Preliminary kinetic study on the degradation of nitrobenzene by modified ceramic honeycomb-catalytic ozonation in aqueous solution

Journal of Hazardous Materials

Volumn 161, Issue 2-3, 2009, Pages 988-994

  Zhao, Lei ^a   Ma, Jun ^a   Sun, Zhi zhong ^b   Zhai, Xue dong ^a  

^a HARBIN INSTITUTE OF TECHNOLOGY   (China)

^b HEILONGJIANG UNIVERSITY   (China)

Author keywords

Catalytic ozonation; Ceramic honeycomb; Kinetics; Nitrobenzene; Pseudo first order

Indexed keywords

CATALYSIS; CATALYST ACTIVITY; CERAMIC MATERIALS; CONCENTRATION (PROCESS); COPPER; DEGRADATION; HONEYCOMB STRUCTURES; KINETIC THEORY; MANGANESE; MANGANESE COMPOUNDS; NITROBENZENE; OZONE; OZONIZATION; SOLUTIONS;

AQUEOUS SOLUTIONS; CATALYTIC ACTIVITIES; CATALYTIC OZONATION; CERAMIC HONEYCOMB; CERAMIC HONEYCOMBS; DEGRADATION RATES; EXPERIMENTAL CONDITIONS; FIRST ORDERS; HYDROXYL RADICALS; INFLUENCING FACTORS; INITIAL CONCENTRATIONS; INITIAL PH; KINETIC MODELS; KINETIC STUDIES; KINETICS OF DEGRADATIONS; OZONE CONCENTRATIONS; POSITIVE EFFECTS; PSEUDO-FIRST-ORDER; REACTION TEMPERATURES;

RATE CONSTANTS;

COPPER; HYDROXYL RADICAL; MANGANESE; NITROBENZENE; OZONE; POTASSIUM;

AQUEOUS SOLUTION; CATALYSIS; CERAMICS; CONCENTRATION (COMPOSITION); DEGRADATION; KINETICS; ORGANIC COMPOUND;

AQUEOUS SOLUTION; ARTICLE; CATALYSIS; CERAMICS; OZONATION;

CATALYSIS; CERAMICS; EQUIPMENT DESIGN; HYDROGEN-ION CONCENTRATION; HYDROXYL RADICAL; KINETICS; METALS; MODELS, CHEMICAL; NITROBENZENES; OZONE; SOLUTIONS; TEMPERATURE; TIME FACTORS; WATER POLLUTANTS, CHEMICAL; WATER PURIFICATION;

EID: 56249103773     PISSN: 03043894     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.jhazmat.2008.04.045     Document Type: Article

References (27)

1. Kasprzyk-Hordern B., Ziółek M., and Nawrocki J. Catalytic ozonation and methods of enhancing molecular ozone reactions in water treatment. Appl. Catal. B: Environ. 46 (2003) 639-669
2. Bellamy W.D., Damez F., Langlais B., Montiel A., Rakness K.L., Reckhow D.A., and Robson C.M. Engineering aspects. In: Langlais B., Reckhow D.A., and Brink D.R. (Eds). Ozone in Water Treatment: Application and Engineering (1991), Lewis Publishers, Chelsea, MI, USA 317-468
3. Camel V., and Bermond A. The use of ozone and associated oxidation processes in drinking water treatment. Water Res. 32 (1998) 3208-3222
4. Hoigné J. The Chemistry of Ozone in Water, Process Technologies for Water Treatment (1988), Plenum Press, New York
5. Legube B., and Karpel V.L.N. Catalytic ozonation: a promising advanced oxidation technology for water treatment. Catal. Today 53 (1999) 61-72
6. Ma J., Sui M.H., Chen Z.L., and Wang L.N. Degradation of refractory organic pollutants by catalytic ozonation-activated carbon and Mn-loaded activated carbon as catalysts. Ozone Sci. Eng. 26 (2004) 3-10
7. x/GAC catalyzed ozonation for degradation of nitrobenzene. Water Res. 39 (2005) 779-786
8. 2 catalyzed ozonation. J. Mol. Catal. A: Chem. 267 (2007) 41-48
9. Zhang T., and Ma J. Catalytic ozonation of trace nitrobenzene in water with synthetic goethite. J. Mol. Catal. A: Chem. 279 (2007) 82-89
10. Sun Z.Z., Ma J., Wang L.B., and Zhao L. Degradation of nitrobenzene in aqueous solution by ozone-ceramic honeycomb. J. Environ. Sci. 17 (2005) 716-721
11. Zhao L., Ma J., and Sun Z.Z. Oxidation products and pathway of ceramic honeycomb-catalyzed ozonation for the degradation of nitrobenzene in aqueous solution. Appl. Catal. B: Environ. 79 (2008) 244-253
12. Bardhan P. Ceramic honeycombs filters and catalysts. Curr. Opin. Solid State Mater. Sci. 2 (1997) 577-583
13. Bader H., and Hoigné J. Determination of ozone in water by the indigo method. Water Res. 19 (1981) 445-456
14. Staechlin J., and Hoigné J. Decomposition of ozone in water in the presence of organic solutes acting as promoters and inhibitors of radical chain reactions. Environ. Sci. Technol. 19 (1983) 1206-1213
15. Hoigné J., and Bader H. Rate constants of reactions of ozone with organic and inorganic compounds in water. I. Non-dissociating organic compounds. Water Res. 17 (1983) 173-183
16. Hoigné J., and Bader H. Rate constants of reactions of ozone with organic and inorganic compounds in water. II. Dissociating organic compounds. Water Res. 17 (1983) 185-194
17. Colin C., and Robbie B. An investigation of catalytic ozonation for the oxidation of halocarbons in drinking water preparation. Water Res. 23 (1999) 3695-3700
18. Farhataziz, A.B. Ross, Selected specific rates of reactions of transients from water in aqueous solutions. III. Hydroxyl radical and perhydroxyl radical and their radical ions. National Standard Reference Data System, U.S. Department of Commerce, National Bureau of Standards, Washington, DC, NSRDS-NBS59, 1977.
19. Hoigné J., Bader H., Haag W.R., and Staehelin J. Rate constants of reactions of ozone with organic and inorganic compounds in water. III. Inorganic compounds and radicals. Water Res. 19 (1985) 993-1004
20. Martín S.M.A., Fernández B.J.L., Martín M.A., and García G.I. Ozonation of vinasse in acid and alkaline media. J. Chem. Technol. Biot. 78 (2003) 1121-1127
21. Joon W.K., and Hoffmann M.R. Kinetics and mechanism of the sonolytic destruction of methyl tert-butyl ether by ultrasonic irradiation in the presence of ozone. Environ. Sci. Technol. 32 (1998) 3194-3199
22. Ma J., and Graham N.J.D. Preliminary investigation of manganese-catalyzed for the destruction of atrazine. Ozone Sci. Eng. 19 (1997) 227-240
23. Buxton G.V., Greenstock C.L., Helman W.P., and Ross A.B. Critical review of rate constants for reactions of hydrated electrons, hydrogen atoms and hydroxyl radicals in aqueous solution. J. Phys. Chem. Ref. Data 17 (1988) 513-817
24. Hoigné J., and Bader H. The role of hydroxyl radical reactions in ozonation process in aqueous solutions. Water Res. 10 (1997) 377-386
25. Masschelein W.J. Unit Processes in Drinking Water Treatment (1992), Marcel Dekker, New York
26. Park H.S., Huang T.M., Kang J.W., Choi H., and Oh H.J. Characterization of raw water for the ozone application measuring ozone consumption rate. Water Res. 35 (2001) 2607-2614
27. Wu I.N., and Wang T.W. Ozonation of aqueous azo dye in a semi-batch reactor. Water Res. 35 (2001) 1093-1099