Three pyrazine derivatives as corrosion inhibitors for steel in 1.0M H2SO4 solution

Corrosion Science

Volumn 53, Issue 10, 2011, Pages 3241-3247

  Li, Xianghong ^a   Deng, Shuduan ^a   Fu, Hui ^a  

^a SOUTHWEST FORESTRY UNIVERSITY   (China)

Author keywords

A. Steel; B. EIS; B. Polarization; B. Weight loss; C. Acid inhibition

Indexed keywords

A. STEEL; B. EIS; B. POLARIZATION; C. ACID INHIBITION; WEIGHT LOSS;

ADSORPTION; COLD ROLLING; ELECTROCHEMICAL CORROSION; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; METAL CLADDING; POLARIZATION;

CORROSION INHIBITORS;

EID: 79960708708     PISSN: 0010938X     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.corsci.2011.05.068     Document Type: Article

References (71)

1. Trabanelli G. Inhibitors an old remedy for a new challenge. Corrosion 1991, 47:410-419.
2. Bentiss F., Traisnel M., Gengembre L., Lagrenée M. Inhibition of acidic corrosion of mild steel by 3,5-diphenyl-4H-1,2,4-triazole. Appl. Surf. Sci. 2000, 161:194-202.
3. Cruz J., Martínez R., Genesca J., García-Ochoa E. Experimental and theoretical study of 1-(2-ethylamino)-2-methylimidazoline as an inhibitor of carbon steel corrosion in acid media. J. Electroanal. Chem. 2004, 566:111-121.
4. Wahdan M.H., Gomma G.K. Effect of copper cation on electrochemical behaviour of steel in presence of imidazole in acid medium. Mater. Chem. Phys. 1997, 47:176-183.
5. Abdennaby A.M.S., Abdulhady A.I., Abu-Oribi S.T., Saricimen H. The inhibition action of 1 (benzyl)1-H-4,5-dibenzoyl -1,2,3-triazole on mild steel in hydrochloric acid media. Corros. Sci. 1996, 38:1791-1800.
6. Granese S.L., Rosales B.M., Oviedo C., Zerbino J.O. The inhibition action of heterocyclic nitrogen organic compounds on Fe and steel in HCl media. Corros. Sci. 1992, 33:1439-1453.
7. Bentiss F., Traisnel M., Gengembre L., Lagrenée M. A new triazole derivative as inhibitor of the acid corrosion of mild steel: electrochemical studies, weight loss determination, SEM and XPS. Appl. Surf. Sci. 1999, 152:237-249.
8. Wang L. Inhibition of mild steel corrosion in phosphoric acid solution by triazole derivatives. Corros. Sci. 2006, 48:608-616.
9. Quraishi M.A., Sharma H.K. 4-Amino-3-butyl-5-mercapto-1,2,4-triazole: a new corrosion inhibitor for mild steel in sulphuric acid. Mater. Chem. Phys. 2002, 78:18-21.
10. García-Ochoa E., Genesca J. Understanding the inhibiting properties of 3-amino-1,2,4-triazole from fractal analysis. Surf. Coat. Tech. 2004, 184:322-330.
11. Li W.H., He Q., Zhang S.T., Pei C.L., Hou B.R. Some new triazole derivatives as inhibitors for mild steel corrosion in acidic medium. J. Appl. Electrochem. 2008, 38:289-295.
12. Wang H.L., Liu R.B., Xin J., 0 M HCl medium Inhibiting effects of some mercapto-triazole derivatives on the corrosion of mild steel in 1. Corros. Sci. 2004, 46:2455-2466.
13. Bentiss F., Traisnel M., Vezin H., Lagrenée M. Linear resistance model of the inhibition mechanism of steel in HCl by triazole and oxadiazole derivatives: structure-activity correlations. Corros. Sci. 2003, 45:371-380.
14. Lebrini M., Traisnel M., Lagrenée M., Mernari B., Bentiss F. Inhibitive properties, adsorption and a theoretical study of 3,5-bis(n-pyridyl)-4-amino-1,2,4-triazoles as corrosion inhibitors for mild steel in perchloric acid. Corros. Sci. 2008, 50:473-479.
15. Bentiss F., Lagrenee M., Traisnel M., Hornez J.C. The corrosion inhibition of mild steel in acidic media by a new triazole derivative. Corros. Sci. 1999, 41:789-803.
16. Li W.H., Zhao X., Liu F.Q., Hou B.R. Investigation on inhibition behavior of S-triazole-triazole derivatives in acidic solution. Corros. Sci. 2008, 50:3261-3266.
17. Bentiss F., Jama C., Mernari B., El Attari H., El Kadi L., Lebrini M., Traisnel M., Lagrenée M. Corrosion control of mild steel using 3,5-bis(4-methoxyphenyl)-4-amino-1,2,4-triazole in normal hydrochloric acid medium. Corros. Sci. 2009, 51:1628-1635.
18. Tao Z.H., Zhang S.T., Li W.H., Hou B.R. Corrosion inhibition of mild steel in acidic solution by some oxo-triazole derivatives. Corros. Sci. 2009, 51:2588-2595.
19. Gomma G.K. Corrosion inhibition of steel by benzotriazole in sulphuric acid. Mater. Chem. Phys. 1998, 55:235-240.
20. Qu Q., Jiang S.A., Bai W., Li L. Effect of ethylenediamine tetraacetic acid disodium on the corrosion of cold rolled steel in the presence of benzotriazole in hydrochloric acid. Electrochim. Acta 2007, 52:6811-6820.
21. Hudson R.M., Bulter T.J., Warning C.J. The effect of pyrrole-halide mixtures in inhibiting the dissolution of low-carbon steel in sulphuric acid. Corros. Sci. 1977, 17:571-581.
22. Bouklah M., Ouassini A., Hammouti B., El Idrissi A., 5 M H2 SO4 by [(2-pyridin-4-ylethyl) thio] acetic acid Corrosion inhibition of steel in 0. Appl. Surf. Sci. 2005, 250:50-56.
23. Ouchrif A., Zegmout M., Hammouti B., El-Kadiri S., Ramdani A., 5 M H2 SO4 solution 1,3-Bis(3-hyroxymethyl-5-methyl-1-pyrazole) propane as corrosion inhibitor for steel in 0. Appl. Surf. Sci. 2005, 252:339-344.
24. Gomma G.K. Corrosion of low-carbon steel in sulphuric acid solution in the presence of pyrazole-halides mixture. Mater. Chem. Phys. 1998, 55:241-246.
25. Abdallah M., El-Naggar M.M. Cu+2 cation + 3,5-dimethyl pyrazole mixture as a corrosion inhibitor for carbon steel in sulfuric acid solution. Mater. Chem. Phys. 2001, 71:291-298.
26. Elayyachy M., Elkodadi M., Aouniti A., Ramdani A., Hammouti B., Malek F., Elidrissi A. New bipyrazole derivatives as corrosion inhibitors for steel in hydrochloric acid solutions. Mater. Chem. Phys. 2005, 93:281-285.
27. Tebbji K., Aouniti A., Benkaddour M., Oudda H., Bouabdallah I., Hammouti B., Ramdani A. New bipyrazolic derivatives as corrosion inhibitors of steel in 1 M HCl. Prog. Org. Coat. 2005, 54:170-174.
28. Zucchi F., Trabanelli G., Brunoro G., Monticelli C., Rocchini G. Corrosion inhibition of carbon and low-alloy steel in sulfuric acid solutions by 2-mercaptopyrimidine derivatives. Mater. Corros. 1993, 44:264-268.
29. Chetouani A., Aouniti A., Hammouti B., Benchat N., Benhadda T., Kertit S. Corrosion inhibitors for iron in hydrochloride acid solution by newly synthesised pyridazine derivatives. Corros. Sci. 2003, 45:1675-1684.
30. Bouklah M., Benchat N., Aouniti A., Hammouti B., Benkaddour M., Lagrenée M., Vezin H., Bentiss F. Effect of the substitution of an oxygen atom by sulphur in a pyridazinic molecule towards inhibition of corrosion of steel in 0.5M H2 SO4 medium. Prog. Org. Coat. 2005, 51:118-124.
31. Bouklah M., Benchat N., Hammouti B., Aouniti A. Thermodynamic characterization of steel corrosion inhibitor adsorption of pyridazine compounds in 0.5 M H2SO4. Mater. Lett. 2006, 60:1901-1905.
32. Moretti G., Quartarone G., Tassan A., Zingales A. 5-amino and 5-chloro-indole as mild steel corrosion inhibitors in 1N sulphuric acid. Electrochim. Acta 1996, 41:1971-1980.
33. Ismail A.A., Sanad S.H., El-Meligi A.A. Inhibiting effect of indole and some of its derivatives on corrosion of C-steel in HCl. J. Mater. Sci. Technol. 2000, 16:397-400.
34. Wang L. Evaluation of 2-mercaptobenzimidazole as corrosion inhibitor for mild steel in phosphoric acid. Corros. Sci. 2001, 43:2281-2289.
35. Popova A., Christov M., Deligeorigiev T. Influence of the Molecular Structure on the inhibitor properties of benzimidazole derivatives on mild steel corrosion in 1 M hydrochloric acid. Corrosion 2003, 59:756-764.
36. Popova A., Christov M., Raicheva S., Sokolova E. Adsorption and inhibitive properties of benzimidazole derivatives in acid mild steel corrosion. Corros. Sci. 2004, 46:1333-1350.
37. Khaled K.F. The inhibition of benzimidazole derivatives on corrosion of iron in1 M HCl solutions. Electrochim. Acta 2003, 48:2493-2503.
38. Wahdan M.H. The synergistic inhibition effect and thermodynamic properties of 2-mercaptobenzimidazol and some selected cations as a mixed inhibitor for pickling of mild steel in acid solution. Mater. Chem. Phys. 1997, 49:135-140.
39. Tang L.B., Li X.M., Si Y.S., Mu G.N., Liu G.H. The synergistic inhibition between 8-hydroxyquinoline chloride ion for the corrosion of cold rolled steel in 0.5 M sulfuric acid. Mater. Chem. Phys. 2006, 95:29-38.
40. Yan Y., Li W.H., Cai L.K., Hou B.R. Electrochemical and quantum chemical study of purines as corrosion inhibitors for mild steel in 1M HCl solution. Electrochim. Acta 2008, 53:5953-5960.
41. Li X.H., Deng S.D., Fu H., Li T.H. Adsorption inhibition of 6-benzylaminopurine on cold rolled steel in 1.0 M HCl. Electrochim. Acta 2009, 54:4089-4098.
42. Li X.H., Deng S.D., Fu H., Mu G.N. Inhibition effect of 6-benzylaminopurine on the corrosion of cold rolled steel in H2 SO4 solution. Corros. Sci. 2009, 51:620-634.
43. Bensajjay E., Alehyen S., El Achouri M., Kertit S. Corrosion inhibition of steel by 1-phenyl-5-mercapto 1.2,3,4-tetrazole in acidic environments (0.5 M H2SO4 1/3 M H3PO4). Anti-Corros. Meth. Mater. 2003, 50:402-409.
44. Morales-Gil P., Negrón-Silva G., Romero-Romoa M., Ángeles-Chávez C., Palomar-Pardavé M. Corrosion inhibition of pipeline steel grade API 5L X52 immersed in 1 M H2SO4 aqueous solution using heterocyclic organic molecules. Electrochim. Acta 2004, 49:4733-4741.
45. Li X.H., Deng S.D., Fu H. Corrosion inhibition of red tetrazolium for cold rolled steel in hydrochloric acid media. Chin. J. Appl. Chem. 2009, 26:1075-1079. in Chinese.
46. Li X.H., Deng S.D., Fu H. Synergism between red tetrazolium and uracil on the corrosion of cold rolled steel in H2SO4 solution. Corros. Sci. 2009, 51:1344-1355.
47. Li X.H., Deng S.D., Fu H. Synergistic inhibition effect of red tetrazolium and uracil on the corrosion of cold rolled steel in H3PO4 solution: weight loss, electrochemical, and AFM approaches. Mater. Chem. Phys. 2009, 115:815-824.
48. Li X.H., Deng S.D., Fu H. Blue tetrazolium as a novel corrosion inhibitor for cold rolled steel in hydrochloric acid solution. Corros. Sci. 2010, 52:2786-2792.
49. Deng S.D., Li X.H., Fu H. Nitrotetrazolium blue chloride as a novel corrosion inhibitor of steel in sulfuric acid solution. Corros. Sci. 2010, 52:3840-3846.
50. Bouklah M., Attayibat A., Kertit S., Ramdani A., Hammouti B. A pyrazine derivative as corrosion inhibitor for steel in sulphuric acid solution. Appl. Surf. Sci. 2005, 242:399-406.
51. Kissi M., Bouklah M., Hammouti B., Establishment of equivalent circuits from electrochemical impedance spectroscopy study of corrosion inhibition of steel by pyrazine in sulphuric acidic solution M.Benkaddour. Appl. Surf. Sci. 2005, 252:4190-4197.
52. Deng S.D., Li X.H., Fu H. Two pyrazine derivatives as inhibitors of the cold rolled steel corrosion in hydrochloric acid solution. Corros. Sci. 2011, 53:822-828.
53. Cano E., Polo J.L., La Iglesia A., Bastidas J.M. A study on the adsorption of benzotriazole on copper in hydrochloric acid using the inflection point of the isotherm. Adsorption 2004, 10:219-225.
54. Bentiss F., Lebrini M., Lagrenée M. Thermodynamic characterization of metal dissolution and inhibitor adsorption processes in mild steel/2,5-bis(n-thienyl)-1,3,4-thiadiazoles/hydrochloric acid system. Corros. Sci. 2005, 47:2915-2931.
55. Yurt A., Ulutas S., Dal H. Electrochemical and theoretical investigation on the corrosion of aluminium in acidic solution containing some Schiff bases. Appl. Surf. Sci. 2006, 253:919-925.
56. Okafor P.C., Zheng Y.G. Synergistic inhibition behaviour of methylbenzyl quaternary imidazoline derivative and iodine ions on mild steel in H2SO4 solutions. Corros. Sci. 2009, 51:850-859.
57. Cao C. On electrochemical techniques for interface inhibitor research. Corros. Sci. 1996, 38:2073-2082.
58. Labjar N., Lebrini M., Bentiss F., Chihib N.E., El Hajjaji S., Jama C. Corrosion inhibition of carbon steel and antibacterial properties of aminotris-(methylnephosnic) acid. Mater. Chem. Phys. 2010, 119:330-336.
59. Lagrenée M., Mernari B., Bouanis M., Traisnel M., Bentiss F. Study of the mechanism and inhibiting efficiency of 3,5-bis(4-metylthiophenyl)-4H-1,2,4-triazole on mild steel corrosion in acidic media. Corros. Sci. 2002, 44:573-588.
60. Singh A.K., Quraishi M.A. Effect of Cefazolin on the corrosion of mild steel in HCl solution. Corros. Sci. 2010, 52:152-160.
61. Lebrini M., Lagrenée M., Vezin H., Traisnel M., Bentiss F. Experimental and theoretical study for corrosion inhibition of mild steel in normal hydrochloric acid solution by some new macrocyclic polyether compounds. Corros. Sci. 2007, 49:2254-2269.
62. Priya A.R.S., Muralidharam V.S., Subramania A. Development of novel acidizing inhibitors for carbon steel corrosion in 15% boiling hydrochloric acid. Corrosion 2008, 64:541-552.
63. Bommersbach P., Alemany-Dumont C., Millet J.P., Normand B. Hydrodynamic effect on the behaviour of a corrosion inhibitor film: Characterization by electrochemical impedance spectroscopy. Electrochim. Acta 2006, 51:4011-4018.
64. Schweinsberg D.P., Ashworth V. The inhibition of the corrosion of pure iron in 0.5 M sulphuric acid by n-alkyl quaternary ammonium iodides. Corros. Sci. 1988, 28:539-545.
65. Roy S.C., Roy S.K., Sircar S.C. Critique of inhibitor evaluation by polarization measurement. Br. Corro. J. 1988, 32:102-104.
66. Bentiss F., Traisnel M., Lagrenée M. The substituted 1,3,4-oxadiazoles: a new class of corrosion inhibitors of mild steel in acidic media. Corros. Sci. 2000, 42:127-146.
67. Kilner C.A., Halcrow M.A. An iron(II) complex of 26-di(pyrazol-1-yl)pyrazine that crystallises in three forms, two of which exhibit an unusual angular Jahn-Teller distortion. Polyhedron 2006, 25:235-240.
68. Beaufort L., Benvenuti F., Noels A.F. Iron(II)-ethylene polymerization catalysts bearing 2,6-bis(imino)pyrazine ligands: part I. Synthesis and characterization. J. Mol. Catal. A-Chem. 2006, 260:210-214.
69. Hackerman N., Kaesche H. Corrosion inhibition by organic amines. J. Electrochem. Soc. 1958, 105:191-198.
70. Hong B., Qiu Y.Q. DFT study on electronic structures pyrazine derivatives with donor and acceptor group. J. Molecu. Sci. 2004, 20:54-58. in Chinese.
71. Qiu Y.Q., Yu H.Y., Su Z.M., Zhao L., Wang R.S., Zhu Y.L. Teheoretial studies on electronic spectrum and third-order nonlinear optical properties of centrosymmetric pyrazine derivatives. Chem. J. Chine. Univ. 2004, 25:2335-2338. in Chinese.