Novel inherently flame-retardant poly(trimethylene terephthalate) copolyester with the phosphorus-containing linking pendent group

Industrial and Engineering Chemistry Research

Volumn 49, Issue 15, 2010, Pages 7052-7059

  Chen, Hong Bing ^a   Zhang, Yi ^a   Chen, Li ^a   Shao, Zhu Bao ^a   Liu, Ya ^a   Wang, Yu Zhong ^a  

^a SICHUAN UNIVERSITY   (China)

Author keywords

[No Author keywords available]

Indexed keywords

CHEMICAL STRUCTURE; CONE CALORIMETER; COPOLYESTERS; FLAME RETARDANCY; FLAME RETARDANT PROPERTIES; INITIAL DECOMPOSITION TEMPERATURES; INTRINSIC VISCOSITY; LIMITING OXYGEN INDEX; MELTING TEMPERATURES; NITROGEN ATMOSPHERES; PENDENT GROUPS; PHOSPHORUS CONTENTS; POLY (TRIMETHYLENE TEREPHTHALATE); TEREPHTHALIC ACIDS; THERMAL BEHAVIORS; TRIMETHYLENE;

DIFFERENTIAL SCANNING CALORIMETRY; ESTERS; FLAME RETARDANTS; FLAMMABILITY; OXYGEN; PHOSPHORUS; POLYCONDENSATION; PROPANE;

THERMOGRAVIMETRIC ANALYSIS;

EID: 77955044159     PISSN: 08885885     EISSN: 15205045     Source Type: Journal    
DOI: 10.1021/ie1006917     Document Type: Article

References (43)

1. Chuah, H. H.; Lin-Vien, D.; Soni, U. Poly(trimethylene terephthalate) molecular weight and Mark-Houwink equation Polymer 2001, 42, 7137-7139
2. Dangayach, K.; Chuah, H. H.; Gergen, W.; Dalton, P.; Smith, F. Plastic-saving planet earth 55th Annu. Tech. Conf. Proc. 1997, 55, 2097
3. Schultz, J. M.; Wu, J. Poly(trimethylene terephthalate)-a newly commercialized member of the polyester family. In Handbook of Thermoplastic Polymers: Homopolymers, Copolymers, Blends, and Composites; Fakirov, S., Ed.; Wiley: Weinheim; 2002; Chapter 12, pp 551 - 578.
4. Srimoaon, P.; Dangseeyun, N.; Supaphol, P. Multiple melting behavior in isothermally crystallized poly(trimethylene terephthalate) Eur. Polym. J. 2004, 40, 599-608
5. Chuah, H. H. Crystallization kinetics of poly(trimethylene terephthalate) Polym. Eng. Sci. 2001, 41, 308-313
6. Chuang, W. T.; Hong, P. D.; Chuah, H. H. Effects of crystallization behavior on morphological change in poly(trimethylene terephthalate) spherulites Polymer 2004, 45, 2413-2415
7. Apiwanthanakorn, N.; Supaphol, P.; Nithitanakul, M. Non-isothermal melt-crystallization kinetics of poly(trimethylene terephthalate) Polym. Test 2004, 23, 817-826
8. Eberl, A.; Heumann, S.; Kotek, R.; Kaufmann, F.; Mitsche, S.; Cavaco-Paulo, A.; Gubitz, G. M. Enzymatic hydrolysis of PTT polymers and oligomers J. Biotechnol. 2008, 135, 45-51
9. Wang, Y. J.; Liu, W. Y.; Zhang, H. R. The morphology and non-isothermal crystallization characteristics of poly(trimethylene terephthalate)/BaSO4 nanocomposites prepared by in situ polycondensation Polym. Test 2009, 28, 402-411
10. Hao, J.; Liu, H. J.; Liu, D. H. Novel route of reactive extraction to recover 1,3-propanediol from a dilute aqueous solution Ind. Eng. Chem. Res. 2005, 44, 4380-4385
11. McAndrew, F. B.; Freed, W. T. Polyalkylene terphthalate resin compositions. GB Patent 147336, May 11, 1977.
12. Kenji, M.; Masaaki, N.; Hiroshi, K.; Tomomi, N.; Akiyoshi, S. Flame-retardant polyester resin composition and its production. JP Patent 3115195 (B), September 5, 1995.
13. Chang, S. J.; Chang, F. C. Synthesis and characterization of copolyesters containing the phosphorus linking pendent groups J. Appl. Polym. Sci. 1999, 72, 109-122
14. Levchik, S. V.; Weil, E. D. Flame retardancy of thermoplastic polyester-a review of the recent literature Polym. Int. 2005, 54, 11-35
15. Chen, L.; Wang, Y. Z. A review on flame retardant technology in China. Part I: development of flame retardants Polym. Adv. Technol. 2010, 21, 1-26
16. Asrar, J.; Berger, P. A.; Hurlbut, J. Synthesis and characterization of a fire-retardant polyester: Copolymers of ethylene terephthalate and 2-carboxyethyl(phenylphosphinic) acid J. Poly. Sci. Part A: Polym. Chem. 1999, 37, 3119-3128
17. Wang, L. S.; Wang, X. L.; Yan, G. L. Synthesis, characterisation and flame retardance behaviour of poly(ethylene terephthalate) copolymer containing triaryl phosphine oxide Polym. Degrad. Stab. 2000, 69, 127-130
18. Ma, Z. L.; Zhao, W. G.; Liu, Y. F.; Shi, J. R. Synthesis and properties of intumescent, phosphorus-containing, flame-retardant polyesters J. Appl. Polym. Sci. 1997, 63, 1511-1515
19. Shyr, T. W.; Lo, C. M.; Ye, S. R. Sequence distribution and crystal structure of poly (ethylene/trimethylene terephthalate) copolyesters Polymer 2005, 46, 5284-5298
20. Wei, G. F.; Hua, D. B.; Gu, L. X. Thermal stability of poly(ethylene-co-trimethylene terephthalate)s J. Appl. Polym. Sci. 2006, 101, 3330-3335
21. Kiibler, K. S.; Kelsey, D. R.; Tutunjian, P. N. Thermal stability of poly(trimethylene terephthalate) Polymer 2005, 46, 8937-8946
22. Chang, S. J.; Sheen, Y. C.; Chang, R. S.; Chang, F. C. The thermal degradation of phosphorus-containing copolyesters Polym. Degrad. Stab. 1996, 54, 365-371
23. Wu, B.; Wang, Y. Z.; Wang, X. L.; Yang, K. K.; Jin, Y. D.; Zhao, H. Kinetics of thermal oxidative degradation of phosphorus-containing flame retardant copolyesters Polym. Degrad. Stab. 2002, 76, 401-409
24. Zhao, H.; Wang, Y. Z.; Wang, D. Y.; Wu, B.; Chen, D. Q.; Wang, X. L.; Yang, K. K. Kinetics of thermal degradation of flame retardant copolyesters containing phosphorus linked pendent groups Polym. Degrad. Stab. 2003, 80, 135-140
25. Lustig, S. R.; Burch, R. R.; McCarron, I. E. Catalysis with titanium oxides. U.S. Patent 6,034,203, 2000.
26. Papageorgiou, G. Z.; Vassiliou, A. A.; Karavelidis, V. D.; Koumbis, A.; Bikiaris, D. N. Novel poly(propylene terephthalate-co-suceinate) random copolymers: Synthesis, solid structure, and enzymatic degradation study Macromolecules 2008, 41, 1675-1684
27. Chang, S. J.; Chang, F. C. Sequential distribution of copolyesters containing the phosphorus linking pendent groups characterized by H-1-NMR Polymer 1998, 39, 3233-3240
28. Chang, S.; Han, C. D. Effect of bulky pendent side groups on the structure of mesophase in a thermotropic main-chain liquid-crystalline polymer Macromolecules 1996, 29, 2103-2112
29. Frisch, M. J.; Trucks, G. W.; Schlegel, H. B.; Scuseria, G. E.; Robb, M. A.; Cheeseman, J. R., Jr.; Vreven, T.; Kudin, K. N.; Burant, J. C.; Millam, J. M.; Iyengar, S. S.; Tomasi, J.; Barone, V.; Mennucci, B.; Cossi, M.; Scalmani, G.; Rega, N.; Petersson, G. A.; Nakatsuji, H.; Hada, M.; Ehara, M.; Toyota, K.; Fukuda, R.; Hasegawa, J.; Ishida, M.; Nakajima, T.; Honda, Y.; Kitao, O.; Nakai, H.; Klene, M.; Li, X.; Knox, J. E.; Hratchian, H. P.; Cross, J. B.; Bakken, V.; Adamo, C.; Jaramillo, J.; Gomperts, R.; Stratmann, R. E.; Yazyev, O.; Austin, A. J.; Cammi, R.; Pomelli, C.; Ochterski, J. W.; Ayala, P. Y.; Morokuma, K.; Voth, G. A.; Salvador, P.; Dannenberg, J. J.; Zakrzewski, V. G.; Dapprich, S.; Daniels, A. D.; Strain, M. C.; Farkas, O.; Malick, D. K.; Rabuck, A. D.; Raghavachari, K.; Foresman, J. B.; Ortiz, J. V.; Cui, Q.; Baboul, A. G.; Clifford, S.; Cioslowski, J.; Stefanov, B. B.; Liu, G.; Liashenko, A.; Piskorz, P.; Komaromi, I.; Martin, R. L.; Fox, D. J.; Keith, T.; Al-Laham, M. A.; Peng, C. Y.; Nanayakkara, A.; Challacombe, M.; Gill, P. M. W.; Johnson, B.; Chen, W.; Wong, M. W.; Gonzalez, C.; Pople, J. A. Gaussian03, version 6.0. Gaussian, Inc.: Pittsburgh PA, 2003.
30. Poulindandurand, S.; Perez, S.; Revol, J. F.; Brisse, F. Crystal-structure of poly(trimethylene terephthalate) by X-ray and electron-diffraction Polymer 1979, 20, 419-426
31. Desborough, I. J.; Hall, I. H.; Neisser, J. Z. Structure of poly(trimethylene terephthalate) Polymer 1979, 20, 545-552
32. Yang, J.; Sidoti, G.; Liu, J.; Geil, P. H.; Li, C. Y.; Cheng, S. Z. D. Morphology and crystal structure of CTFMP and bulk polymerized poly(trimethylene terephthalate) Polymer 2001, 42, 7181-7195
33. Ho, R. M.; Ke, K. Z.; Chen, M. Crystal structure and banded spherulite of poly(trimethylene terephthalate) Macromolecules 2000, 33, 7529-7537
34. Chiang, C. L.; Ma, C. C. M.; Wang, F. Y.; Kuan, H. C. Thermo-oxidative degradation of novel epoxy containing silicon and phosphorous nanocomposites Eur. Polym. J. 2003, 39, 825-830
35. Ge, X. G.; Wang, C.; Hu, Z.; Xiang, X.; Wang, J. S.; Wang, D. Y.; Liu, C. P.; Wang, Y. Z. Phosphorus-containing telechelic polyester-based ionomer: Facile synthesis and antidripping effects J. Polym. Sci., Part A: Polym. Chem. 2008, 46, 2994-3006
36. Qu, M. H.; Wang, Y. Z.; Liu, Y.; Ge, X. G.; Wang, D. Y.; Wang, C. Flammability and thermal degradation behaviors of phosphorus-containing copolyester/BaSO4 nanocomposites J. Appl. Polym. Sci. 2006, 102, 564-570
37. Wang, D. Y.; Wang, Y. Z.; Wang, J. S.; Chen, D. Q.; Zhou, Q.; Yang, B.; Li, W. Y. Thermal oxidative degradation behaviours of flame-retardant copolyesters containing phosphorous linked pendent group/montmorillonite nanocomposites Polym. Degrad. Stab. 2005, 87, 171-176
38. Wang, D. Y.; Liu, X. Q.; Wang, J. S.; Wang, Y. Z.; Stec, A. A.; Hull, T. R. Preparation and characterisation of a novel fire retardant PET/alpha-zirconium phosphate nanocomposite Polym. Degrad. Stab. 2009, 94, 544-549
39. Davis, J. Characterisation for blends of phosphorus-containing copolyester with poly(ethylene terephthalate) J. Vinyl Addit. Technol. 1996, 2, 69-75
40. Morgan, A. B.; Bundy, M. Cone calorimeter analysis of UL-94 V-rated plastics Fire Mater. 2007, 31, 257-283
41. Price, D.; Liu, Y.; Hull, T. R.; Milnes, G. J.; Kandola, B. K.; Horrocks, A. R. Flame retardance of poly(methyl methacrylate) modified with phosphorus-containing compounds Polym. Degrad. Stab. 2002, 77, 227
42. Schartel, B.; Bartholmai, M.; Knoll, U. Some comments on the use of cone calorimeter data Polym. Degrad. Stab. 2005, 88, 540-547
43. Schartel, B.; Hull, T. R. Development of fire-retarded materials-Interpretation of cone calorimeter data Fire Mater. 2007, 31, 327-354