Complete reconstruction of the wave function of a reacting molecule by four-wave mixing spectroscopy

Physical Review Letters

Volumn 106, Issue 17, 2011, Pages

  Avisar, David ^a   Tannor, David J ^a  

^a WEIZMANN INSTITUTE OF SCIENCE   (Israel)

Author keywords

[No Author keywords available]

Indexed keywords

COHERENT ANTI-STOKES RAMAN SPECTROSCOPY; FOUR-WAVE MIXING SPECTROSCOPY; GROUND POTENTIAL; POLYATOMICS; REAL-TIME DYNAMICS; TIME-DEPENDENT WAVE FUNCTION;

EXCITED STATES; MOLECULES; RAMAN SPECTROSCOPY; WAVE FUNCTIONS;

FOUR WAVE MIXING;

EID: 79960686803     PISSN: 00319007     EISSN: 10797114     Source Type: Journal    
DOI: 10.1103/PhysRevLett.106.170405     Document Type: Article

References (30)

1. A.H. Zewail, Science 242, 1645 (1988). SCIEAS 0036-8075 10.1126/science.242.4886.1645
2. J.C. Polanyi and A.H. Zewail, Acc. Chem. Res. 28, 119 (1995). ACHRE4 0001-4842 10.1021/ar00051a005
3. P. Kukura, Science 310, 1006 (2005). SCIEAS 0036-8075 10.1126/science.1118379 (Pubitemid 41611910)
4. S. Takeuchi, Science 322, 1073 (2008). SCIEAS 0036-8075 10.1126/science.1160902
5. U. Banin and S. Ruhman, J. Chem. Phys. 99, 9318 (1993). JCPSA6 0021-9606 10.1063/1.465501
6. M. Shapiro, J. Chem. Phys. 103, 1748 (1995); JCPSA6 0021-9606 10.1063/1.469748
7. see also C. Leichtle, Phys. Rev. Lett. 80, 1418 (1998). PRLTAO 0031-9007 10.1103/PhysRevLett.80.1418
8. J.A. Cina, J. Chem. Phys. JCPSA6 0021-9606 113, 9488 (2000); 10.1063/1.1319873 (Pubitemid 32085128)
9. J.A. Cina Annu. Rev. Phys. Chem. 59, 319 (2008). ARPLAP 0066-426X 10.1146/annurev.physchem.59.032607.093753 (Pubitemid 351703389)
10. R.M. Roth, M.A. Ratner, and R.B. Gerber, Phys. Rev. Lett. 52, 1288 (1984). PRLTAO 0031-9007 10.1103/PhysRevLett.52.1288
11. R.B. Bernstein and A.H. Zewail, J. Chem. Phys. 90, 829 (1989). JCPSA6 0021-9606 10.1063/1.456108
12. T. Ho and H. Rabitz, J. Chem. Phys. 89, 5614 (1988). JCPSA6 0021-9606 10.1063/1.455568
13. R. Baer and R. Kosloff, J. Phys. Chem. 99, 2534 (1995). JPCHAX 0022-3654 10.1021/j100009a011
14. M. Shapiro, Phys. Chem. Chem. Phys. 12, 15760 (2010); PPCPFQ 1463-9076 10.1039/c0cp01417f
15. X. Li and M. Shapiro, J. Chem. Phys. JCPSA6 0021-9606 134, 094113 (2011). 10.1063/1.3561494
16. N.F. Scherer, J. Chem. Phys. 95, 1487 (1991). JCPSA6 0021-9606 10.1063/1.461064
17. K. Ohmori, Phys. Rev. Lett. 96, 093002 (2006); PRLTAO 0031-9007 10.1103/PhysRevLett.96.093002 (Pubitemid 43344774)
18. K. Ohmori, Annu. Rev. Phys. Chem. 60, 487 (2009). ARPLAP 0066-426X 10.1146/annurev.physchem.59.032607.093818
19. T.C. Weinacht, J. Ahn, and P.H. Bucksbaum, Phys. Rev. Lett. 80, 5508 (1998). PRLTAO 0031-9007 10.1103/PhysRevLett.80.5508
20. A. Monmayrant, B. Chatel, and B. Girard, Phys. Rev. Lett. 96, 103002 (2006). PRLTAO 0031-9007 10.1103/PhysRevLett.96.103002
21. D.J. Tannor, Introduction to Quantum Mechanics: A Time-Dependent Perspective (University Science, Sausalito, CA, 2007), Eq. (13.8).
22. Soo-Y. Lee and E.J. Heller, J. Chem. Phys. 71, 4777 (1979); JCPSA6 0021-9606 10.1063/1.438316
23. E.J. Heller, R.L. Sundberg, and D. Tannor, J. Phys. Chem. 86, 1822 (1982); JPCHAX 0022-3654 10.1021/j100207a018
24. A.B. Myers, J. Chem. Phys. 77, 3857 (1982); JCPSA6 0021-9606 10.1063/1.444339
25. D. Imre, J. Phys. Chem. 88, 3956 (1984). JPCHAX 0022-3654 10.1021/j150662a017
26. P.L. Decola, J.R. Andrews, and R.M. Hochstrasser, J. Chem. Phys. 73, 4695 (1980). JCPSA6 0021-9606 10.1063/1.440664
27. N.A. Mathew, J. Phys. Chem. A 114, 817 (2010). JPCAFH 1089-5639 10.1021/jp9088063
28. J. Faeder, J. Chem. Phys. 115, 8440 (2001). JCPSA6 0021-9606 10.1063/1.1412253 (Pubitemid 33084385)
29. See supplemental material at http://link.aps.org/supplemental/10.1103/ PhysRevLett.106.170405 for a proof of the time dependence of the potential V [Eq. ] and a table containing the parameters used in the simulations.
30. J.M.D. Feit, J.A. Fleck, and A. Steinger, J. Comput. Phys. 47, 412 (1982). JCTPAH 0021-9991 10.1016/0021-9991(82)90091-2