메뉴 건너뛰기




Volumn 132, Issue 3, 2010, Pages

Probe molecules in polymer melts near the glass transition: A molecular dynamics study of chain length effects

Author keywords

[No Author keywords available]

Indexed keywords

AUTOCORRELATION FUNCTIONS; CAGE EFFECT; CENTER OF MASS; COARSE GRAINED MODELS; CRITICAL TEMPERATURES; DENSE MELT; FLUORESCENT PROBE MOLECULES; FUNCTION OF TIME; GLASS TRANSITION TEMPERATURE; INCOHERENT SCATTERING FUNCTIONS; LINEAR DICHROISM; MATRIX; MEAN-SQUARE DISPLACEMENT; MODE COUPLING; MODE COUPLING THEORY; MOLECULAR DYNAMICS SIMULATIONS; POLYMER CHAINS; PROBE MOLECULES; STOKES-EINSTEIN RELATION; TIME EVOLUTIONS; VOGEL-FULCHER;

EID: 78651445929     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.3284780     Document Type: Article
Times cited : (17)

References (66)
  • 3
    • 0037213549 scopus 로고    scopus 로고
    • Glass transition of polymer melts: Test of theoretical concepts by computer simulation
    • DOI 10.1016/S0079-6700(02)00030-8, PII S0079670002000308
    • K. Binder, J. Baschnagel, and W. Paul, Prog. Polym. Sci. 0079-6700 28, 115 (2003). 10.1016/S0079-6700(02)00030-8 (Pubitemid 35465707)
    • (2003) Progress in Polymer Science (Oxford) , vol.28 , Issue.1 , pp. 115-172
    • Binder, K.1    Baschnagel, J.2    Paul, W.3
  • 6
    • 0033548657 scopus 로고    scopus 로고
    • Illuminating single molecules in condensed matter
    • DOI 10.1126/science.283.5408.1670
    • W. E. Moerner and M. Orrit, Science 0036-8075 283, 1670 (1999). 10.1126/science.283.5408.1670 (Pubitemid 29143792)
    • (1999) Science , vol.283 , Issue.5408 , pp. 1670-1676
    • Moerner, W.E.1    Orrit, M.2
  • 7
    • 0001468698 scopus 로고    scopus 로고
    • 0066-426X,. 10.1146/annurev.physchem.49.1.441
    • X. -S. Xie and J. K. Trautmann, Annu. Rev. Phys. Chem. 0066-426X 49, 441 (1998). 10.1146/annurev.physchem.49.1.441
    • (1998) Annu. Rev. Phys. Chem. , vol.49 , pp. 441
    • Xie, X.-S.1    Trautmann, J.K.2
  • 8
    • 3342951259 scopus 로고    scopus 로고
    • 0066-426X,. 10.1146/annurev.physchem.54.011002.103816
    • F. Kulzer and M. Orrit, Annu. Rev. Phys. Chem. 0066-426X 55, 585 (2004). 10.1146/annurev.physchem.54.011002.103816
    • (2004) Annu. Rev. Phys. Chem. , vol.55 , pp. 585
    • Kulzer, F.1    Orrit, M.2
  • 10
    • 0037038585 scopus 로고    scopus 로고
    • Heterogeneous dynamics and domains in supercooled o-terphenyl: A single molecule study
    • DOI 10.1021/jp025843m
    • L. A. Deschenes and D. A. Vanden Bout, J. Phys. Chem. B 1089-5647 106, 11438 (2002). 10.1021/jp025843m (Pubitemid 35369301)
    • (2002) Journal of Physical Chemistry B , vol.106 , Issue.44 , pp. 11438-11445
    • Deschenes, L.A.1    Vanden Bout, D.A.2
  • 15
    • 0012112253 scopus 로고    scopus 로고
    • Orientational imaging of single molecules by annular illumination
    • DOI 10.1103/PhysRevLett.85.4482
    • B. Sick, B. Hecht, and L. Novotny, Phys. Rev. Lett. 0031-9007 85, 4482 (2000). 10.1103/PhysRevLett.85.4482 (Pubitemid 32024871)
    • (2000) Physical Review Letters , vol.85 , Issue.21 , pp. 4482-4485
    • Sick, B.1    Hecht, B.2    Novotny, L.3
  • 17
    • 0038512550 scopus 로고    scopus 로고
    • 0740-3224,. 10.1364/JOSAB.20.000554
    • M. Böhmer and J. Enderlein, J. Opt. Soc. Am. B 0740-3224 20, 554 (2003). 10.1364/JOSAB.20.000554
    • (2003) J. Opt. Soc. Am. B , vol.20 , pp. 554
    • Böhmer, M.1    Enderlein, J.2
  • 18
    • 0037042981 scopus 로고    scopus 로고
    • 0031-9007,. 10.1103/PhysRevLett.89.026101
    • A. P. Bartko, K. Xu, and R. M. Dickson, Phys. Rev. Lett. 0031-9007 89, 026101 (2002). 10.1103/PhysRevLett.89.026101
    • (2002) Phys. Rev. Lett. , vol.89 , pp. 026101
    • Bartko, A.P.1    Xu, K.2    Dickson, R.M.3
  • 20
    • 18644383173 scopus 로고    scopus 로고
    • Fluorescence lifetime fluctuations of single molecules probe local density fluctuations in disordered media: A bulk approach
    • DOI 10.1063/1.1861881, 114704
    • R. A. L. Valĺe, N. Tomczak, G. J. Vancso, L. Kuipers, and N. F. van Hulst, J. Chem. Phys. 0021-9606 122, 114704 (2005). 10.1063/1.1861881 (Pubitemid 40661776)
    • (2005) Journal of Chemical Physics , vol.122 , Issue.11 , pp. 1-9
    • Valle, R.A.L.1    Tomczak, N.2    Vancso, G.J.3    Kuipers, L.4    Van Hulst, N.F.5
  • 22
    • 0002805179 scopus 로고    scopus 로고
    • 0022-3093,. 10.1016/S0022-3093(98)00831-X
    • H. Sillescu, J. Non-Cryst. Solids 0022-3093 243, 81 (1999). 10.1016/S0022-3093(98)00831-X
    • (1999) J. Non-Cryst. Solids , vol.243 , pp. 81
    • Sillescu, H.1
  • 23
    • 0002055106 scopus 로고    scopus 로고
    • 0066-426X,. 10.1146/annurev.physchem.51.1.99
    • M. D. Ediger, Annu. Rev. Phys. Chem. 0066-426X 51, 99 (2000). 10.1146/annurev.physchem.51.1.99
    • (2000) Annu. Rev. Phys. Chem. , vol.51 , pp. 99
    • Ediger, M.D.1
  • 24
    • 0037124631 scopus 로고    scopus 로고
    • Heterogeneous dynamics in liquids: Fluctuations in space and time
    • DOI 10.1088/0953-8984/14/23/201, PII S0953898402267211
    • R. Richert, J. Phys.: Condens. Matter 0953-8984 14, R703 (2002). 10.1088/0953-8984/14/23/201 (Pubitemid 34715147)
    • (2002) Journal of Physics Condensed Matter , vol.14 , Issue.23
    • Richert, R.1
  • 25
    • 33751264586 scopus 로고    scopus 로고
    • Fluorescence lifetime of a single molecule as an observable of Meta-Basin dynamics in fluids near the glass transition
    • DOI 10.1103/PhysRevLett.97.217801
    • R. A. L. Valĺe, M. Van der Auweraer, W. Paul, and K. Binder, Phys. Rev. Lett. 0031-9007 97, 217801 (2006). 10.1103/PhysRevLett.97.217801 (Pubitemid 44800799)
    • (2006) Physical Review Letters , vol.97 , Issue.21 , pp. 217801
    • Vallee, R.A.L.1    Van Der Auweraer, M.2    Paul, W.3    Binder, K.4
  • 27
    • 39349106157 scopus 로고    scopus 로고
    • Single molecule probing of the glass transition phenomenon: Simulations of several types of probes
    • DOI 10.1063/1.2794334
    • R. A. L. Valĺe, W. Paul, and K. Binder, J. Chem. Phys. 0021-9606 127, 154903 (2007). 10.1063/1.2794334 (Pubitemid 351260815)
    • (2007) Journal of Chemical Physics , vol.127 , Issue.15 , pp. 154903
    • Vallee, R.A.L.1    Paul, W.2    Binder, K.3
  • 30
    • 0000423527 scopus 로고
    • 0014-3057, () (and references therein). 10.1016/0014-3057(70)90038-8
    • G. Pezzin, F. Zilio-Grande, and P. Sanmartin, Eur. Polym. J. 0014-3057 6, 1053 (1970) (and references therein). 10.1016/0014-3057(70)90038-8
    • (1970) Eur. Polym. J. , vol.6 , pp. 1053
    • Pezzin, G.1    Zilio-Grande, F.2    Sanmartin, P.3
  • 33
    • 0000428453 scopus 로고
    • 0021-9606,. 10.1063/1.461274
    • H. -P. Wittmann, J. Chem. Phys. 0021-9606 95, 8449 (1991). 10.1063/1.461274
    • (1991) J. Chem. Phys. , vol.95 , pp. 8449
    • Wittmann, H.-P.1
  • 35
    • 78651422352 scopus 로고    scopus 로고
    • See the discussion on 324 of Ref..
    • See the discussion on p. 324 of Ref..
  • 41
    • 0001463786 scopus 로고    scopus 로고
    • 1292-8941, () 10.1007/s101890170078;, Eur. Phys. J. E 1292-8941 5, 245 (2001). 10.1007/s101890170079
    • M. Aichele and J. Baschnagel, Eur. Phys. J. E 1292-8941 5, 229 (2001) 10.1007/s101890170078; M. Aichele and J. Baschnagel, Eur. Phys. J. E 1292-8941 5, 245 (2001). 10.1007/s101890170079
    • (2001) Eur. Phys. J. e , vol.5 , pp. 229
    • Aichele, M.1    Baschnagel, J.2    Aichele, M.3    Baschnagel, J.4
  • 42
    • 0037109594 scopus 로고    scopus 로고
    • Cooling rate dependence of the glass transition temperature of polymer melts: Molecular dynamics study
    • DOI 10.1063/1.1508366
    • J. Buchholz, W. Paul, F. Varnik, and K. Binder, J. Chem. Phys. 0021-9606 117, 7364 (2002). 10.1063/1.1508366 (Pubitemid 35354182)
    • (2002) Journal of Chemical Physics , vol.117 , Issue.15 , pp. 7364-7372
    • Buchholz, J.1    Paul, W.2    Varnik, F.3    Binder, K.4
  • 43
    • 23644434104 scopus 로고    scopus 로고
    • Computer simulations of supercooled polymer melts in the bulk and in confined geometry
    • DOI 10.1088/0953-8984/17/32/R02, PII S095389840538338X
    • J. Baschnagel and F. Varnik, J. Phys.: Condens. Matter 0953-8984 17, R851 (2005). 10.1088/0953-8984/17/32/R02 (Pubitemid 41130206)
    • (2005) Journal of Physics Condensed Matter , vol.17 , Issue.32
    • Baschnagel, J.1    Varnik, F.2
  • 44
    • 66149095481 scopus 로고    scopus 로고
    • (Wiley, New York), Vol.,. 10.1002/9780470189078.ch1
    • W. Paul, Reviews in Computational Chemistry (Wiley, New York, 2007), Vol. 25, p. 1. 10.1002/9780470189078.ch1
    • (2007) Reviews in Computational Chemistry , vol.25 , pp. 1
    • Paul, W.1
  • 45
    • 2942680923 scopus 로고
    • 0021-9606,. 10.1063/1.1672587
    • M. Goldstein, J. Chem. Phys. 0021-9606 51, 3728 (1969). 10.1063/1.1672587
    • (1969) J. Chem. Phys. , vol.51 , pp. 3728
    • Goldstein, M.1
  • 46
    • 4243264015 scopus 로고
    • 1050-2947,. 10.1103/PhysRevA.28.2408
    • F. H. Stillinger and T. H. Weber, Phys. Rev. A 1050-2947 28, 2408 (1983). 10.1103/PhysRevA.28.2408
    • (1983) Phys. Rev. A , vol.28 , pp. 2408
    • Stillinger, F.H.1    Weber, T.H.2
  • 47
    • 0347947118 scopus 로고    scopus 로고
    • 0031-9007,. 10.1103/PhysRevLett.91.235501
    • B. Doliwa and A. Heuer, Phys. Rev. Lett. 0031-9007 91, 235501 (2003). 10.1103/PhysRevLett.91.235501
    • (2003) Phys. Rev. Lett. , vol.91 , pp. 235501
    • Doliwa, B.1    Heuer, A.2
  • 52
    • 4644335930 scopus 로고    scopus 로고
    • 0021-9606,. 10.1063/1.1776553
    • J. Kim and T. Keyes, J. Chem. Phys. 0021-9606 121, 4237 (2004). 10.1063/1.1776553
    • (2004) J. Chem. Phys. , vol.121 , pp. 4237
    • Kim, J.1    Keyes, T.2
  • 53
    • 33748576917 scopus 로고    scopus 로고
    • Are there localized saddles behind the heterogeneous dynamics of supercooled liquids?
    • DOI 10.1209/epl/i2006-10175-8
    • D. Coslovich and G. Pastore, Europhys. Lett. 0295-5075 75, 784 (2006). 10.1209/epl/i2006-10175-8 (Pubitemid 44369676)
    • (2006) Europhysics Letters , vol.75 , Issue.5 , pp. 784-790
    • Coslovich, D.1    Pastore, G.2
  • 54
    • 33244492445 scopus 로고    scopus 로고
    • Democratic particle motion for metabasin transitions in simple glass formers
    • DOI 10.1103/PhysRevLett.96.057801
    • G. A. Appignanesi, J. A. Rodrigues Fris, R. A. Montani, and W. Kob, Phys. Rev. Lett. 0031-9007 96, 057801 (2006). 10.1103/PhysRevLett.96.057801 (Pubitemid 43273474)
    • (2006) Physical Review Letters , vol.96 , Issue.5 , pp. 057801
    • Appignanesi, G.A.1    Fris, J.A.R.2    Montani, R.A.3    Kob, W.4
  • 55
    • 0004986545 scopus 로고
    • 0034-4885,. 10.1088/0034-4885/55/3/001
    • W. Götze and L. Sjögren, Rep. Prog. Phys. 0034-4885 55, 241 (1992). 10.1088/0034-4885/55/3/001
    • (1992) Rep. Prog. Phys. , vol.55 , pp. 241
    • Götze, W.1    Sjögren, L.2
  • 56
    • 4243104032 scopus 로고
    • 0034-4885,. 10.1088/0034-4885/49/2/002
    • J. Jäckle, Rep. Prog. Phys. 0034-4885 49, 171 (1986). 10.1088/0034-4885/49/2/002
    • (1986) Rep. Prog. Phys. , vol.49 , pp. 171
    • Jäckle, J.1
  • 57
  • 58
    • 0000119222 scopus 로고
    • 0369-982X, ();, J. Am. Ceram. Soc. 0002-7820 8, 339 (1925). 10.1111/j.1151-2916.1925.tb16731.x
    • H. Vogel, Phys. Z. 0369-982X 22, 645 (1921); G. S. Fulcher, J. Am. Ceram. Soc. 0002-7820 8, 339 (1925). 10.1111/j.1151-2916.1925.tb16731.x
    • (1921) Phys. Z. , vol.22 , pp. 645
    • Vogel, H.1    Fulcher, G.S.2
  • 59
    • 78651422683 scopus 로고    scopus 로고
    • The software package OCTA () was used.
    • The software package OCTA (http://octa.jp) was used.
  • 60
    • 0004036594 scopus 로고    scopus 로고
    • edited by K. Binder and G. Ciccotti (Societa Italiana di Fisica, Bologna).
    • Monte Carlo and Molecular Dynamics of Condensed Matter, edited by, K. Binder, and, G. Ciccotti, (Societa Italiana di Fisica, Bologna, 1996).
    • (1996) Monte Carlo and Molecular Dynamics of Condensed Matter
  • 61
    • 0036830563 scopus 로고    scopus 로고
    • 0301-0104,. 10.1016/S0301-0104(02)00536-0
    • W. Paul, Chem. Phys. 0301-0104 284, 59 (2002). 10.1016/S0301-0104(02) 00536-0
    • (2002) Chem. Phys. , vol.284 , pp. 59
    • Paul, W.1
  • 65
    • 33746869252 scopus 로고    scopus 로고
    • What can be learned about molecular reorientation from single molecule polarization microscopy?
    • DOI 10.1063/1.2227395
    • M. F. Gelin and D. S. Kosov, J. Chem. Phys. 0021-9606 125, 054708 (2006). 10.1063/1.2227395 (Pubitemid 44188432)
    • (2006) Journal of Chemical Physics , vol.125 , Issue.5 , pp. 054708
    • Gelin, M.F.1    Kosov, D.S.2
  • 66
    • 33749256240 scopus 로고    scopus 로고
    • Effect of finite trajectory length on the correlation function analysis of single molecule data
    • DOI 10.1063/1.2352748
    • C. -Y. Lu and D. A. Vanden Bout, J. Chem. Phys. 0021-9606 125, 124701 (2006). 10.1063/1.2352748 (Pubitemid 44484215)
    • (2006) Journal of Chemical Physics , vol.125 , Issue.12 , pp. 124701
    • Lu, C.-Y.1    Vanden Bout, D.A.2


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.