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An example would be the optical excitation electrons at a surface, inducing nuclear motion of an adsorbate atom, leading to shifting electronic energy levels and changing wave function overlap, causing changes in the dipole moments and electronic transition rates, and finally feeding back onto the induced nuclear motion in the next time step (Ref.). Inclusion of such processes would introduce additional nonlinear character into the system of Eq.
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An example would be the optical excitation electrons at a surface, inducing nuclear motion of an adsorbate atom, leading to shifting electronic energy levels and changing wave function overlap, causing changes in the dipole moments and electronic transition rates, and finally feeding back onto the induced nuclear motion in the next time step (Ref.). Inclusion of such processes would introduce additional nonlinear character into the system of Eq..
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