Linking rigidity transitions with enthalpic changes at the glass transition and fragility: Insight from a simple oscillator model

Journal of Physics Condensed Matter

Volumn 22, Issue 28, 2010, Pages

  Micoulaut, Matthieu ^a  

^a UNIVERSITÉ PIERRE ET MARIE CURIE   (France)

Author keywords

[No Author keywords available]

Indexed keywords

ARRHENIUS; GLASS FORMATION; GLASS-FORMING LIQUID; HARMONIC INTERACTIONS; LOW TEMPERATURES; MONTE CARLO DYNAMICS; NETWORK GLASS; OSCILLATOR MODEL; OXIDE GLASS; PHILLIPS; RIGIDITY TRANSITION; THEORETICAL PREDICTION; THERMAL REVERSIBILITY;

ACTIVATION ENERGY; GLASS; GLASS FORMING MACHINES; IONIC LIQUIDS; IONIZATION OF LIQUIDS; OSCILLATORS (MECHANICAL); RIGIDITY;

GLASS TRANSITION;

GLASS;

ARTICLE; CHEMICAL MODEL; CHEMISTRY; COLD; COMPUTER SIMULATION; ENERGY TRANSFER; METHODOLOGY; OSCILLOMETRY; PHASE TRANSITION;

COLD TEMPERATURE; COMPUTER SIMULATION; ENERGY TRANSFER; GLASS; MODELS, CHEMICAL; OSCILLOMETRY; PHASE TRANSITION;

EID: 77953789218     PISSN: 09538984     EISSN: 1361648X     Source Type: Journal    
DOI: 10.1088/0953-8984/22/28/285101     Document Type: Article

References (43)

1. Angell C A 1995 Formation of glasses from liquids and biopolymers Science 267 1924
2. Gupta P K and Mauro J C 2009 Composition dependence of glass transition temperature and fragility. I. A topological model incorporating temperature-dependent constraints J. Chem. Phys. 130 094503
3. Trachenko K 2008 The Vogel-Fulcher-Tammann law in the elastic theory of glass transition J. Non-Cryst. Solids 354 3903
4. Sciortino F 2002 Disordered materials: one liquid, two glasses Nat. Mater. 1 145
5. Gupta P K and Mauro J C 2008 Two factors governing fragility: stretching exponent and configurational entropy Phys. Rev. E 78 062501
6. Wang L M, Angell C A and Richert R 2006 Fragility and thermodynamics in nonpolymeric glass-forming liquids J. Chem. Phys. 125 074505
7. Buchenau U and Wischnewski A 2004 Fragility and compressibility at the glass transition Phys. Rev. B 70 092201
8. Novikov V N and Sokolov A P 2004 Poisson's ratio and the fragility of glass-forming liquids Nature 431 961
9. Yannopoulos S N and Johari J P 2006 Poisson's ratio and liquid's fragility Nature 442 E7
10. Mauro J C and Loucks R J 2008 Impact of fragility on enthalpy relaxation in glass Phys. Rev. E 78 021502
11. Phillips J C 2006 Axiomatic theories of ideal stretched exponential relaxation (SER) J. Non-Cryst. Solids 352 4490
12. Naumis G G and Flores-Ruiz H M 2008 Low-frequency vibrational mode anomalies and glass transition: thermal stability, phonon scattering, and pressure effects Phys. Rev. B 78 094203
13. Phillips J C 1979 Topology of covalent non-crystalline solids 1. Short-range order in chalcogenide alloys J. Non-Cryst. Solids 34 153
14. Wyart M 2005 On the rigidity of amorphous solids Ann. Phys. Fr. 30 1
15. Lagrange J L 1788 Mécanique Analytique Paris
16. Maxwell J C 1864 Phil. Mag. 27 294
17. Thorpe M F 1983 Continuous deformations in random networks J. Non-Cryst. Solids 57 355
18. He H and Thorpe M F 1985 Elastic properties of glasses Phys. Rev. Lett. 54 2107
19. Wooten F, Winer K and Weaire D 1985 Computer-generation of structural models of amorphous Si and Ge Phys. Rev. Lett. 54 1392
20. Djordjević B R, Thorpe M F and Wooten F 1995 Computer-model of tetrahedral amorphous diamond Phys. Rev. B 52 5685
21. Naumis G G 2006 Variation of the glass transition temperature with rigidity and chemical composition Phys. Rev. B 73 172202
22. Naumis G G 2005 Energy landscape and rigidity Phys. Rev. E 71 026114
23. Kamitakahara W et al. 1991 Vibrational densities of states andnetwork rigidity in chalcogenide glasses Phys. Rev. B 44 94
24. Bonilla L L, Padilla F G and Ritort F 1998 Aging in the linear harmonic oscillator Physica A 250 315
25. Ritort F 2005 Resonant nonequilibrium temperatures J. Phys. Chem. B 109 6787
26. Wang R W, Thorpe M F and Mousseau N 1995 Length mismatch in random semiconductor alloys. 4. General multinary compounds Phys. Rev. B 52 17191
27. Garriga A and Ritort F 2005 Mode-dependent nonequilibrium temperature in aging systems Phys. Rev. E 72 031505
28. Feng W, Bresser W and Boolchand P 1997 Direct evidence for stiffness threshold in chalcogenide glasses Phys. Rev. Lett. 78 4422
29. 1 - x glasses from Raman scattering and temperature-modulated differential scanning calorimetry Phys. Rev. B 61 15061
30. Wang F, Mamedov S, Boolchand P, Goodman B and Chandrasekhar M 2005 Pressure Raman effects and internal stress in network glasses Phys. Rev. B 71 174201
31. 2-Se liquids Phys. Chem. Chem. Phys. 4 3396
32. Borisova Z U 1981 Glassy Semiconductors (New York: Plenum)
33. 1 - x glasses Phys. Rev. B 62 9228
34. Wang Y, Boolchand P and Micoulaut M 2000 Glass structure, rigidity transitions and the intermediate phase in the Ge-As-Se ternary Europhys. Lett. 52 633
35. Tatsumisago M, Halfpap B L, Green J L, Lindsay S M and Angell C A 1990 Fragility of Ge-As-Se glass-forming liquids in relation to rigidity percolation, and the Kauzmann paradox Phys. Rev. Lett. 64 1549
36. Böhmer R and Angell C A 1992 Correlations of the nonexponentiality and state dependence of mechanical relaxations with bond connectivity in Ge-As-Se supercooled liquids Phys. Rev. B 45 10091
37. Bockris J O M, Mackenzie J D and Kitchener J A 1955 Viscous flow in silica and binary liquid silicates Trans. Faraday Soc. 51 1734
38. Vaills Y, Qu T, Micoulaut M, Chaimbault F and Boolchand P 2005 Direct evidence of rigidity loss and self-organization in silicate glasses J. Phys.: Condens. Matter 17 4889
39. Galeener F L and Thorpe M F 1983 Rings in central-force network dynamics Phys. Rev. B 28 5802
40. Trachenko V and Brazhkin V V 2009 Understanding the problem of glass transition on the basis of elastic waves in a liquid J. Phys.: Condens. Matter 21 425104
41. Phillips J C 2006 Ideally glassy hydrogen-bonded networks Phys. Rev. B 73 024210
42. Boolchand P, Micoulaut M and Chen P 2008 Nature of glasses Phase Change Materials: Science and Applications ed S Raoux and M Wuttig (Heidelberg: Springer) p37
43. DeGusseme A, Carpentier L, Willart J F and Descamps M 2003 Molecular mobility in supercooled trehalose J. Phys. Chem. B 107 10879