Isotropic and anisotropic collision-induced Raman scattering by monoatomic gas mixtures: Ne-Ar

Physical Review A - Atomic, Molecular, and Optical Physics

Volumn 80, Issue 2, 2009, Pages

  Dixneuf, S ^a,b   Chrysos, M ^a   Rachet, F ^a  

^a UNIVERSITÉ D'ANGERS   (France)

^b UNIVERSITY COLLEGE CORK   (Ireland)

Author keywords

[No Author keywords available]

Indexed keywords

AB INITIO; ATMOSPHERIC ENVIRONMENT; DENSITY FUNCTIONAL THEORY METHODS; DEPOLARIZATION RATIO; FREQUENCY SHIFT; INCOMPLETE KNOWLEDGE; POLARIZABILITIES; RAMAN SCATTERING SPECTRA; RARE GAS ATOMS; ROOM-TEMPERATURE MIXTURES; SCATTERING INTENSITY; SECOND VIRIAL COEFFICIENTS;

ANISOTROPY; ATOMIC SPECTROSCOPY; DENSITY FUNCTIONAL THEORY; EQUATIONS OF STATE; GAS MIXTURES; INERT GASES; RAMAN SCATTERING; SCATTERING;

NEON;

EID: 68949157393     PISSN: 10502947     EISSN: 10941622     Source Type: Journal    
DOI: 10.1103/PhysRevA.80.022703     Document Type: Article

References (48)

1. Z. J. Kiss and H. L. Welsh, Phys. Rev. Lett. 2, 166 (1959). 10.1103/PhysRevLett.2.166
2. D. R. Bosomworth and H. P. Gush, Can. J. Phys. 43, 729 (1965).
3. L. Frommhold, Collision-induced Absorption in Gases (Cambridge University Press, Cambridge, 1993).
4. J. P. C. McTague and G. Birnbaum, Phys. Rev. Lett. 21, 661 (1968). 10.1103/PhysRevLett.21.661
5. J. P. C. McTague and G. Birnbaum, Phys. Rev. A 3, 1376 (1971). 10.1103/PhysRevA.3.1376
6. M. H. Proffitt and L. Frommhold, Phys. Rev. Lett. 42, 1473 (1979). 10.1103/PhysRevLett.42.1473
7. M. H. Proffitt and L. Frommhold, J. Chem. Phys. 72, 1377 (1980). 10.1063/1.439202
8. L. Frommhold and M. H. Proffitt, Phys. Rev. A 21, 1249 (1980). 10.1103/PhysRevA.21.1249
9. F. Rachet, M. Chrysos, C. Guillot-Noël, and Y. Le Duff, Phys. Rev. Lett. 84, 2120 (2000). 10.1103/PhysRevLett.84.2120
10. C. Guillot-Noël, M. Chrysos, Y. Le Duff, and F. Rachet, J. Phys. B 33, 569 (2000). 10.1088/0953-4075/33/3/323
11. F. Rachet, Y. Le Duff, C. Guillot-Noël, and M. Chrysos, Phys. Rev. A 61, 062501 (2000). 10.1103/PhysRevA.61.062501
12. F. Rachet, M. Chrysos, G. Lothon, R. Moszynski, and A. Milet, J. Raman Spectrosc. 34, 972 (2003). 10.1002/jrs.1101
13. S. Dixneuf, F. Rachet, and M. Chrysos (unpublished).
14. F. Rachet, S. Dixneuf, and M. Chrysos (unpublished).
15. F. Chapeau-Blondeau, V. Teboul, J. Berrué, and Y. Le Duff, Phys. Lett. A 173, 153 (1993). 10.1016/0375-9601(93)90179-4
16. O. Gaye, M. Chrysos, V. Teboul, and Y. Le Duff, Phys. Rev. A 55, 3484 (1997). 10.1103/PhysRevA.55.3484
17. M. Chrysos, O. Gaye, and Y. Le Duff, J. Phys. B 29, 583 (1996). 10.1088/0953-4075/29/3/022
18. M. Chrysos, O. Gaye, and Y. Le Duff, J. Chem. Phys. 105, 31 (1996). 10.1063/1.472813
19. T. Müller, Computational Nanoscience: Do It Yourself!, edited by, J. Grotendorst, S. Blügel, and, D. Marx, NIC series (John von Neumann Institute for Computing, Julich, 2006), vol. 31, p. 19.
20. T. H. Dunning, Jr., J. Chem. Phys. 90, 1007 (1989). 10.1063/1.456153
21. T. H. Dunning, Jr., K. A. Peterson, and A. K. Wilson, J. Chem. Phys. 114, 9244 (2001). 10.1063/1.1367373
22. C. Hättig, H. Larsen, J. Olsen, P. Jørgensen, H. Koch, B. Fernández, and A. Rizzo, J. Chem. Phys. 111, 10099 (1999). 10.1063/1.480361
23. C. Hättig, J. L. Cacheiro, B. Fernández, and A. Rizzo, Mol. Phys. 101, 1983 (2003). 10.1080/0026897031000109374
24. B. Fernández, C. Hättig, H. Koch, and A. Rizzo, J. Chem. Phys. 110, 2872 (1999). 10.1063/1.477930
25. J. L. Cacheiro, B. Fernández, D. Marchesan, S. Coriani, C. Hättig, and A. Rizzo, Mol. Phys. 102, 101 (2004). 10.1080/ 00268970410001668606
26. G. Maroulis and A. Haskopoulos, Chem. Phys. Lett. 358, 64 (2002). 10.1016/S0009-2614(02)00588-2
27. A. Rizzo, S. Coriani, D. Marchesan, J. L. Cacheiro, B. Fernández, and C. Hättig, Mol. Phys. 104, 305 (2006). 10.1080/00268970500282133
28. By using the notations of Ref.
29. G. Herzberg, Molecular Spectra and Molecular Structure, Part I: Spectra of Diatomic Molecules, 2nd ed. (D Van Nostrand, Princeton, 1950).
30. K. Fox and I. Ozier, J. Chem. Phys. 52, 5044 (1970). 10.1063/1.1672742
31. S.-I. Tomonaga, The Story of Spin (University of Chicago Press, Chicago, 1998).
32. A. Barrow and R. A. Aziz, J. Chem. Phys. 89, 6189 (1988). 10.1063/1.455435
33. R. A. Aziz and M. J. Slaman, Chem. Phys. 130, 187 (1989). 10.1016/0301-0104(89)87048-X
34. R. A. Aziz and M. J. Slaman, J. Chem. Phys. 92, 1030 (1990). 10.1063/1.458165
35. G. Maroulis, J. Phys. Chem. A 104, 4772 (2000). 10.1021/jp9941615
36. L. Frommhold, Adv. Chem. Phys. 46, 1 (1981). 10.1002/9780470142653.ch1
37. These values were estimated by plotting, as a function of r, the quantities Fn (β) and Gn (α), which are implied in the calculation of the nth -order anisotropic and isotropic moments [38,39]. We thus observed that Fn and Gn, n=0,2,4,6, get a zero value below 4, 4.5, and 5 bohr for (Ne) 2, Ne-Ar, and (Ar) 2, respectively. As moments are not seen to be affected by separations below those bounds, spectra are not expected to be affected either.
38. U. Bafile, R. Magli, F. Barocchi, M. Zoppi, and L. Frommhold, Mol. Phys. 49, 1149 (1983). 10.1080/00268978300101831
39. C. G. Joslin, J. D. Goddard, and S. Goldman, Mol. Phys. 89, 791 (1996). 10.1080/002689796173697
40. In practice, this combination was slightly corrected in order to account for the aperture of the scattering angle [41].
41. M. H. Proffitt, J. W. Keto, and L. Frommhold, Can. J. Phys. 59, 1459 (1981).
42. Since signals by pairs of unlike atoms scale with density as ρa ρb whereas signals by pairs of like atoms scale as ρa2 /2!, the factor 14/45 in Eq. (4) of Ref. should be halved.
43. J. H. Dymond and E. B. Smith, The Virial Coefficients of Pure Gases and Mixtures: A Critical Compilation, Published by Oxford University Press (Watton Street, Oxford, 1980).
44. A. Michels, T. Wassenaar, and P. Louwerse, Physica Grav. 26, 539 (1960).
45. A. Michels, H. Wijker, and H. K. Wijker, Physica Grav. 15, 627 (1949).
46. H. Schmiedel, R. Gehrmann, and B. Schramm, Ber. Bunsenges. Phys. Chem 84, 721 (1980).
47. J. Brewer and G. W. Vaughn, J. Chem. Phys. 50, 2960 (1969). 10.1063/1.1671491
48. To that purpose, use was made of the formula BK (0), α2 =2π N2 M0 / (405 kB T) (CGS), which describes the major contribution to the static Kerr second virial coefficient component [27]; N is Avogadro's number.