Photosensitized oxidation of emerging organic pollutants by tetrakis C 60 aminofullerene-derivatized silica under visible light irradiation

Environmental Science and Technology

Volumn 45, Issue 24, 2011, Pages 10598-10604

  Lee, Jaesang ^a   Hong, Seokwon ^a   MacKeyev, Yuri ^b   Lee, Changha ^c   Chung, Eunhyea ^a   Wilson, Lon J ^b   Kim, Jae Hong ^d   Alvarez, Pedro J J ^e  

^a Korea Institute of Science and Technology   (South Korea)

^b RICE UNIVERSITY   (United States)

^c Ulsan National Institute of Science and Technology   (South Korea)

^d Georgia Institute of Technology   (United States)

^e Rice University   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ALKALINE PH; BISPHENOL A; CARBAMAZEPINE; ELECTRON-RICH; ENDOCRINE DISRUPTOR; KINETICALLY ENHANCED; NATURAL ORGANIC MATTERS; ORGANIC CONTAMINANT; OXIDATIVE DEGRADATION; PHENOLIC MOIETY; PHOTO-CATALYTIC; PHOTOSENSITIZED OXIDATION; RANITIDINE; REMOVAL EFFICIENCIES; SEMICONDUCTOR PHOTOCATALYST; SILICA SUPPORTS; SINGLET OXYGEN; SULFISOXAZOLE; TETRAKIS; TIO; TRIMETHOPRIM; VISIBLE-LIGHT IRRADIATION;

ADSORPTION; ALKALINITY; AMIDES; BIOLOGICAL MATERIALS; IRRADIATION; ORGANIC POLLUTANTS; OXYGENATION; PHENOLS; PHOTOCATALYSTS; PHOTODEGRADATION; SILICA; TITANIUM DIOXIDE; VIRUSES; WATER TREATMENT;

LIGHT;

4,4' ISOPROPYLIDENEDIPHENOL; AMINOFULLERENE; CARBAMAZEPINE; CARBON; CIMETIDINE; FULLERENE DERIVATIVE; ORGANIC MATTER; PARACETAMOL; PENTACHLOROPHENOL; PROPRANOLOL; RANITIDINE; SILICON DIOXIDE; SINGLET OXYGEN; SULFAFURAZOLE; TITANIUM DIOXIDE; TRIMETHOPRIM; UNCLASSIFIED DRUG;

ANATASE; BACTERIUM; CATALYST; DEGRADATION; DRUG; ENDOCRINE DISRUPTOR; FULLERENE; IRRADIATION; ORGANIC POLLUTANT; OXIDATION; PH; PHENOLIC COMPOUND; PHOTOCHEMISTRY; POLLUTANT REMOVAL; REACTION KINETICS; SILICA; TUNGSTEN; VIRUS;

ARTICLE; ELECTRON SPIN RESONANCE; LIGHT; PH; PHOTOCATALYSIS; PHOTOCHEMISTRY; PHOTOOXIDATION; SEMICONDUCTOR;

ENDOCRINE DISRUPTORS; ENVIRONMENTAL REMEDIATION; FULLERENES; LIGHT; OXIDATION-REDUCTION; PHARMACEUTICAL PREPARATIONS; PHOTOCHEMICAL PROCESSES; SILICON DIOXIDE; WASTE DISPOSAL, FLUID; WATER POLLUTANTS, CHEMICAL;

EID: 83455255621     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es2029944     Document Type: Article

References (48)

1. 60 aminofullerene immobilized on silica as a visible-light-activated photocatalyst Environ. Sci. Technol. 2010, 44, 9488-9495
2. Hoffmann, M. R.; Martin, S. T.; Choi, W. Y.; Bahnemann, D. W. Environmental applications of semiconductor photocatalysis Chem. Rev. 1995, 95, 69-96
3. Mills, A.; LeHunte, S. An overview of semiconductor photocatalysis J. Photochem. Photobiol., A 1997, 108, 1-35 (Pubitemid 127165886)
4. Asahi, R.; Morikawa, T.; Ohwaki, T.; Aoki, K.; Taga, Y. Visible light photocatalysis in nitrogen doped titanium oxides Science 2001, 293, 269-271 (Pubitemid 32694736)
5. 2 J. Phys. Chem. C 2010, 114, 783-792
6. 3 as an environmental photocatalyst that generates OH radicals under visible light Environ. Sci. Technol. 2010, 44, 6849-6854
7. 2 photocatalyst synthesized without using an external carbon precursor and the visible light activity Appl. Catal. B: Environ. 2009, 91, 355-361
8. 2 for the redox conversion of water pollutants under visible light Chem. Commun. 2010, 46, 2477-2479
9. 2 Environ. Sci. Technol. 2009, 43, 7079-7085
10. 2 and CdS-AgI systems J. Phys. Chem. 1990, 94, 6435-6440
11. Kim, H. G.; Hwang, D. W.; Lee, J. S. An undoped, single phase oxide photocatalyst working under visible light J. Am. Chem. Soc. 2004, 126, 8912-8913 (Pubitemid 38971062)
12. 4 through nanocasting: A superior visible light driven photocatalyst Chem. Mater. 2008, 20, 3983-3992
13. Kim, W.; Park, J.; Jo, H. J.; Kim, H. J.; Choi, W. Visible light photocatalysts based on homogeneous and heterogenized tin porphyrins J. Phys. Chem. C 2008, 112, 491-499 (Pubitemid 351189891)
14. 60 J. Phys. Chem. 1991, 95, 11-12
15. 2 J. Am. Chem. Soc. 2003, 125, 12803-12809 (Pubitemid 37280449)
16. Badireddy, A. R.; Hotze, E. M.; Chellam, S.; Alvarez, P.; Wiesner, M. R. Inactivation of Bacteriophages via photosensitization of fullerol nanoparticles Environ. Sci. Technol. 2007, 41, 6627-6632 (Pubitemid 47438010)
17. 60 fullerene aggregates Environ. Sci. Technol. 2009, 43, 6208-6213
18. 60 derivative Environ. Sci. Technol. 2010, 44, 6685-6691
19. 60 derivatives in aqueous systems Environ. Sci. Technol. 2009, 43, 6604-6610
20. 2 acceptor properties and reactivity J. Am. Chem. Soc. 1974, 96, 6846-6850
21. Tratnyek, P. G.; Holgne, J. Oxidation of substituted phenols in the environment-A QSAR analysis of rate constants for reaction with singlet oxygen Environ. Sci. Technol. 1991, 25, 1596-1604
22. Jensen, A. W.; Daniels, C. Fullerene-coated beads as reusable catalysts J. Org. Chem. 2003, 68, 207-210 (Pubitemid 36125948)
23. Schwarzenbach, R. P.; Escher, B. I.; Fenner, K.; Hofstetter, T. B.; Johnson, C. A.; von Gunten, U.; Wehrli, B. The challenge of micropollutants in aquatic systems Science 2006, 313, 1072-1077 (Pubitemid 44300225)
24. Stumn, W.; Morgan, J. J. Aquatic Chemistry; John Wiley & Sons: New York, 1996.
25. Haag, W. R.; Hoigné, J. Singlet oxygen in surface waters. 3. Photochemical formation and steady-state concentrations in various types of waters Environ. Sci. Technol. 1986, 20, 341-348 (Pubitemid 16028797)
26. Hoigné, J.; Faust, B. C.; Haar, W. R.; Scully, F. E.; Zepp, R. G., Aquatic humic substances as sources and sinks of photochemically produced transient reactants. In In Aquatic Humic Substances: Influence on Fate and Treatment of Pollutants; American Chemical Society: Washington, DC, 1989.
27. Zepp, R. G.; Hoigné, J.; Bader, H. Nitrate-induced photooxidation of trace organic chemicals in water Environ. Sci. Technol. 1987, 21, 443-450 (Pubitemid 17118030)
28. Sandvik, S. L. H.; Bilski, P.; Pakulski, J. D.; Chignell, C. F.; Coffin, R. B. Photogeneration of singlet oxygen and free radicals in dissolved organic matter isolated from the Mississippi and Atchafalaya River plumes Mar. Chem. 2000, 69, 139-152 (Pubitemid 30168031)
29. 60 photoreactivity in water: Fate of triplet state and radical anion and production of reactive oxygen species Environ. Sci. Technol. 2008, 42, 3459-3464
30. Halling-Sorensen, B.; Nielsen, S. N.; Lanzky, P. F.; Ingerslev, F.; Lutzhoft, H. C. H.; Jorgensen, S. E. Occurrence, fate and effects of pharmaceutical substances in the environment-A review Chemosphere 1998, 36, 357-394
31. Richardson, M. L.; Bowron, J. M. The fate of pharmaceutical chemicals in the aquatic environment J. Pharm. Pharmacol. 1985, 37, 1-12 (Pubitemid 15189939)
32. Wilkinson, F.; Helman, W. P.; Ross, A. B. Rate constants for the decay and reactions of the lowest electronically excited singlet state of molecular oxygen in solution-An expanded and revised compilation J. Phys. Chem. Ref. Data 1995, 24, 663-1021
33. Merkel, P. B.; Kearns, D. R. Radiationless decay of singlet molecular oxygen in solution. An experimental and theoretical study of electronic-to-vibrational energy transfer J. Am. Chem. Soc. 1972, 94, 7244-7253
34. Bailey, D. N.; Briggs, J. R. The binding of acetaminophen, lidocaine, and valproic acid to human milk Amer. J. Clin. Pathol. 2004, 121, 754-757 (Pubitemid 38534008)
35. 2O System Ind. Eng. Chem. Res. 1991, 30, 462-467
36. Serjeant, E. P.; Dempsey, B. Ionisation Constants of Organic Acids in Aqueous Solution; Pergamon: Oxford, UK, 1979.
37. Hoigné, J.; Bader, H. Rate constants of reactions of ozone with organic and inorganic compounds in water. 2. Dissociating organic compounds Wat. Res. 1983, 17, 185-194
38. Cessna, A. J.; Grover, R. Spectrophotometric determination of dissociation constants of selected acidic herbicides J. Agric. Food Chem. 1978, 26, 289-292 (Pubitemid 8284786)
39. Abe, R.; Takami, H.; Murakami, N.; Ohtani, B. Pristine simple oxides as visible light driven photocatalysts: Highly efficient decomposition of organic compounds over platinum-loaded tungsten oxide J. Am. Chem. Soc. 2008, 130, 7780-7781 (Pubitemid 351875026)
40. 2 photocatalysts under visible illumination J. Phys. Chem. B 2004, 108, 17269-17273
41. 2 an effective visible light photocatalyst for remediation? Appl. Catal. B: Environ. 2009, 91, 554-562
42. 2-Correlation between photoreactivity and charge carrier recombination dynamics J. Phys. Chem. 1994, 98, 13669-13679
43. 2 particles J. Phys. Chem. 1994, 98, 13695-13704
44. •-) in aqueous solution J. Phys. Chem. Ref. Data 1988, 17, 513-886
45. Lee, Y.; von Gunten, U. Oxidative transformation of micropollutants during municipal wastewater treatment: Comparison of kinetic aspects of selective (chlorine, chlorine dioxide, ferrate(VI), and ozone) and non-selective oxidants (hydroxyl radical) Wat. Res. 2010, 44, 555-566
46. Lee, Y.; Escher, B. I.; Von Gunten, U. Efficient removal of estrogenic activity during oxidative treatment of waters containing steroid estrogens Environ. Sci. Technol. 2008, 42, 6333-6339
47. Lawton, L. A.; Robertson, P. K. J. Physico-chemical treatment methods for the removal of microcystins (cyanobacterial hepatotoxins) from potable waters Chem. Soc. Rev. 1999, 28, 217-224
48. Szpyrkowicz, L.; Juzzolino, C.; Kaul, S. N. A comparative study on oxidation of disperse dyes by electrochemical process, ozone, hypochlorite and Fenton reagent Wat. Res. 2001, 35, 2129-2136 (Pubitemid 32381027)