Preparation, characterization, and performance of HMS-supported Ni catalysts for hydrodechlorination of chorobenzene

Industrial and Engineering Chemistry Research

Volumn 48, Issue 8, 2009, Pages 3802-3811

  Chen, Jixiang ^a   Zhou, Jianjun ^a   Wang, Rijie ^a   Zhang, Jiyan ^a  

^a TIANJIN UNIVERSITY   (China)

Author keywords

[No Author keywords available]

Indexed keywords

ATOMIC ABSORPTION SPECTROSCOPIES; BET SURFACE AREAS; CATALYST STRUCTURES; CHLOROBENZENE CONVERSIONS; DIRECT SYNTHESIS; DIRECT SYNTHESIS METHODS; FIXED-BED REACTORS; HYDRODECHLORINATION; HYDROGEN CHEMISORPTIONS; IMPREGNATION METHODS; INTRAPARTICLE; MASS TRANSFER LIMITATIONS; MATRIXES; MESO STRUCTURES; NI CATALYSTS; NI CONTENTS; NI2+ IONS; NICKEL PARTICLES; NICKEL SILICATES; PH VALUES; PHYSICO-CHEMICAL PROPERTIES; PORE VOLUMES; REDUCTION TEMPERATURES; STRONG INTERACTIONS; TEMPERATURE-PROGRAMMED DESORPTIONS; TEMPERATURE-PROGRAMMED REDUCTIONS; TRANSMISSION ELECTRON MICROSCOPES; WIDE-ANGLE X-RAY DIFFRACTIONS;

ABSORPTION SPECTROSCOPY; ATMOSPHERIC PRESSURE; ATOMIC SPECTROSCOPY; CATALYSIS; CATALYST ACTIVITY; CATALYST SUPPORTS; CHEMISORPTION; GAS ADSORPTION; HYDROGEN; IMPREGNATION; NICKEL ALLOYS; PH EFFECTS; SILICATES; TEMPERATURE PROGRAMMED DESORPTION; TRANSMISSION ELECTRON MICROSCOPY;

NICKEL;

EID: 65249141148     PISSN: 08885885     EISSN: None     Source Type: Journal    
DOI: 10.1021/ie801792h     Document Type: Article

References (60)

1. Tanev, P. T.; Pinnavaia, T. J. A neutral templating route to mesoporous molecular sieves. Science 1995, 267, 865-867.
2. Tanev, P. T.; Chibwe, M.; Pinnavaia, T. J. Titanium-containing mesoporous molecular sieves for catalytic oxidation of aromatic compounds. Nature 1994, 368, 321-323.
3. Pauly, T. R.; Liu, Y.; Pinnavaia, T. J.; Billinge, S. J. L.; Rieker, T. P. Textural mesoporosity and the catalytic activity of mesoporous molecular sieves with wormhole framework structures. J. Am. Chem. Soc. 1999, 121, 8835-8842.
4. Zhang, W.; Froba, M.; Wang, J.; Tanev, P. T.; Wong, J.; Pinnavaia, T. J. Mesoporous titanosilicate molecular sieves prepared at ambient temperature by electrostatic (S+I-, S+X-I+) and neutral (S0I0) assembly pathwayssA comparison of physical properties and catalytic activity for peroxide oxidations. J. Am. Chem. Soc. 1996, 118, 9164-9171.
5. Jin, C. Z.; Li, G.; Wang, X. S.; Zhao, L. X.; Liu, L. P.; Liu, H. Synthesis, characterization and catalytic performance of ti-containing mesoporous molecular sieves assembled from titanosilicate precursors. Chem. Mater. 2007, 19, 1664-1670.
6. Liu, Y. Y.; Murata, K.; Inaba, M.; Mimura, N. Syntheses of Ti- and Al-containing hexagonal mesoporous silicas for gas-phase epoxidation of propylene by molecular oxygen. Appl. Catal., A 2006, 309, 91-105.
7. Bhoware, S. S.; Shylesh, S.; Kamble, K. R.; Singh, A. P. Cobaltcontaining hexagonal mesoporous molecular sieves (Co-HMS): Synthesis, characterization and catalytic activityin the oxidation reaction of ethylbenzene. J. Mol Catal. A: Chem. 2006, 255, 123-130.
8. Lira, E.; López, C. M.; Oropeza, F.; Bartolini, M.; Alvarez, J.; Goldwasser, M.; Linares, F. L.; Lamonier, J. -F.; Zurita, M. J. P. HMS mesoporous silica as cobalt support for the Fischer-Tropsch Synthesis: Pretreatment, cobalt loading and particle size effects. J. Mol. Catal. A: Chem. 2008, 281, 146-153.
9. Shiraishi, Y.; Morishita, M.; Teshima, Y.; Hirai, T. Vanadiumcontaining mesoporous silica of high photocatalytic activity and stability even in water. J. Phys. Chem. B 2006, 110, 6587-6594.
10. Ke, I.-S.; Liu, S.-T. Synthesis and catalysis of tungsten oxide in hexagonal mesoporous silicas (W-HMS). Appl. Catal., A 2007, 317, 91- 96.
11. Zepeda, T. A.; Pawelec, B.; Fierro, J. L. G.; Halachev, T. Removal of refractory S-containing compounds from liquid fuels on novel bifunctional CoMo/HMS catalysts modified with Ti. Appl. Catal., B 2007, 223-236.
12. Nava, R.; Morales, J.; Alonso, G.; Ornelas, C.; Pawelec, B.; Fierro, J. L. G. Influence of the preparation method on the activity of phosphatecontaining CoMo/HMS catalysts in deep hydrodesulphurization. Appl. Catal., A 2007, 321, 58-70.
13. Onaka, M.; Hashimoto, N.; Kitabata, Y.; Yamasaki, R. Aluminumrich mesoporous aluminosilicate (Al-HMS) as a solid acid catalyst for the Diels-Alder reaction of acrylates with 1,3-dienes. Appl. Catal., A 2003, 241, 307-317.
14. Wang, W.; Song, M. Preparation of high nickel-containing MCM- 41-type mesoporous silica via a modified direct synthesis method. Mater. Res. Bull. 2005, 40, 1737-1744.
15. Wang, W.; Song, M.; Zhang, Z. Y.; Richardson, M. Synthesis and characterization of high nickel-containing mesoporous silica via a modified direct synthesis method. J. Non-Cryst. Solids 2006, 352, 2180-2186.
16. Yang, Y. H.; Lim, S.; Du, G.; Chen, Y.; Ciuparu, D.; Haller, G. L. Synthesis and Characterization of Highly Ordered Ni-MCM-41 Mesoporous Molecular Sieves. J. Phys. Chem. B 2005, 109, 13237-13246.
17. Lewandowska, A.; Monteverdi, S.; Bettahar, M.; Ziolek, M. MCM- 41 mesoporous molecular sieves supported nickelsphysico-chemical properties and catalytic activity in hydrogenation of benzene. J. Mol. Catal. A: Chem. 2002, 188, 85-95.
18. Wojcieszak, R.; Monteverdi, S.; Mercy, M.; Nowak, I.; Ziolek, M.; Bettahar, M. M. Nickel containing MCM-41 and AlMCM-41 mesoporous molecular sieves characteristics and activity in the hydrogenation of benzene. Appl. Catal., A 2004, 268, 241-253.
19. Cesteros, Y.; Salagre, P.; Medina, F.; Sueiras, J. E. Use of Ni/Al- MCM-41 catalysts for exhaustive hydrodechlorination of 1,2,4-trichlorobenzene. Catal. Lett. 2002, 79, 83-88.
20. Parvulescu, V.; Dascalescu, C.; Su, B. L. Highly selective oxidation of styrene with hydrogen peroxide catalyzed by mono- and bimetallic (Ni, Ni-Cr and Ni-Ru) incorporated MCM-41 silicas. Stud. Surf. Sci. Catal. 2003, 146, 629-632.
21. Park, Y.; Kang, T.; Lee, J.; Kim, P.; Kim, H.; Yi, J. Single-step preparation of Ni catalysts supported on mesoporous silicas (SBA-15 and SBA-16) and the effect of pore structure on the selective hydrodechlorination of 1,1,2-trichloroethane to VCM. Catal. Today 2004, 97, 195-203.
22. Kang, T.; Park, Y.; Yi, J. Facile synthesis and characterization of ordered mesostructured nickel catalysts. J. Mol. Catal. A: Chem. 2006, 244, 151-159.
23. Cho, Y. S.; Park, J. C.; Lee, B.; Kim, Y.; Yi, J. Preparation of mesoporus catalyst supported on silica with finely dispersed Ni particles. Catal. Lett. 2002, 81, 89-96.
24. Park, J. G.; Ko, C. H.; Yi, K. B.; Park, J.-H.; Han, S. S.; Cho, S. H.; Kim, J. N. Reactive adsorption of sulfur compounds in diesel on nickel supported on mesoporous silica. Appl. Catal., B 2008, 81, 244-250.
25. Li, H. Y.; Sun, Y.; Yue, Y. H.; Gao, Z. Dehydrogenation and hydrodesulfurization activity of heteroatom-containing HMS mesoporous molecular sieve catalysts. Chin. J. Catal. 1999, 20, 455-458.
26. Keane, M. A. Advances in greener separation processes-case study: Recovery of chlorinated aromatic compounds. Green Chem. 2003, 5, 309.
27. Kim, P.; Joo, J. B.; Kim, H.; Kim, W.; Kim, Y.; Song, I. K.; Yi, J. Preparation of mesoporous Ni-alumina catalyst by one-step sol-gel method: control of textural properties and catalytic application to the hydrodechlorination of o-dichlorobenzene. Catal. Lett. 2005, 104, 181- 189.
28. Cesteros, Y.; Salagrea, P.; Medina, F.; Sueiras, J. E.; Tichi, D.; Coq, B. Hydrodechlorination of 1,2,4-trichlorobenzene on nickel-based catalysts prepared from several Ni/Mg/Al hydrotalcite-like precursor. Appl. Catal., B 2001, 32, 25-35.
29. Keane, M. A.; Pina, G.; Tavoularis, G. The catalytic hydrodechlorination of mono-, di- and trichlorobenzenes over supported nickel. Appl. Catal., B 2004, 48, 275-286.
30. Kang, T.; Park, Y.; Yi, J. Facile synthesis and characterization of ordered mesostructured nickel catalysts. J. Mol. Catal. A: Chem. 2006, 244, 151-159.
31. Pauly, T. R.; Pinnavaia, T. J. Pore size modification of mesoporous HMS molecular sieve silicas with wormhole framework structures. Chem. Mater. 2001, 13, 987-993.
32. Sing, K. S. W.; Everett, D. H.; Haul, R. A. W.; Moscow, L.; Pierotti, R. A.; Rouquerol, J.; Siemieniewska, T. Reporting physisorption data for gas/solid systems with special reference to the determination of surface area and porosity (Recommendations 1984). Pure Appl. Chem. 1985, 57, 603-619.
33. Tanev, P. T.; Pinnavaia, T. J. Mesoporous silica molecular sieves prepared by ionic and neutral surfactant templating: A comparison of physical properties. Chem. Mater. 1996, 8, 2068-2079.
34. Zepeda, T. A.; Fierro, J. L. G.; Pawelec, B.; Nava, R.; Klimova, T.; Fuentes, G. A.; Halachev, T. Synthesis and characterization of Ti-HMS and CoMo/Ti-HMS oxide materials with varying Ti Content. Chem. Mater. 2005, 17, 4062-4073.
35. Liu, H.; Lu, G. Z.; Guo, Y. L.; Guo, Y.; Wang, J. S. Study on the synthesis and the catalytic properties of Fe-HMS materials in the hydroxylation of phenol. Microporous Mesoporous Mater. 2008, 108, 56-64.
36. Chiranjeevi, T.; Kumaran, G. M.; Gupta, J. K.; Dhar, G. M. Synthesis and characterization of acidic properties of Al-HMS materials of varying Si/Al ratios. Thermochim. Acta 2006, 443, 87-92.
37. Lin, H. Y.; Chen, Y. W. Preparation of spherical hexagonal mesoporus silica. J. Porous Mater. 2005, 12, 95-105.
38. Mile, B.; Stirling, D.; Zammitt, M.; Lovell, A.; Webb, M. The location of nickel oxide and nickel in silica-supported catalysts: Two forms of "NiO" and the assignment of temperature-programmed reduction profiles. J. Catal. 1988, 114, 217-229.
39. Castaño, P.; Pawelec, B.; Fierro, J. L. G.; Arandes, J. M.; Bilbao, J. Aromatics reduction of pyrolysis gasoline (PyGas) over HY-supported transition metal catalysts. Appl. Catal., A 2006, 315, 101-113.
40. Castaño, P.; Pawelec, B.; Fierro, J. L. G.; Arandes, J. M.; Bilbao, J. Enhancement of pyrolysis gasoline hydrogenation over Pd-promoted Ni/ SiO2-Al2O3 catalysts. Fuel 2007, 86, 2262-2274.
41. Paál, Z.; Menon, P. G. Hydrogen effects in metal catalysts. Catal. Rev. Sci. Eng. 1983, 25, 229-324.
42. Conner, W. C.; Falconer, J. L. Spillover in heterogeneous catalysis. Chem. Rev. 1995, 95, 759-788.
43. Keane, M. A.; Murzin, D. Yu. A kinetic treatment of the gas phase hydrodechlorination of chlorobenzene over nickel/silica: beyond conventional kinetics. Chem. Eng. Sci. 2001, 56, 3185-3195.
44. Keane, M. A.; Tavoularis, G. The role of spillover hydrogen in gas phase catalytic aromatic hydrodechlorination and hydrogenation over nickel/silica. React. Kinet. Catal. Lett. 2003, 78, 11-18.
45. Shin, E.-J.; Spiller, A.; Tavoularisa, G.; Keane, M. A. Chlorinenickel interactions in gas phase catalytic hydrodechlorination: catalyst deactivation and the nature of reactive hydrogen. Phys. Chem. Chem. Phys. 1999, 1, 3173-3181.
46. Stakheev, A.; Yu.; Kustov, L. M. Effects of the support on the morphology and electronic properties of supported metal clusters-modern concepts and progress in 1990s. Appl. Catal., A 1999, 188, 3-351.
47. Bond, G. C. The origins of particle size effects in heterogeneous catalysis. Surf. Sci. 1985, 156, 966-981.
48. Bond, G. C. Supported metal catalysts: Some unsolved problems. Chem. Soc. Rev. 1991, 20, 441-475.
49. Che, M.; Bennett, C. O. The influence of particle size on the catalytic properties of supported metals. Adv. Catal. 1989, 36, 55-172.
50. Bodnariuk, P.; Coq, B.; Ferrat, G.; Figueras, F. Carbon-chlorine hydrogenolysis over PdRh and PdSn bimetallic catalysts. J. Catal. 1989, 116, 459-466.
51. Coq, B.; Ferrat, G.; Figueras, F. Conversion of chlorobenzene over palladium and rhodium catalysts of widely varying dispersion. J. Catal. 1986, 101, 434-445.
52. Estellé, J.; Ruz, J.; Cesteros, Y.; Fernandez, R.; Salagre, P.; Medina, F.; Sueiras, J.-E. Surface structure of bulk nickel catalysts, active in the gas-phase hydrodechlorination reaction of aromatics. J. Chem. Soc., Faraday Trans. 1996, 92, 2811-2816.
53. Murthy, K. V.; Patterson, P. M.; Jacobs, G.; Davis, B. H.; Keane, M. A. An exploration of activity loss during hydrodechlorination and hydrodebromination over Ni/SiO2. J. Catal. 2004, 223, 74-85.
54. Chen, J. X.; Ci, D. H.; Wang, R. J.; Zhang, J. Y. Hydrodechlorination of chlorobenzene over NiB/SiO2, NiP/SiO2 amorphous catalysts after being partially crystallized: Effect of electronic and geometrical factors. Appl. Surf. Sci. 2008, 255, 3300-3309.
55. Liu, X. G.; Chen, J. X.; Zhang, J. Y. Hydrodechlorination of chlorobenzene over silica-supported nickel phosphide catalysts. Ind. Eng. Chem. Res. 2008, 47, 5362-5368.
56. Gopinath, R.; Lingaiah, N.; Babu, N. S.; Suryanarayana, I.; Sai Prasad, P. S.; Obuchi, A. A highly active low Pd content catalyst synthesized by deposition-precipitation method for hydrodechlorination of chlorobenzene. J. Mol. Catal. A: Chem. 2004, 223, 289-293.
57. Ozali, A.; Kimura, K. The effective site on acid catalysts revealed in n-butane isomerization. J. Catal. 1964, 3, 395-405.
58. Kimura, K.; A-I H.; Ozaki, A. Tracer study of ethylene dimerization over nickel oxide-silica catalyst. J. Catal. 1970, 18, 271-280.
59. Sohn, J. R.; Ozaki, A. Acidity of nickel silicate and its bearing on the catalytic activity for ethylene dimerization and butene isomerization. J. Catal. 1980, 61, 29-38.
60. Hashimoto, Y.; Uemichi, Y.; Ayame, A. Low-temperature hydrodechlorination mechanism of chlorobenzenes over platinum-supported and palladium-supported alumina catalysts. Appl. Catal., A 2005, 287, 89-97.