Desulfurization from thiophene by SO42-/ZrO2 catalytic oxidation at room temperature and atmospheric pressure

Journal of Hazardous Materials

Volumn 164, Issue 1, 2009, Pages 256-264

  Wang, Bo ^a   Zhu, Jianpeng ^a   Ma, Hongzhu ^a  

^a SHAANXI NORMAL UNIVERSITY   (China)

Author keywords

Desulfurization; Ozone; SO42 ZrO2; Sulfur compounds; Thiophene

Indexed keywords

CATALYST SURFACES; CATALYST SYSTEMS; COMBUSTION PRODUCTS; FOURIER TRANSFORMATIONS; GAS CHROMATOGRAPHY-MASS SPECTROMETRIES; H SYSTEMS; HIGH CONCENTRATIONS; LONG-CHAIN HYDROCARBONS; NOVEL METHODS; OXIDATIVE DESULFURIZATIONS; ROOM TEMPERATURES; SCANNING ELECTRON MICROSCOPES; SO42-/ZRO2; TOTAL EFFICIENCIES; X-RAY DIFFRACTIONS; X-RAY PHOTOELECTRON SPECTROSCOPIES;

AIR QUALITY; ATMOSPHERIC PRESSURE; CATALYSIS; CATALYSTS; CATALYTIC OXIDATION; CHROMATOGRAPHIC ANALYSIS; DESULFURIZATION; FOURIER ANALYSIS; FOURIER TRANSFORMS; GAS CHROMATOGRAPHY; HIGH PERFORMANCE LIQUID CHROMATOGRAPHY; HYDROCARBONS; INFRARED SPECTROSCOPY; MASS SPECTROMETRY; ORGANIC POLYMERS; OZONE; SCANNING ELECTRON MICROSCOPY; SPECTROSCOPIC ANALYSIS; SPECTRUM ANALYSIS; SULFUR; SULFUR DETERMINATION; THIOPHENE; ZIRCONIUM ALLOYS;

X RAY PHOTOELECTRON SPECTROSCOPY;

ATMOSPHERIC PRESSURE; CATALYSIS; OXIDATION; SULFATE; SULFUR; TEMPERATURE GRADIENT; ZIRCON;

ATMOSPHERIC PRESSURE; CATALYSIS; MICROSCOPY, ELECTRON, SCANNING; OXIDATION-REDUCTION; OZONE; SPECTROSCOPY, FOURIER TRANSFORM INFRARED; SULFATES; TEMPERATURE; THIOPHENES; ZIRCONIUM;

EID: 61749091271     PISSN: 03043894     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.jhazmat.2008.08.003     Document Type: Article

References (33)

1. Li F.F., Song L.J., Duan L.H., Li X.Q., and Sun Z.L. A frequency response study of thiophene adsorption in zeolite catalysts. Appl. Surf. Sci. 253 (2007) 8802-8809
2. Stern A.C., Boubel R.W., Turner D.B., and Fox D.L. Fundamentals of Air Pollution. 2nd ed. (1984), Academic Press, New York
3. 3 model sulfide catalysts for hydrodesulfurization and their application to the study of the effects of catalyst preparation. J. Catal. 217 (2003) 12-22
4. Ma X.L., Sakanishi K., and Mochida I. Hydrodesulfurization reactivities of various sulfur compounds in diesel fuel. Ind. Eng. Chem. Res. 33 (1994) 218-222
5. Kanda Y., Aizawa T., Kobayashi T., Uemichi Y., Namba S., and Sugioka M. Preparation of highly active AlSBA-15-supported platinum catalyst for thiophene hydrodesulfurization. Appl. Catal. B 77 (2007) 117-124
6. Yang R.T. Adsorbents: Fundamentals and Applications (2003), Wiley, New York Chapter 10
7. Hernández-Maldonado A.J., and Yang R.T. Desulfurization of liquid fuels by adsorption via {eth}-complexation with Cu(I)-Y and Ag-Y zeolites. Ind. Eng. Chem. Res. 42 (2003) 123-129
8. Takahashi A., Yang F.H., and Yang R.T. New sorbents for desulfurization by {eth}-complexation: thiophene/benzene adsorption. Ind. Eng. Chem. Res. 41 (2002) 2487-2496
9. Huang C.P., Chen B.H., Zhang J., Liu Z.C., and Li Y.X. Desulfurization of gasoline by extraction with new ionic liquids. Energ. Fuel 18 (2004) 1862-1864
10. Kumagai A., Fukumoto H., and Yamamoto T. Chemical and electrochemical oxidation of thiophene-pyridine thiophene-pyrimidine Co-Oligomers in solutions. J. Phys. Chem. B 111 (2007) 8020-8026
11. Song C. An overview of new approaches to deep desulfurization for ultra-clean gasoline, diesel fuel and jet fuel. Catal. Today 86 (2003) 211-263
12. Zhao D.H., Sun F.X., Zhou E.P., and Liu Y. A review of desulfurization of light oil based on selective oxidation. Chem. J. Internet 6 (2004) 17
13. Nehlsen J., Benziger J., and Kevrekidis I. Oxidation of aliphatic and aromatic sulfides using sulfuric acid. Ind. Eng. Chem. Res. 45 (2006) 518-524
14. 8. J. Am. Chem. Soc. 95 (1973) 5173-5178
15. Reddy B.M., Sreekanth P.M., and Reddy V.R. Modified zirconia solid acid catalysts for organic synthesis and transformations. J. Mol. Catal. 225 (2005) 71-78
16. 2 catalysts under mild conditions. J. Hazard. Mater. 147 (2007) 800-805
17. 2) as a reusable solid acid catalyst for the Mannich-type reaction between ketene silylacetals and Aldimines. Tetrahedron Lett. 48 (2007) 6449-6452
18. 2 solid catalysts on the products of transformation and reaction mechanism of R-(+)-limonene diepoxides. J. Mol. Catal. A: Chem. 269 (2007) 72-80
19. Satuf M.L., Brandi R.J., Cassano A.E., and Alfano O.M. Scaling-up of slurry reactors for the photocatalytic degradation of 4-chlorophenol. Catal. Today 129 (2007) 110-117
20. 2 in the air. Energ. Fuel 21 (2007) 1859-1862
21. Teo S.H., and Zeng H.C. Surface and textural properties of network-modified silica as a function of transition metal dopant Zirconium. J. Phys. Chem. B 105 (2001) 9093-9100
22. 2: effects of sulfation in the cyclohexene isomerization reaction. J. Catal. 161 (1996) 605-613
23. Ishida T., and Choi N. High-resolution X-ray photoelectron spectra of organosulfur monolayers on Au(111): S(2p) spectral dependence on molecular species. Langmuir 15 (1999) 6799-6806
24. Wagner C.D., and Taylor J.A. Generation of XPS auger lines by bremsstrahlung. J. Electron Spectrosc. Relat. Phenom. 20 (1980) 83-93
25. Paal Z., Xu X.L., Paal-Lukacs J., Vogel W., Muhler M., and Schlogl R. Pt-Black catalysts sintered at different temperatures: surface analysis and activity in reactions of n-hexane. J. Catal. 152 (1995) 252-263
26. 2 with Ce and modifying with sulfate and its catalytic activity for acid catalysis. Catal. Today 116 (2006) 143-150
27. Morterra C., Meligrana G., Cerrato G., Solinas V., Rombi E., and Sini M.F. 2,6-Dimethylpyridine adsorption on Zirconia and sulfated Zirconia systems. An FT-IR and microcalorimetric study. Langmuir 19 (2003) 5344-5356
28. 2 systems. Langmuir 13 (1997) 888-894
29. Li B., and Gonzalez R.D. An in situ DRIFTS study of the deactivation and regeneration of sulfated zirconia. Catal. Today 46 (1998) 55-67
30. Morterra C., and Cerrato G. Brosted acidity of a superacid sulfate-doped ZrO2 system. J. Phys. Chem. 98 (1994) 12373-12381
31. Czerwinski W., Nowaczyk J., and Kania K. Ozonization of electronic conducting polymers. I. Copolymers based on poly [3-nonylthiophene]. Polym. Degrad. Stabil. 80 (2003) 93-101
32. 3 solid superacid catalysts for electrochemical reaction of toluene with methanol. J. Hazard. Mater. 145 (2007) 453-458
33. Corma A., and Garcia H. Naphthalene included within all-silica zeolites: influence of the host on the naphthalene photophysics. Chem. Rev. 102 (2002) 3837-3849