The resistance of polyelectrolyte multilayers in a free-hanging configuration

Journal of Physical Chemistry B

Volumn 114, Issue 44, 2010, Pages 13982-13987

  Sugihara, Kaori ^a   Vörös, János ^a   Zambelli, Tomaso ^a  

^a ETH ZURICH   (Switzerland)

Author keywords

[No Author keywords available]

Indexed keywords

ATOMIC SPECTROSCOPY; ELECTROCHEMICAL CORROSION; MULTILAYERS; POLYELECTROLYTES;

AFM; ATOMIC FORCE; CONVENTIONAL SYSTEMS; ELECTRODE SYSTEMS; ORDERS OF MAGNITUDE; POLYELECTROLYTE MULTILAYER; REDOX-ACTIVE;

ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY;

EID: 78149231402     PISSN: 15206106     EISSN: 15205207     Source Type: Journal    
DOI: 10.1021/jp107362y     Document Type: Article

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34. By neglecting the PEM film outside of the pore, the calculated resistivity is slightly overestimated as we saw in the case with the buffer solution previously. However, this is not relevant since only orders of magnitude are taken into account in the discussion.
35. One may suppose the change in the spectra may not be due to the change in the resistance but the capacitance. In the following fitting, indeed the fluctuation in the capacitance was also obtained, however, the feature of the resistance resulting from the fitting was well-correlated with the EIS spectra in low frequency, indicating that it dominantly represents the resistance change.
36. -) but not positively charged ones.