Interactions of chelating agents with Pb-goethite at the solid-liquid interface: Pb extraction and re-adsorption

Chemosphere

Volumn 81, Issue 3, 2010, Pages 415-421

  Yip, Theo C M ^a   Tsang, Daniel C W ^b   Lo, Irene M C ^a  

^a HONG KONG UNIVERSITY OF SCIENCE AND TECHNOLOGY   (Hong Kong)

^b UNIVERSITY OF CANTERBURY   (New Zealand)

Author keywords

ATR FT IR; EDDS; EDTA; Pb extraction; Solid liquid interface; Zwitterions

Indexed keywords

ADSORPTION; ALKALINITY; BIODEGRADABILITY; CHELATION; ETHYLENEDIAMINETETRAACETIC ACID; HYDROGEN BONDS; ISOMERS; LIQUIDS; MORPHOLOGY; PARTICLE SIZE; PHASE INTERFACES; PLANTS (BOTANY); SOIL CONSERVATION; SOIL POLLUTION;

ATR/FT-IR; ATTENUATED TOTAL REFLECTANCE FOURIER TRANSFORM INFRARED; EDDS; EXTRACTION EFFICIENCIES; INTRA-MOLECULAR HYDROGEN BONDS; SOLID-LIQUID INTERFACES; ZWITTERIONIC STRUCTURE; ZWITTERIONS;

EXTRACTION;

AMINE; AMPHOLYTE; CARBOXYL GROUP; EDETIC ACID; ETHYLENEDIAMINE DISUCCINATE; FERRIC HYDROXIDE; LEAD; SUCCINIC ACID; UNCLASSIFIED DRUG;

ADSORPTION; BIODEGRADATION; CHELATING AGENT; EDTA; FTIR SPECTROSCOPY; GOETHITE; LEAD; PARTICLE SIZE; PH; SOIL REMEDIATION; SURFACE AREA; TOXICITY;

ADSORPTION; ALKALINITY; AQUEOUS SOLUTION; ARTICLE; CHEMICAL STRUCTURE; EXTRACTION; HYDROGEN BOND; INFRARED SPECTROSCOPY; ISOMER; LIQUID PHASE MICROEXTRACTION; PH MEASUREMENT; PROTON TRANSPORT; REFLECTOMETRY; SOLID PHASE EXTRACTION;

EID: 79951856399     PISSN: 00456535     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.chemosphere.2010.06.069     Document Type: Article

References (36)

1. Bargar J.R., Persson P., Brown G.E. Outer-sphere adsorption of Pb(II)EDTA on goethite. Geochim. Cosmochim. Acta 1999, 63:2957-2969.
2. Chapman D. An infrared and nuclear magnetic resonance study of the nature of ethylenediaminetetra-acetic acid and some related substances in solution: hydrogen bonding in α-amino-polycarboxylic acid systems. J. Chem. Soc. 1963, 686:3645-3658.
3. Cornell R.M., Schwertmann U. The Iron Oxides 2003, Verlag Chemie, Berlin. second ed.
4. Duckworth O.W., Martin S.T. Surface complexation and dissolution of hematite by C1-C6 dicarboxylic acids at pH=5.0. Geochim. Cosmochim. Acta 2001, 65:4289-4301.
5. Elless M.P., Bray C.A., Blaylock M.J. Chemical behavior of residential lead in urban yards in the United States. Environ. Pollut. 2007, 148:291-300.
6. Elzinga E.J., Sparks D.L. X-ray absorption spectroscopy study of the effects of pH and ionic strength on Pb (II) sorption to amorphous silica. Environ. Sci. Technol. 2002, 36:4352-4357.
7. Gustafsson, J.P., 2008. Visual MINTEQ Version 2.53. Department of Land and Water Resources Engineering, Royal Institute of Technology, Stockholm, Sweden.
8. Heil D.M., Samani Z., Hanson A.T., Rudd B. Remediation of lead contaminated soil by EDTA. I. Batch and column studies. Water Air Soil Pollut. 1999, 75:205-225.
9. 2 in the aqueous phase. Langmuir 1994, 10:3587-3597.
10. Komarek M., Vanek A., Szakova J., Balik J., Chrastny V. Interactions of EDDS with Fe- and Al-(hydr)oxides. Chemosphere 2009, 77:87-93.
11. Lanigan K.C., Pidsosny K. Reflectance FTIR spectroscopic analysis of metal complexation to EDTA and EDDS. Vib. Spectrosc. 2007, 45:2-9.
12. Martell A.E., Smith R.M., Motekaitis R.J. NIST Critically Selected Stability Constants of Metal Complexes, Version 8.0 2004, National Institute of Standards and Technology, Gaithersburg, MD.
13. Mulligan C.N., Yong R.N., Gibbs B.F. Remediation technologies for metal-contaminated soils and groundwater: an evaluation. Eng. Geol. 2001, 60:193-207.
14. Nissen M.S., Youn B., Knowles B.D., Ballinger J.W., Jun S., Belchik S.M., Xun L., Kang C. Crystal structures of NADH:FMN oxidoreductase (EmoB) at different stages of catalysis. J. Biol. Chem. 2008, 283:28710-28720.
15. Noren K., Loring J.S., Persson P. Adsorption of alpha amino acids at the water/goethite interface. J. Colloid Interface Sci. 2008, 319:416-428.
16. Noren K., Loring J.S., Bargar J.R., Persson P. Adsorption mechanisms of EDTA at the water-iron oxide interface. Implications for dissolution. J. Phys. Chem. C 2009, 113:7762-7771.
17. Nowack B. Environmental chemistry of aminopolycarboxylate chelating agents. Environ. Sci. Technol. 2002, 36:4009-4016.
18. Nowack B., Sigg L. Adsorption of EDTA and metal-EDTA complexes onto goethite. J. Colloid Interface Sci. 1996, 177:106-121.
19. Paul C., Ford R., Wilkin R.T. Assessing the selectivity of extractant solutions for recovering labile arsenic associated with iron (hydro) oxides and sulfides in sediments. Geoderma 2009, 152:137-144.
20. Peters R.W. Chelant extraction of heavy metals from contaminated soils. J. Hazard. Mater. 1999, 66:151-210.
21. Pimentel G.C., McClellan A.L. The Hydrogen Bond 1960, Reinhold Publishing Corporation, New York.
22. Ryczkowski J. Spectroscopic evidences of EDTA interaction with inorganic supports during the preparation of supported metal catalysts. Vib. Spectrosc. 2007, 43:203-209.
23. Sparks D.L. Environmental Soil Chemistry 2003, Academic Press, Amsterdam. second ed.
24. Stumm W. Reactivity at the mineral-water interface. Dissolution and inhibition. Colloids Surf. 1997, 120:143-166.
25. Sun B., Zhao F.J., Lombi E., McGrath S.P. Leaching of heavy metals from contaminated soils using EDTA. Environ. Pollut. 2001, 113:111-120.
26. Tandy S., Bossart K., Mueller R., Ritschel J., Hauser L., Schulin R., Nowack B. Extraction of heavy metals from soils using biodegradable chelating agents. Environ. Sci. Technol. 2004, 38:937-944.
27. Tsang D.C.W., Zhang W., Lo I.M.C. Copper extraction effectiveness and soil dissolution issues of EDTA-flushing of artificially contaminated soils. Chemosphere 2007, 68:234-243.
28. Tsang D.C.W., Lo I.M.C., Chan K.L. Modeling the transport of metals with rate-limited EDTA-promoted extraction and dissolution during EDTA-flushing of copper-contaminated soils. Environ. Sci. Technol. 2007, 41:3660-3667.
29. Tsang D.C.W., Yip T.C.M., Lo I.M.C. Kinetic interactions of EDDS with soils. 2. Metal-EDDS complexes in uncontaminated and metal-contaminated soils. Environ. Sci. Technol. 2009, 43:837-842.
30. Vandevivere P.C., Hammes F., Verstraete W., Feijtel T., Schowanek D. Metal decontamination of soil, sediment, and sewage sludge by means of transition metal chelant [S,S]-EDDS. J. Environ. Eng. 2001, 127:802-811.
31. Yip T.C.M., Tsang D.C.W., Ng K.T.W., Lo I.M.C. Kinetic interactions of EDDS with soils: 1. Metal resorption and competition under EDDS deficiency. Environ. Sci. Technol. 2009, 43:831-836.
32. Yip T.C.M., Tsang D.C.W., Ng K.T.W., Lo I.M.C. Empirical modeling of heavy metal extraction by EDDS from single-metal and multi-metal contaminated soils. Chemosphere 2009, 74:301-307.
33. Yoon T.H., Johnson S.B., Musgrave C.B., Brown G.E. Adsorption of organic matter at mineral/water interfaces: I. ATR/FT-IR spectroscopic and quantum chemical study of oxalate adsorbed at boehmite/water and corundum/water interfaces. Geochim. Cosmochim. Acta 2004, 68:4505-4518.
34. Zhang W., Tsang D.C.W., Lo I.M.C. Removal of MDF and Pb from contaminated soils by EDTA- and SDS-enhanced washing. Chemosphere 2007, 66:2025-2034.
35. Zhang H., Herman J.P., Bolton H., Zhang Z., Clark S., Xun L. Evidence that bacterial ABC-type transporter imports free EDTA for metabolism. J. Appl. Bacteriol. 2007, 189:7991-7997.
36. Zou Z., Qiu R., Zhang W., Dong H., Zhao Z., Zhang T., Wei X., Cai X. The study of operating variables in soil washing with EDTA. Environ. Pollut. 2009, 157:229-236.