Strong field effects in rotational femtosecond degenerate four-wave mixing

Journal of Chemical Physics

Volumn 132, Issue 13, 2010, Pages

  Gelin, Maxim F ^a   Riehn, Christoph ^b   Kunitski, Maksim ^c   Brutschy, Bernhard ^c  

^a TECHNICAL UNIVERSITY OF MUNICH   (Germany)

^b Rheinland Pfälzische Technische Universität Kaiserslautern Landau   (Germany)

^c GOETHE UNIVERSITY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

DEGENERATE FOUR-WAVE MIXING; FEMTOSECONDS; HETERODYNE DETECTION; HIGH INTENSITY LASER PULSE; LASER INTENSITIES; NON-ADIABATIC; NONPERTURBATIVE; PERTURBATIVE APPROACH; STRONG FIELD;

ALIGNMENT;

FOUR WAVE MIXING;

EID: 78649762217     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.3367726     Document Type: Article

References (49)

1. H. Stapelfeldt and T. Seideman, Rev. Mod. Phys. RMPHAT 0034-6861 75, 543 (2003). 10.1103/RevModPhys.75.543
2. T. Seideman and E. Hamilton, Adv. At., Mol., Opt. Phys. AAMPE9 1049-250X 52, 289 (2005). 10.1016/S1049-250X(05)52006-8
3. P. M. Felker, J. Phys. Chem. JPCHAX 0022-3654 96, 7844 (1992). 10.1021/j100199a005
4. P. M. Felker and A. H. Zewail, in Femtochemistry, edited by, J. Manz, and, L. Wöste, (VCH, New York, 1994), Vol. I, pp. 193-260.
5. C. Riehn, Chem. Phys. CMPHC2 0301-0104 283, 297 (2002). 10.1016/S0301-0104(02)00572-4
6. S. Mukamel, Principles of Nonlinear Optical Spectroscopy (Oxford University Press, New York, 1995), Chap.
7. B. I. Grimberg, V. V. Lozovoy, M. Dantus, and S. Mukamel, J. Phys. Chem. A JPCAFH 1089-5639 106, 697 (2002). 10.1021/jp010451l
8. B. Lavorel, H. Tran, E. Hertz, O. Faucher, P. Joubert, M. Motzkus, T. Buckup, T. Lang, H. Skenderovi, G. Knopp, P. Beaud, and H. M. Frey, C. R. Phys. CRPOBN 1631-0705 5, 215 (2004). 10.1016/j.crhy.2004.01.013
9. E. J. Brown, Q. Zhang, and M. Dantus, J. Chem. Phys. JCPSA6 0021-9606 110, 5772 (1999). 10.1063/1.478476
10. M. Morgen, W. Price, L. Hunziker, P. Ludowise, M. Blackwell, and Y. Chen, Chem. Phys. Lett. CHPLBC 0009-2614 209, 1 (1993). 10.1016/0009-2614(93)87192-6
11. M. Morgen, W. Price, L. Hunziker, P. Ludowise, and Y. Chen, J. Chem. Phys. JCPSA6 0021-9606 102, 8780 (1995). 10.1063/1.468931
12. M. Comstock, V. Senekerimyan, and M. Dantus, J. Phys. Chem. A JPCAFH 1089-5639 107, 8271 (2003). 10.1021/jp0278115
13. (a) V. V. Matylitsky, W. Jarzba, C. Riehn, and B. Brutschy, J. Raman Spectrosc. JRSPAF 0377-0486 33, 877 (2002) 10.1002/jrs.945; (b) V. V. Matylitsky and C. Riehn (unpublished).
14. W. Jarzba, V. V. Matylitsky, C. Riehn, and B. Brutschy, Chem. Phys. Lett. CHPLBC 0009-2614 368, 680 (2003). 10.1016/S0009-2614(02)01927-9
15. V. G. Stavros, E. Harel, and S. R. Leone, J. Chem. Phys. JCPSA6 0021-9606 122, 064301 (2005). 10.1063/1.1843817
16. V. G. Stavros and S. R. Leone, Chem. Phys. Lett. CHPLBC 0009-2614 452, 33 (2008). 10.1016/j.cplett.2007.12.034
17. V. Renard, M. Renard, S. Gúrin, Y. T. Pashayan, B. Lavorel, O. Faucher, and H. R. Jauslin, Phys. Rev. Lett. PRLTAO 0031-9007 90, 153601 (2003). 10.1103/PhysRevLett.90.153601
18. A. Rouźe, V. Renard, S. Gúrin, O. Faucher, and B. Lavorel, J. Raman Spectrosc. JRSPAF 0377-0486 38, 969 (2007). 10.1002/jrs.1679
19. A. Rouźe, V. Renard, S. Gúrin, O. Faucher, and B. Lavorel, Phys. Rev. A PLRAAN 1050-2947 75, 013419 (2007). 10.1103/PhysRevA.75.013419
20. Y. Mairesse, D. Zeidler, N. Dudovich, M. Spanner, J. Levesque, D. M. Villeneuve, and P. B. Corkum, Phys. Rev. Lett. PRLTAO 0031-9007 100, 143903 (2008). 10.1103/PhysRevLett.100.143903
21. M. D. Poulsen, E. Ṕronne, H. Stapelfeldt, C. Z. Bisgaard, S. S. Viftrup, E. Hamilton, and T. Seideman, J. Chem. Phys. JCPSA6 0021-9606 121, 783 (2004). 10.1063/1.1760731
22. M. F. Gelin, C. Riehn, V. V. Matylitsky, and B. Brutschy, Chem. Phys. CMPHC2 0301-0104 290, 307 (2003). 10.1016/S0301-0104(03)00172-1
23. T. Steffen, J. T. Fourkas, and K. Duppen, J. Chem. Phys. JCPSA6 0021-9606 105, 7364 (1996). 10.1063/1.472594
24. M. F. Gelin, D. Egorova, and W. Domcke, J. Chem. Phys. JCPSA6 0021-9606 131, 194103 (2009). 10.1063/1.3265213
25. 1 (t) is not considered explicitly, since it does not obey the phase matching conditions and disappears upon the action of projector.
26. 2 (t′) =1/2.
27. The difference of k-values in Ref. and in the present paper is caused by different normalizations of the nonlinear response functions.
28. L. Jensen, P. O. Åstrand, A. Osted, J. Kongsted, and K. V. Mikkelsen, J. Chem. Phys. JCPSA6 0021-9606 116, 4001 (2002). 10.1063/1.1433747
29. M. Castillejo, S. Couris, E. Koudoumas, and M. Martín, Chem. Phys. Lett. CHPLBC 0009-2614 308, 373 (1999). 10.1016/S0009-2614(99)00636-3
30. S. Fleischer, I. Sh. Averbukh, and Y. Prior, J. Phys. B JPAPEH 0953-4075 41, 074018 (2008). 10.1088/0953-4075/41/7/074018
31. K. F. Lee, I. V. Litvinyuk, P. W. Dooley, M. Spanner, D. M. Villeneuve, and P. B. Corkum, J. Phys. B JPAPEH 0953-4075 37, L43 (2004). 10.1088/0953-4075/37/3/L02
32. C. Z. Bisgaard, M. D. Poulsen, E. Ṕronne, S. S. Viftrup, and H. Stapelfeldt, Phys. Rev. Lett. PRLTAO 0031-9007 92, 173004 (2004). 10.1103/PhysRevLett.92.173004
33. 2. This causes an effective twice shortening of the period of rotational recurrences, see, e.g., Refs.
34. H. -M. Frey, P. Beaud, T. Gerber, B. Mischler, P. P. Radi, and A. P. Tzannis, Appl. Phys. B: Lasers Opt. APBOEM 0946-2171 68, 739 (1999).
35. C. Riehn, M. I. Kunitski, V. V. Matylitsky, M. F. Gelin, and B. Brutschy, Phys. Chem. Chem. Phys. PPCPFQ 1463-9076 7, 3955 (2005). 10.1039/b510363k
36. M. Leibscher, I. Sh. Averbukh, and H. Rabitz, Phys. Rev. Lett. PRLTAO 0031-9007 90, 213001 (2003). 10.1103/PhysRevLett.90.213001
37. M. Leibscher, I. Sh. Averbukh, and H. Rabitz, Phys. Rev. A PLRAAN 1050-2947 69, 013402 (2004). 10.1103/PhysRevA.69.013402
38. K. Hartinger and R. A. Bartels, J. Opt. Soc. Am. B JOBPDE 0740-3224 25, 407 (2008). 10.1364/JOSAB.25.000407
39. O R (t) was calculated via the trapezoidal integration formula. Eleven points were found to be enough for getting convergent results in all our calculations.
40. See Appendix for a more mathematically oriented discussion of this question.
41. A. Kumara, W. J. Meatha, P. Bündgen, and A. J. Thakkar, J. Chem. Phys. JCPSA6 0021-9606 105, 4297 (1996).
42. A. S. Meijer, Y. Zhang, D. H. Parker, W. J. van der Zande, A. Gijsbertsen, and M. J. J. Vrakking, Phys. Rev. A PLRAAN 1050-2947 76, 023411 (2007). 10.1103/PhysRevA.76.023411
43. H. Hasegawa, and Y. Ohshima, J. Phys.: Conf. Ser. JPCSDZ 1742-6588 185, 012014 (2009). 10.1088/1742-6596/185/1/012014
44. N. Owschimikow, B. Schmidt, and N. Schwentner, Phys. Rev. A PLRAAN 1050-2947 80, 053409 (2009). 10.1103/PhysRevA.80.053409
45. C. Wu, G. Zeng, Y. Gao, N. Xu, L. -Y. Peng, H. Jiang, and Q. Gong, J. Chem. Phys. JCPSA6 0021-9606 130, 231102 (2009). 10.1063/1.3155063
46. V. Loriot, E. Hertz, B. Lavorel, and O. Faucher, J. Phys. B JPAPEH 0953-4075 41, 015604 (2008). 10.1088/0953-4075/41/1/015604
47. A. P. Blokhin, M. F. Gelin, I. I. Kalosha, S. A. Polubisok, and V. A. Tolkachev, J. Chem. Phys. JCPSA6 0021-9606 110, 978 (1999). 10.1063/1.477918
48. D. A. Varshalovich, A. N. Moskalev, and V. K. Hersonski, Quantum Theory of Angular Momentum (World Scientific, Singapore, 1989).
49. 2 r, the projection operator in Eq. should be modified accordingly.