Degradation of amoxicillin in aqueous solution using sulphate radicals under ultrasound irradiation

Ultrasonics Sonochemistry

Volumn 19, Issue 3, 2012, Pages 469-474

  Su, Shengnan ^a   Guo, Weilin ^a   Yi, Chunliang ^a   Leng, Yanqiu ^a   Ma, Zhenmin ^a  

^a UNIVERSITY OF JINAN   (China)

Author keywords

Advanced oxidation processes; Amoxicillin; Degradation; Sulfate radicals; Ultrasound

Indexed keywords

COBALT; DEGRADATION; ENERGY EFFICIENCY; IRRADIATION; ORGANIC POLLUTANTS; POTASH; SOLUTIONS; SULFUR COMPOUNDS; ULTRASONICS;

ADVANCED OXIDATION PROCESSES; AMOXICILLIN; CHEMICAL OXYGEN DEMAND REMOVALS; COD REMOVAL EFFICIENCY; OPERATIONAL CONDITIONS; OXIDATION POTENTIALS; SULFATE RADICALS; ULTRASOUND IRRADIATION;

CHEMICAL OXYGEN DEMAND;

AMOXICILLIN; COBALT; SODIUM PEROXIDE; SULFATE;

AQUEOUS SOLUTION; ARTICLE; CHEMICAL OXYGEN DEMAND; COMPARATIVE STUDY; CONCENTRATION (PARAMETERS); CONTROLLED STUDY; DRUG DEGRADATION; DRUG STRUCTURE; OXIDATION; PRIORITY JOURNAL; TEMPERATURE; ULTRASOUND;

EID: 84855284287     PISSN: 13504177     EISSN: 18732828     Source Type: Journal    
DOI: 10.1016/j.ultsonch.2011.10.005     Document Type: Article

References (38)

1. V. Homem, A. Alves, L. Santos, Amoxicillin degradation at ppb levels by Fenton oxidation using design of experiments, Sci. Total Environ. 408 (2010) 6272-6280.
2. E.S. Elmolla, M. Chaudhuri, Degradation of the antibiotics amoxicillin, ampicillin and cloxacillin in aqueous solution by the photo-Fenton process, J. Hazard. Mater. 172 (2009) 1476-1481.
3. E. Elmolla, M. Chaudhuri, Optimization of Fenton process for treatment of amoxicillin, ampicillin and cloxacillin antibiotics in aqueous solution, J. Hazard. Mater. 170 (2009) 666-672.
4. F. Ay, F. Kargi, Advanced oxidation of amoxicillin by Fenton's reagent treatment, J. Hazard. Mater. 179 (2010) 622-627.
5. J. Madhavan, P. Maruthamuthu, S. Murugesan, S. Anandan, Kinetic studies on visible light-assisted degradation of acid red 88 in presence of metal-ion coupled oxone reagent, Appl. Catal. B: Environ. 83 (2008) 8-14.
6. Y.S. Ma, C.F. Sun, J.G. Lin, Degradation of carbofuran in aqueous solution by ultrasound and Fenton processes: effect of system parameters and kinetic study, J. Hazard. Mater. 178 (2010) 320-325.
7. G.P. Anipsitakis, D. Dionysiou, Degradation of organic contaminants in water with sulfate radicals generated by the conjunction of peroxymonosulfate with cobalt, Environ. Sci. Technol. 37 (2003) 4790-4797. (Pubitemid 37266401)
8. P. Shukla, H.Q. Sun, S.B. Wang, H. MingAng, M.O. Tade, Co-SBA-15 for heterogeneous oxidation of phenol with sulfate radical for wastewater treatment, Catal. Today (2011) 1-6.
9. W. Chu, W.K. Choy, C.Y. Kwan, Selection of supported cobalt substrates in the presence of oxone for the oxidation of monuron, J. Agric. Food Chem. 55 (2007) 5708-5713. (Pubitemid 47092947)
10. 2+ oxidation as an advanced oxidation process comparison with traditional Fenton oxidation for treatment of landfill leachate, Water Res. 43 (2009) 4363-4369.
11. 2+ reagent in dark and light processes, J. Mol. Catal. A: Chem. 252 (2006) 113-119.
12. Y.T. Lin, C.J. Liang, J.H. Chen, Feasibility study of ultraviolet activated persulfate oxidation of phenol, Chemosphere 82 (2011) 1168-1172.
13. - transfer mechanisms, Appl. Catal. B: Environ. 96 (2010) 290-298.
14. 2+ reagent through Fenton-like chemistry, Chem. Commun. 18 (2003) 2382-2383.
15. G.P. Anipsitakis, D.D. Dionysiou, Degradation of organic contaminants in water with sulfate radicals generated by the conjunction of peroxymonosulfate with cobalt, Environ. Sci. Technol. 37 (2003) 4790-4797. (Pubitemid 37266401)
16. 2+ reagent in Fenton-like processes, Appl. Catal. B: Environ. 49 (2004) 207-215.
17. 2+ reagent in dark and light processes, J. Mol. Catal. A: Chem. 252 (2006) 113-119.
18. X.Y. Chen, X.L. Qiao, D.G. Wang, J. Lin, J.W. Chen, Kinetics of oxidative decolorization and mineralization of Acid Orange 7 by dark and photo assisted Co2+-catalyzed peroxymonosulfate system, Chemosphere 67 (2007) 802-808. (Pubitemid 46107608)
19. 4/peroxymonosulfate system: kinetics and mechanism study using Acid Orange 7 as a model compound, Appl. Catal. B: Environ. 80 (2008) 116-121.
20. P.R. Shukla, S.B. Wang, H.M. Ang, M.O. Tadé, Photocatalytic oxidation of phenolic compounds using zinc oxide and sulphate radicals under artificial solar light, Sep. Purif. Technol. 30 (2010) 338-344.
21. G.P. Anipsitakis, D.D. Dionysiou, M.A. Gonzalez, Cobalt-mediated activation of peroxymonosulfate and sulfate radical attack on phenolic compounds. Implications of chloride ions, Environ. Sci. Technol. 40 (2006) 1000-1007. (Pubitemid 43222191)
22. 2+/ peroxymonosulfate, J. Hazard. Mater. 178 (2010) 385-389.
23. P. Shukla, S.-B. Wang, H.-Q. Sun, H.-M. Ang, M. Tadé, Activated carbon supported cobalt catalysts for advanced oxidation of organic contaminants in aqueous solution, Appl. Catal. B: Environ. 100 (2010) 529-534.
24. P. Shukla, I. Fatimah, S.-B. Wang, H.M. Ang, M.O. Tadé, Photocatalytic generation of sulphate and hydroxyl radicals using zinc oxide under low-power UV to oxidise phenolic contaminants in wastewater, Catal. Today 157 (2010) 410-414.
25. P. Shukla, S.-B. Wang, K. Singh, H.M. Ang, M.O. Tadé, Cobalt exchanged zeolites for heterogeneous catalytic oxidation of phenol in the presence of peroxymonosulphate, Appl. Catal. B: Environ. 99 (2010) 163-169.
26. K.H. Chan, W. Chu, Degradation of atrazine by cobalt-mediated activation of peroxymonosulfate: different cobalt counteranions in homogenous process and cobalt oxide catalysts in photolytic heterogeneous process, Water Res. 43 (2009) 2513-2521.
27. S. Yang, P. Wang, X. Yang, G. Wei, W. Zhang, L. Shan, A novel advanced oxidation process to degrade organic pollutants in wastewater: microwave-activated persulfate oxidation, J. Environ Sci. 21 (2009) 1175-1180.
28. H. Hori, A. Yamamoto, E. Hayakawa, S. Taniyasu, N. Yamashita, S. Kutsuna, et al., Efficient decomposition of environmentally persistent perfluorocarboxylic acids by use of persulfate as a photochemical oxidant, Environ. Sci. Technol. 39 (2005) 2383-2388. (Pubitemid 40490333)
29. 2-Fe(II,III) two-stage oxidation process, J. Hazard. Mater. 162 (2009) 1211-1216.
30. C.J. Liang, C.J. Bruell, Thermally activated persulfate oxidation of trichloroethylene: experimental investigation of reaction orders, Ind. Eng. Chem. Res. 47 (2008) 2912-2918. (Pubitemid 351747405)
31. A. Rastogi, S.R. Al-Abed, D.D. Dionysiou, Sulfate radical-based ferrous-peroxymonosulfate oxidative system for PCBs degradation in aqueous and sediment systems, Appl. Catal. B: Environ. 85 (2009) 171-179.
32. B. Neppolian, H. Jung, H. Choi, J.H. Lee, J.W. Kang, Sonolytic degradation of methyl tertbutyl ether: the role of coupled Fenton process and persulphate ion, Water Res. 36 (2002) 4699-4708. (Pubitemid 35341101)
33. E.V. Rokhna, E. Repo, J. Virkutyte, Comparative kinetic analysis of silent and ultrasound-assisted catalytic wet peroxide oxidation of phenol, Ultrason. Sonochem. 17 (2010) 541-546.
34. P. Gayathri, R. Praveena Juliya Dorathi, K. Palanivelu, Sonochemical degradation of textile dyes in aqueous solution using sulphate radicals activated by immobilized cobalt ions, Ultrason. Sonochem. 17 (2010) 566-571.
35. APHA-AWWA-WEF Standard Methods for the Examination of Water and Wastewater, 20th ed., American Public Health Association, Washington, 1999
36. G.P. Anipsitakis, D.D. Dionysiou, Chemical and microbial decontamination of pool water using activated potassium peroxymonosulfate, Environ. Eng. Sci. 25 (2008) 234-245.
37. W.L. Guo, Y.H. Shi, H.Z. Wang, H. Yang, Guangyou Zhang, Sonochemical decomposition of levofloxacin in aqueous solution, Water. Environ. Res. 82 (2010) 696-700.
38. P. Gayathri, R.P. Juliya Dorathi, K. Palanivelu, Sonochemical degradation of textile dyes in aqueous solution using sulphate radicals activated by immobilized cobalt ions, Ultrason. Sonochem. 17 (2010) 566-571.