sager, P., Carouge, C., Holmes, C. D., Yantosca, R. M., Batchelor, R. L., Strong, K., Diskin, G. S., Fuelberg, H. E., Holloway, J. S., Hyer, E. J., McMillan, W. W., Warner, J., Streets, D. G., Zhang, Q., Wang, Y., and Wu, S.: Source attribution and in-terannual variability of Arctic pollution in spring constrained by aircraft (ARCTAS, ARCPAC) and satellite (AIRS) observations of carbon monoxide, Atmos. Chem. Phys., 10, 977-996, doi:10.5194/acp-10-977-2010, 2010.
21. Generoso, S., Bey, I., Attie, J.-L., and Breon, F.-M.: A satellite-and model-based assessment of the 2003 Russian forest Ares: impact on the Arctic region, J. Geophys. Res., 112, D15302, doi:10.1029/2006JD008344, 2007. (Pubitemid 47534420)
22. Hannigan, J. W., Coffey, M. T., and Goldman, A.: Semiautonomous FTS Observation System for Remote Sensing of Stratospheric and Tropospheric Gases, J. Atmos. Oceanic Technol., 26, 1814-1828, doi:10.1175/2009JTECHA1230.1, 2008.
23. Hudman, R. C., Jacob, D. J., Cooper, O. R., Evans, M. J., Heald, C. L., Park, R. J., Fehsenfeld, F., Flocke, F., Holloway, J., Hubler, G., Kita, K., Koike, M., Kondo, Y., Neuman, A., Nowak, J., Olt-mans, S., Parrish, D., Roberts, J. M., and Ryerson, T.: Ozone production in transpacific Asian pollution plumes and implications for ozone air quality in California, J. Geophys. Res., 109, D23S10, doi:10.1029/2004JD004974, 2004. (Pubitemid 40318582)
24. Hudman, R. C., Jacob, D. J., Turquety, S., Leibensperger, E. M., Murray, L. T., Wu, S., Gilliland, A. B., Avery, M., Bertram, T. H., and Brune, W.: Surface and lightning sources of nitrogen oxides over the United States: Magnitudes, chemical evolution, and outflow, J. Geophys. Res.-Atmos, 112, D12S05, doi:10.1029/2006JD007912, 2007. (Pubitemid 47241661)
25. Huey, L. G., Tanner, D. J., Slusher, D. L., Dibb, J. E., Arimoto, R., Chen, G., Davis, D., Buhr, M. P., Nowak, J. B., Mauldin III, R. L., Eisele, F. L., and Kosciuch, E.: CIMS measurements of HNO3 and SO2 at the South Pole during ISCAT 2000, Atmos. Environ., 5411-5421, doi:10.1016/j.atmosenv.2004.04.037, 2004. (Pubitemid 39185845)
26. Hurtmans, D., Coheur, P.-F., Wespes, C., Clarisse, L., Scharf, O., Clerbaux, C., Hadji-Lazaro, J. George, M., and Turquety, S.: FORLI radiative transfer and retrieval code for IASI, Journal of Quantitative Spectroscopy and Radiative Transfer, submitted, 2011.
27. Irie, H., Sugita, T., Nakajima, H., Yokota, T., Oelhaf, H., Wetzel, G., Toon, G. C., Sen, B., Santee, M. L., Terao, Y., Saitoh, N., Ejiri, M. K., Tanaka, T., Kondo, Y., Kanzawa, H., Kobayashi, H., and Sasano, Y.: Validation of stratospheric nitric acid profiles observed by Improved Limb Atmospheric Spectrometer (ILAS-II), J. Geophys. Res., 111, D11S03, doi:10.1029/2005JD006115, 2006. (Pubitemid 44137688)
28. Jacob, D. J., Crawford, J. H., Maring, H., Clarke, A. D., Dibb, J. E., Emmons, L. K., Ferrare, R. A., Hostetler, C. A., Russell, P. B., Singh, H. B., Thompson, A. M., Shaw, G. E., McCauley, E., Ped-erson, J. R., and Fisher, J. A.: The Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARC-TAS) mission: design, execution, and first results, Atmos. Chem. Phys., 10, 5191-5212, doi:10.5194/acp-10-5191-2010, 2010.
29. Kinnison, D., Brasseur, G. P., Walters, S., Garcia, R. R., Marsh, D. R., Sassi, F., Harvey, V. L., Randall, C. E., Emmons, L., Lamar-que, J. F., Hess, P., Orlando, J. J., Tie, X.X., Randel, W., Pan, L.L., Gettelman, A., Granier, C., Diehl, T., Niemeier, U., and Simmons, A. J.: Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model, J. Geophys. Res., 112, D20302, doi:10.1029/2006JD007879, 2007. (Pubitemid 350285723)
30. Kleinman, L. I., Daum, P. H., Lee, Y.-N., Nunnermacker, L. J., and Springston, S. R.: Ozone production efficiency in an urban area, J. Geophys. Res., 107, 4733, doi:10.1029/2002JD002529, 2002.
31. Klonecki, A., Hess, P., Emmons, L., Smith, L., Orlando, J., and Blake, D.: Seasonal changes in the transport of pollutants into the Arctic troposphere-model study, J. Geophys. Res., 108, 8367, doi:10.1029/2002JD002199, 2003.
32. Kurylo, M. J.: Network for the detection of stratospheric change (NDSC), Proc. Soc. Photo-Opt.Instrum.Eng.,1491,168-174,1991.
33. Kurylo, M. J. and Zander, R.: The NDSC-its status after 10 years of operation. Proceedings of the XIX quadrennial ozone symposium, Hokkaido University Sapporo, Japan, 167-168, 2000.
34. Lamarque, J.-F., Hess, P., Emmons, L., Buja, L., Washington, W., and Granier, C.: Tropospheric ozone evolution between 1890 and 1990, J. Geophys. Res., 110, D08304, doi:10.1029/2004JD005537, 2005. (Pubitemid 40899655)
35. Lamarque, J.-F., Bond, T. C., Eyring, V., Granier, C., Heil, A., Klimont, Z., Lee, D., Liousse, C., Mieville, A., Owen, B., Schultz, M. G., Shindell, D., Smith, S. J., Stehfest, E., Van Aardenne, J., Cooper, O. R., Kainuma, M., Mahowald, N., Mc-Connell, J. R., Naik, V., Riahi, K., and van Vuuren, D. P.: Historical (1850-2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application, Atmos. Chem. Phys., 10, 7017-7039, doi:10.5194/acp-10-7017-2010, 2010.
36. Leung, F.-Y., Logan, J. A., Park, R., Hyer, E., Kasischke, E., Streets, D. and Yurganov, L.: Impacts of enhanced biomass burning in the boreal forests in 1998 on tropospheric chemistry and the sensitivity of model results to the injection height of emissions, J. Geo-phys. Res., 112, D10313, doi:doi:10.1029/2006JD007281, 2007. (Pubitemid 47241660)
37. Liang, Q., Jaegle, L., Jaffe, D. A., Weiss-Penzias, P., Heckman, A., and Snow, J. A.: Long-range transport of Asian pollution to the northeast Pacific: Seasonal variations and transport pathways of carbon monoxide, J. Geophys. Res., 109, D23S07, doi:10.1029/2003JD004402, 2004. (Pubitemid 40318579)
38. Liang, Q., Douglass, A. R., Duncan, B. N., Stolarski, R. S., and Witte, J. C.: The governing processes and timescales of stratosphere-to-troposphere transport and its contribution to ozone in the Arctic troposphere, Atmos. Chem. Phys., 9, 3011-3025, doi:10.5194/acp-9-3011-2009, 2009.
39. Lindenmaier, R., Batchelor, R. L., Strong, K., Fast, H., Goutail, F., Kolonjari, F., McElroy, C. T., Mittermeier, R. L., and Walker, K. A.: An evaluation of infrared microwindows for ozone retrievals using the Eureka Bruker 125HR Fourier transform spectrometer, J. Quant. Spectrosc. Ra., 111, 569-585, 2010.
40. Liu, H., Jacob, D. J., Bey, I., Yantosca, R. M., Duncan, B. N., and Sachse, G. W.: Transport pathways for Asian pollution out now over the Paciec: Interannual and seasonal variations, J. Geophys. Res., 108, 8786, doi:10.1029/2002JD003102, 2003. (Pubitemid 350187710)
41. McPeters, R. D., Labow, G. J., and Logan, J. A.: Ozone clima-tological profiles for satellite retrieval algorithms, J. Geophys. Res.-Atmos., 112, D05308, doi:10.1029/2005JD006823, 2007. (Pubitemid 47386323)
42. Miyazaki, Y., Kondo, Y., Koike, M., Fuelberg, H. E., Kiley, C. M., Kita, K., Takegawa, N., Sachse, G. W., Flocke, F., Weinheimer, A. J., Singh, H. B., Eisele, F. L., Zondlo, M., Talbot, R. W., Sandholm, S. T., Avery, M. A., and Blake, D. R.: Synoptic-scale transport of reactive nitrogen over the western Pacific in spring, J. Geophys. Res., 108, 8788, doi:10.1029/2002JD003248, 2003. (Pubitemid 350187712)
43. Murphy, D. M., Fahey, D. W., Proffitt, M. H., Liu, S. C., Chan, K. R., Eubank, C. S., Kawa, S. R., and Kelly, K. K.: Reactive nitrogen and its correlation with ozone in the lower stratosphere and upper troposphere, J. Geophys. Res., 98, 8751-8773, 1993. (Pubitemid 23383081)
44. Neuman, J. A., Gao, R. S., Fahey, D. W., Holecek, J. C., Ridley, B. A., Walega, J. G., Grahek, F. E., Richard, E. C., McElroy, C. T., Thompson, T. L., Elkins, J. W., Moore, F. L., and Ray, E. A.: In situ measurements of HNO3, NOy, NO, and O3 in the lower stratosphere and upper troposphere, Atmos. Environ., 35, 5789-5797, 2001.
45. Neuman, J. A., Parrish, D. D., Trainer, M., Ryerson, T. B., Hol-loway, J. S., Nowak, J. B., Swanson, A., Flocke, F., Roberts, J. M., Brown, S. S., Stark, H., Sommariva, R., Stohl, A., Peltier, R., Weber, R., Wollny, A. G., Sueper, D. T., Hubler, G., and Fehsen-feld, F. C.: Reactive nitrogen transport and photochemistry in urban plumes over the North Atlantic Ocean, J. Geophys. Res., 111, D23S54, doi:10.1029/2005JD007010, 2006. (Pubitemid 47260849)
46. Pfister, G. G., Emmons, L. K., Hess, P. G., Honrath, R., Lamar-que, J.-F., Val Martin, M., Owen, R. C., Avery, M. A., Brow-ell, E. V., Holloway, J. S., Nedelec, P., Purvis, R., Ryerson, T. B., Sachse, G. W., and Schlager, H.: Ozone production from the 2004 North American boreal fires, J. Geophys. Res., 111, D24S07, doi:10.1029/2006JD007695, 2006. (Pubitemid 47260810)
47. Pfister, G. G., Emmons, L. K., Hess, P. G., Lamarque, J.-F., Thompson, A. M., and Yorks, J. E.: Analysis of the summer 2004 ozone budget over the United States using Intercontinental Transport Experiment Ozonesonde Network Study (IONS) observations and Model of Ozone and Related Tracers (MOZART-4) simulations, J. Geophys. Res., 113, D23306, doi:10.1029/2008JD010190, 2008.
48. Pommier, M., Law, K. S., Clerbaux, C., Turquety, S., Hurtmans, D., Hadji-Lazaro, J., Coheur, P.-F., Schlager, H., Ancellet, G., Paris, J.-D., Nédélec, P., Diskin, G. S., Podolske, J. R., Holloway, J. S., and Bernath, P.: IASI carbon monoxide validation over the Arctic during POLARCAT spring and summer campaigns, Atmos. Chem. Phys., 10, 10655-10678, doi:10.5194/acp-10-10655-2010, 2010.
49. Popp, P. J., Marcy, T. P., Gao, R. S., Watts, L. A., Fahey, D. W., Richard, E. C., Oltmans, S. J., Santee, M. L., Livesey, N. J., Froidevaux, L., Sen, B., Toon, G. C., Walker, K. A., Boone, C. D., and Bernath, P. F.: Stratospheric correlation between nitric acid and ozone, J. Geophys. Res., 114, D03305, doi:10.1029/2008JD010875, 2009.
50. Preston, C. M. and Schmidt, M. W. I.: Black (pyrogenic) carbon: a synthesis of current knowledge and uncertainties with special consideration of boreal regions, Biogeosciences, 3, 397-420, doi:10.5194/bg-3-397-2006, 2006. (Pubitemid 44423089)
51. Price, H. U., Jaffe, D. A., Cooper, O. R., and Doskey, P. V.: Photochemistry, ozone production, and dilution during long-range transport episodes from Eurasia to the northwest United States, J. Geophys. Res., 109, D23S13, doi:10.1029/2003JD004400, 2004. (Pubitemid 40318585)
52. Querol, X., Pey, J., Minguillón, M. C., Pérez, N., Alastuey, A., Viana, M., Moreno, T., Bernabé, R. M., Blanco, S., Cárdenas, B., Vega, E., Sosa, G., Escalona, S., Ruiz, H., and Art́ñano, B.: PM speciation and sources in Mexico during the MILAGRO-2006 Campaign, Atmos. Chem. Phys., 8, 111-128, doi:10.5194/acp-8-111- 2008, 2008.
53. Ramaswamy, V., Boucher, O., Haigh, J., Hauglustaine, D., Hay-wood, J., Myhre, G., Nakajima, T., Shi, G. Y., and Solomon, S.: Radiative forcing of climate change, in Climate Change 2001: The Scientific Basis, edited by: Houghton, J. T., Ding, Y., Griggs, D. J., Noguer, M., van der Linden, P. J., Dai, X., Maskell, K., and Johnson, C. A., 349-416, Cambridge Univ. Press, New York, 2001.
54. Rastigejev, Y., Park, R., Brenner, M. P., and Jacob, D. J.: Resolving intercontinental pollution plumes in global models of atmospheric transport, J. Geophys. Res., 115, D02302, doi:10.1029/2009JD012568, 2009.
55. Ridley, B. A., Walega, J. G. Dye, J. E., and Grahek, F. E.: Distributions of NO, NOx, NOy, and O3 to 12km altitude during the summer monsoon season over New Mexico, J. Geophys. Res., 99, 25519-25534, 1994.
56. Richter, A., Burrows, J. P., Nuß, H., Granier, C., and Niemeier, U.: Increase in tropospheric nitrogen dioxide over China observed from space, Nature, 437, 129-132, doi:10.1038/nature04092, 2005. (Pubitemid 41613438)
57. Rodgers, C. D.: Inverse methods for atmospheric sounding: theory and practice, Ser. Atmos. Ocean. Planet. Phys. 2, World Sci., Hackensack, NJ, 2000.
58. Scannell, C., Hurtmans, D., Boynard, A., Hadji-Lazaro, J., George, M., Delcloo, A., Tuinder, O., Coheur, P.-F., and Clerbaux, C.: A review of the ozone hole from 2008 to 2010 as observed by IASI, Atmos. Meas. Tech. Discuss., 4, 4717-4752, doi:10.5194/amtd-4-4717-2011, 2011.
59. Schneider J., Arnold, F., Curtius, J., Sierau, B., Fischer, H., Hoor, P., Wienhold, F. G., Parchatka, U., Zhang, Y. C., Schlager, H., Ziereis, H., Feigl, Ch., Lelieveld, J., Scheeren, H. A., and Bujok, O.: The temporal evolution of the ratio HNO3/NOy in the Arctic lower stratosphere from January to March 1997, Geophys. Res. Lett, 26, 1125-1128, 1999. (Pubitemid 29390839)
60. Shindell, D. T., Chin, M., Dentener, F., Doherty, R. M., Faluvegi, G., Fiore, A. M., Hess, P., Koch, D. M., MacKenzie, I. A., Sanderson, M. G., Schultz, M. G., Schulz, M., Stevenson, D. S., Teich, H., Textor, C., Wild, O., Bergmann, D. J., Bey, I., Bian, H., Cuvelier, C., Duncan, B. N., Folberth, G., Horowitz, L. W., Jonson, J., Kaminski, J. W., Marmer, E., Park, R., Pringle, K. J., Schroeder, S., Szopa, S., Takemura, T., Zeng, G., Keating, T. J., and Zuber, A.: A multi-model assessment of pollution transport to the Arctic, Atmos. Chem. Phys., 8, 5353-5372, doi:10.5194/acp-8-5353-2008, 2008.
61. Shon, Z.-H., Madronich, S., Song, S.-K., Flocke, F. M., Knapp, D. J., Anderson, R. S., Shetter, R. E., Cantrell, C. A., Hall, S. R., and Tie, X.: Characteristics of the NO-NO2-O3 system in different chemical regimes during the MIRAGE-Mex field campaign, At-mos. Chem. Phys., 8, 7153-7164, doi:10.5194/acp-8-7153-2008, 2008.
62. Singh, H.B., Hertlth, D., Kolyer, R., Salas, L., Bradshaw, J. D., Sandholm, S. T., Davis, D. D., Crawford, J.,Kondo, Y., Koike, M., Talbot, R., Gregory, G. L., Sachse, G. W.,Browell, E., Blake, D. R., Rowland, F. S., Newell, R.,Merrill, J., Heikes, B., Liu, S.C., Crutzen, P. J., and Kanakidou, M.: Reactive nitrogen and ozone over the western Pacific: Distribution, partitioning, and sources, J. Geophys. Res., 101, 1793-1808, 1996.
63. Stohl, A.: Characteristics of atmospheric transport into the Arctic troposphere, J. Geophys. Res., 111, D11306, doi:10.1029/2005JD006888, 2006. (Pubitemid 44137685)
64. Stohl, A., Berg, T., Burkhart, J. F., Fjæraa, A. M., Forster, C., Herber, A., Hov, Ø., Lunder, C., McMillan, W. W., Oltmans, S., Shiobara, M., Simpson, D., Solberg, S., Stebel, K., Ström, J., Tørseth, K., Treffeisen, R., Virkkunen, K., and Yttri, K. E.: Arctic smoke-record high air pollution levels in the European Arctic due to agricultural fires in Eastern Europe in spring 2006, Atmos. Chem. Phys., 7, 511-534, doi:10.5194/acp-7-511- 2007, 2007. (Pubitemid 46181320)
65. Talbot, R. W., Dibb, J. E., Lefer, B. L., Scheuer, E. M., Bradshaw, J. D., Sandholm, S. T., Smyth, S., Blake, D. R., Blake, N. J., Sachse, G. W., Collins, J. E., and Gregory, G. L.: Large-scale distributions of tropospheric nitric, formic, and acetic acids over the western Pacific basin during wintertime, Geophys. Res. Lett, 102, 28303-28313, 1997.
66. Tilmes, S., Emmons, L. K., Law, K. S., Ancellet, G., Schlager, H., Paris, J.-D., Fuelberg, H. E., Streets, D. G., Wiedinmyer, C., Diskin, G. S., Kondo, Y., Holloway, J., Schwarz, J. P., Spackman, J. R., Campos, T., Nédélec, P., and Panchenko, M. V.: Source contributions to Northern Hemisphere CO and black carbon during spring and summer 2008 from POLARCAT and START08/preHIPPO observations and MOZART-4, Atmos. Chem. Phys. Discuss., 11, 5935-5983, doi:10.5194/acpd-11-5935-2011, 2011.
67. Trainer, M., Parrish, D.D., Buhr, M.P., Norton, R. B., Fehsenfeld, F. C., Anlauf, K. G., Bottenheim, J. W., Tang, Y. Z., Wiebe, H. A., Roberts, J. M., Tanner, R. L., Newman, L., Bowersox, V. C., Meagher, J. F., Olszyna, K. J., Rodgers, M. O., Wang, T., Berresheim, H., Demerjian, K. L., and Roychowdhury, U. K.: Correlation of ozone with NOy in photochemically aged air, J. Geophys. Res., 98, 2917-2925, 1993. (Pubitemid 23380957)
68. Turquety, S., Logan, J. A., Jacob, D. J., Hudman, R. C., Leung, F. Y., Heald, C. L., Yantosca, R. M., Wu, S., Emmons, L. K., Edwards, D. P., and Sachse, G.W.: Inventory of boreal fire emissions for North America in 2004: the importance of peat burning and pyro-convective injection, J. Geophys. Res. 112, D12S03, doi:10.1029/2006JD007281, 2007. (Pubitemid 47241660)
69. Turquety, S., Hurtmans, D., Hadji-Lazaro, J., Coheur, P.-F., Cler-baux, C., Josset, D., and Tsamalis, C.: Tracking the emission and transport of pollution from wildfires using the IASI CO retrievals: analysis of the summer 2007 Greek fires, Atmos. Chem. Phys., 9, 4897-4913, doi:10.5194/acp-9-4897-2009, 2009.
70. Vigouroux, C., De Mazière, M., Errera, Q., Chabrillat, S., Mahieu, E., Duchatelet, P., Wood, S., Smale, D., Mikuteit, S., Blumen-stock, T., Hase, F., and Jones, N.: Comparisons between ground-based FTIR and MIPAS N2O and HNO3 profiles before and after assimilation in BASCOE, Atmos. Chem. Phys., 7, 377-396, doi:10.5194/acp-7-377-2007, 2007. (Pubitemid 46173888)
71. Warneke, C., Bahreini, R., Brioude, J., Brock, C. A., de Gouw, J. A., Fahey, D. W., Froyd, K. D., Holloway, J. S., Middlebrook, A., Miller, L., Montzka, S., Murphy, D. M., Peischl, J., Ryerson, T. B., Schwarz, J. P., Spackman, J. R., and Veres, P.: Biomass burning in Siberia and Kazakhstan as the main source for Arctic Haze over the Alaskan Arctic in April 2008, Geophys. Res. Lett., 36, L02813, doi:10.1029/2008GL036194, 2009.
72. Weinheimer, A. J., Walega, J. G., Ridley, B. A., Gary, B. L., Blake, D. R., Blake, N. J., Rowland, F. S., Sachse, G. W., Anderson, B. E., and Collins, J. E.: Meridional distributions of NOx, NOy, and other species in the lower stratosphere and upper troposphere during AASE II, Geophys. Res. Lett., 21, 2583-2586, 1994.
73. Wespes, C., Hurtmans, D., Clerbaux, C., Santee, M. L., Martin, R. V., and Coheur, P. F.: Global distributions of nitric acid from IASI/MetOP measurements, Atmos. Chem. Phys., 9, 7949-7962, doi:10.5194/acp-9-7949-2009, 2009.
74. Wiedinmyer, C., Quayle, B., Geron, C., Belote, A., McKenzie, D., Zhang, X., O'Neill, S., and Wynne, K.: Estimating emissions from fires in North America for air quality modeling, Atmos. Environ., 40, 3419-3432, 2006. (Pubitemid 43766469)
75. Wiedinmyer, C., Akagi, S. K., Yokelson, R. J., Emmons, L. K., Al-Saadi, J. A., Orlando, J. J., and Soja, A. J.: The Fire INventory from NCAR (FINN): a high resolution global model to estimate the emissions from open burning, Geosci. Model Dev., 4, 625-641, doi:10.5194/gmd-4-625-2011, 2011.
76. Yienger, J. and Levy, H.: Empirical model of global soil biogenic NOx emissions, J. Geophys. Res., 100, 11447-11464, 1995.
77. Zellweger, C., Forrer, J., Hofer, P., Nyeki, S., Schwarzenbach, B., Weingartner, E., Ammann, M., and Baltensperger, U.: Partitioning of reactive nitrogen (NOy) and dependence on meteorological conditions in the lower free troposphere, Atmos. Chem. Phys., 3, 779-796, doi:10.5194/acp-3-779-2003, 2003.
78. Zhang, L., Jacob, D. J., Boersma, K. F., Jaffe, D. A., Olson, J. R., Bowman, K. W., Worden, J. R., Thompson, A. M., Avery, M. A., Cohen, R. C., Dibb, J. E., Flock, F. M., Fuelberg, H. E., Huey, L. G., McMillan, W. W., Singh, H. B., and Weinheimer, A. J.: Transpacific transport of ozone pollution and the effect of recent Asian emission increases on air quality in North America: an integrated analysis using satellite, aircraft, ozonesonde, and surface observations, Atmos. Chem. Phys., 8, 6117-6136, doi:10.5194/acp-8-6117-2008, 2008.
79. Zhang, Q., Streets, D. G., Carmichael, G. R., He, K. B., Huo, H., Kannari, A., Klimont, Z., Park, I. S., Reddy, S., Fu, J. S., Chen, D., Duan, L., Lei, Y., Wang, L. T., and Yao, Z. L.: Asian emissions in 2006 for the NASA INTEX-B mission, Atmos. Chem. Phys., 9, 5131-5153, doi:10.5194/acp-9-5131-2009, 2009.