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Volumn 81, Issue 8, 2010, Pages

Critical sizes for the submersion of alkali clusters into liquid helium

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EID: 77954886234     PISSN: 10980121     EISSN: 1550235X     Source Type: Journal    
DOI: 10.1103/PhysRevB.81.085401     Document Type: Article
Times cited : (35)

References (38)
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    • note
    • For example, for the binding energies of alkali dimers to a H 4 e surface (the largest alkali particles for which detailed surface-adsorption calculations are available in the literature) this model yields values on the order of 4 K, which is within a factor of three of the results of a density-functional calculation (Ref.); and the accuracy should increase with cluster size: the particle shape becomes more three dimensional, befitting Eqs., and at the same time the influence of the surface dimple decreases relative to the particle size.
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    • note
    • The energy curves for Cs become so shallow that just a small variation in the parameters of the surface-binding picture in Sec. (e.g., reducing the surface width parameter to 4 Å) is sufficient to completely prevent the submersion energy from exceeding surface binding for any N. For the other alkalis, on the other hand, the N c values are relatively stable upon such variations.


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