Tuning the hydrophobicity of mesoporous silica materials for the adsorption of organic pollutant in aqueous solution

Journal of Hazardous Materials

Volumn 201-202, Issue , 2012, Pages 107-114

  Trouvé, Adeline ^a   Batonneau Gener, Isabelle ^a   Valange, Sabine ^a   Bonne, Magali ^a   Mignard, Samuel ^a  

^a Centre National de la Recherche Scientifique   (France)

Author keywords

HMS; Hydrophobicity; MCM 41; Pollutant removal; Silylation

Indexed keywords

ADSORPTION CAPACITIES; FUNCTIONALIZATIONS; FUNCTIONALIZED; HMS; HYDROPHOBIC CHARACTER; INDEX VALUES; LANGMUIR MODELS; MCM-41; MENISCUS FORMATION; MESO-PORES; MESOPOROUS SILICA; MESOPOROUS SILICA MATERIALS; N ,N-DIETHYL-M-TOLUAMIDE; ORGANIC GROUP; ORGANIC MOIETY; ORGANICALLY FUNCTIONALIZED; ORGANOPHILIC; POLLUTANT REMOVAL; SILANOL GROUPS; SILANOLS; SILICA MATERIAL; SILICA SURFACE; SILYLATIONS; STORAGE CAPACITY; SURFACE FUNCTIONALIZATION; TRIMETHYLSILYL GROUPS; WATER CAPILLARIES;

ADSORBENTS; ADSORPTION; CALCINATION; DRIERS (MATERIALS); HYDROPHILICITY; HYDROPHOBICITY; ORGANIC POLLUTANTS; SILICA; SOLUTIONS; SURFACES; TOLUENE;

MESOPOROUS MATERIALS;

BIOMATERIAL; DIETHYLTOLUAMIDE; ORGANIC COMPOUND; SILANOL; SILICON DIOXIDE;

ADSORPTION; AQUEOUS SOLUTION; CONDENSATION; HYDROPHOBICITY; ISOTHERM; NUMERICAL MODEL; ORGANIC POLLUTANT; POLLUTANT REMOVAL; POROSITY; SILICA; TOLUENE;

ADSORPTION; AQUEOUS SOLUTION; ARTICLE; CONTROLLED STUDY; DENSITY; HYDROPHILICITY; HYDROPHOBICITY; LANGMUIR BLODGETT FILM; POLYMERIZATION; POROSITY; WATER POLLUTANT; WATER POLLUTION;

ADSORPTION; CHROMATOGRAPHY, HIGH PRESSURE LIQUID; DEET; DIFFERENTIAL THERMAL ANALYSIS; HYDROPHOBIC AND HYDROPHILIC INTERACTIONS; POROSITY; SILICON DIOXIDE; SURFACE PROPERTIES; WATER POLLUTANTS, CHEMICAL; WATER PURIFICATION; X-RAY DIFFRACTION;

EID: 84855339860     PISSN: 03043894     EISSN: 18733336     Source Type: Journal    
DOI: 10.1016/j.jhazmat.2011.11.043     Document Type: Article

References (36)

1. Foo K.Y., Hameed B.H. Detoxification of pesticide waste via activated carbon adsorption process. J. Hazard. Mater. 2010, 175:1-11.
2. Sanchez-Martin M.J., Rodriguez-Cruz M.S., Andrades M.S., Sanchez-Camazano M. Efficiency of different clay minerals modified with a cationic surfactant in the adsorption of pesticides: influence of clay type and pesticide hydrophobicity. Appl. Clay Sci. 2006, 31:216-228.
3. Kyriakopoulos G., Doulia D., Anagnostopoulos E. Adsorption of pesticides on porous polymeric adsorbents. Chem. Eng. Sci. 2005, 60:1177-1186.
4. Khalid M., Joly G., Renaud A., Magnoux P. Removal of phenol from water by adsorption using zeolites. Ind. Eng. Chem. Res. 2004, 43:5275-5280.
5. Koubaissy B., Joly G., Batonneau-Gener I., Magnoux P. Adsorptive removal of aromatic compounds present in wastewater by using dealuminated Faujasite zeolite. Ind. Eng. Chem. Res. 2011, 50:5705-5713.
6. Ng E.P., Mintova S. Nanoporous materials with enhanced hydrophilicity and high water sorption capacity. Micropor. Mesopor. Mater. 2008, 114:1-26.
7. Pires J., Moisés Pinto J., Estella J.C., Echeverria Characterisation of the hydrophobicity of mesoporous silica and clays with silica pillars by water adsorption and DRIFT. J. Colloid Interface Sci. 2008, 317:206-213.
8. Zhao X.S., Lu G.Q., Hu X. Organophilicity of MCM-41 adsorbents studied by adsorption and temperature-programmed desorption. Colloids Surf. A 2001, 179:261-269.
9. Zhao X.S., Ma Q., Lu G.Q. VOC removal: comparison of MCM-41 with hydrophobic zeolites and activated carbon. Energy Fuels 1998, 12:1051-1054.
10. Choudhary V.R., Mantri K. Adsorption of aromatic hydrocarbons on highly siliceous MCM-41. Langmuir 2000, 16:7031-7037.
11. Mangrulkar P.A., Kamble S.P., Meshram J., Rayalu S.S. Adsorption of phenol and o-chlorophenol by mesoporous MCM-41. J. Hazard. Mater. 2008, 160:414-421.
12. Goworek J., Kierys A., Iwan M., Stefaniak W. Sorption on as-synthesized MCM-41. J. Therm. Anal. Cal. 2007, 87:165-169.
13. Denoyel R., Sabio Rey E. Solubilization in confined surfactant mesophases. Langmuir 1998, 14:7321-7323.
14. Zhang C., Zhou W., Liu S., Synthesis Characterization of organofunctionalized MCM-41 by the original stepped templated sol-gel technology. J. Phys. Chem. B 2005, 109:24319-24325.
15. Burkett S.L., Sims S.D., Mann S. Synthesis of hybrid inorganic-organic mesoporous silica by co-condensation of siloxane and organosiloxane precursors. Chem. Commun. 1996, 136:7-1368.
16. Macquarrie D.J. Direct preparation of organically modified MCM-type materials. Preparation and characterisation of aminopropyl-MCM and 2-cyanoethyl-MCM. Chem. Commun. 1996, 196:1-1962.
17. Zhao X.S., Lu G.Q. Modification of MCM-41 by surface silylation with trimethylchlorosilane and adsorption study. J. Phys. Chem. B 1998, 102:1556-1561.
18. Guidotti M., Batonneau-Gener I., Gianotti E., Marchese L., Mignard S., Psaro R., Sgobba M., Ravasio N. The effect of silylation on titanium-containing silica catalysts for the epoxidation of functionalised molecules. Micropor. Mesopor. Mater. 2008, 111:39-47.
19. Galarneau A., Lefèvre B., Cambon H., Coasne B., Valange S., Gabelica Z., Bellat J.P., Di Renzo F. Pore-shape effects in the determination of the pore size of ordered mesoporous silicas by mercury intrusion. J. Phys. Chem. C 2008, 112:12921-12927.
20. Macquarrie D.J., Jackson D.B., Mdoe J.E.G., Clark J.H. New J. Chem. 1999, 23:539.
21. Batonneau-Gener I., Yonli A., Trouve A., Mignard S., Guidotti M., Sgobba M. Tailoring the hydrophobic character of mesoporous silica by silylation for VOC removal. Sep. Sci. Technol. 2010, 45:768-775.
22. Yonli A.H., Gener I., Mignard S. Influence of post-synthesis treatment on BEA zeolites hydrophobicity assessed under static and dynamic conditions. Micropor. Mesopor. Mater. 2009, 122:135-142.
23. Koubaissy B., Joly G., Magnoux P. Adsorption and competitive adsorption on zeolites of nitrophenol compounds present in wastewater. Ind. Eng. Chem. Res. 2008, 47:9558-9568.
24. Anwander R., Nagl I., Widenmeyer M., Engelhardt G., Groerger O., Palm C., Röser T. Surface characterization and functionalization of MCM-41 silicas via silazane silylation. J. Phys. Chem. B 2000, 104:3532-3544.
25. Rouquerol F., Rouquerol G., Sing K. Adsorption by Powders and Porous Solids 1999, Academic Press.
26. Galarneau A., Desplantier D., Dutartre R., Di Renzo F. Micelle-templated silicates as a test bed for methods of mesopore size evaluation. Micropor. Mesopor. Mater. 1999, 27:297-308.
27. Jelinek L., Kovats E.sz. True surface areas from nitrogen adsorption experiments. Langmuir 1994, 10:4225-4231.
28. Kim Y.H., Lee B., Choo K.H., Choi S.J. Selective adsorption of bisphenol A by organic-inorganic hybrid mesoporous silicas. Micropor. Mesopor. Mater. 2011, 138:184-190.
29. Blin J.L., Carteret C. Investigation of the silanol groups of mesostructured silica prepared using a fluorinated surfactant: influence of the hydrothermal temperature. J. Phys. Chem. C 2003, 111:14380-14388.
30. Vansant E.F., van der Voort P., Vranken K.C. Characterization and chemical modification of the silica surface 1995, Elsevier, The Netherlands.
31. Legrand A.P., Hommel H., Tuel A., Vidal A., Balard H., Papirer E., Levitz P., Czernichowski M., Erre R., Van Damme H., Gallas J.P., Hemidy J.F., Lavalley J.C., Barres O., Burneau A., Grillet Y. Hydroxyls of silica powders. Adv. Colloid Interface Sci. 1990, 33:91-333.
32. Kozlova S.A., Kirik S.D. Post-synthetic covering in the mesostructured silicate materials MCM-41 and SBA-15. Micropor. Mesopor. Mater. 2010, 133:124-133.
33. Zhuravlev L.T. The surface chemistry of amorphous silica: Zhuravlev model. Colloids Surf. A 2000, 173:1-38.
34. Zhao X.S., Lu G.Q., Whittaker A.K., Millar G.J., Zhu H.Y. Comprehensive study of surface chemistry of MCM-41 using 29Si CP/MAS NMR, FTIR, pyridine-TPD, and TGA. J. Phys. Chem. B 1997, 101:6525-6531.
35. Widenmeyer M., Anwander R. Pore size control of highly ordered mesoporous silica MCM-48. Chem. Mater. 2002, 14:1827-1831.
36. Batonneau-Gener I., Yonli A., Hazael-Pascal S., Pedro Marques J., Madeira Lopes J., Guisnet M., Ramôa Ribeiro F., Mignard S. Influence of steaming and acid-leaching treatments on the hydrophobicity of HBEA zeolite determined under static conditions. Micropor. Mesopor. Mater. 2008, 110:480-487.