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Volumn 78, Issue 16, 2008, Pages

Large third-order optical nonlinearity realized in symmetric nonpolar carotenoids

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EID: 54449085824     PISSN: 10980121     EISSN: 1550235X     Source Type: Journal    
DOI: 10.1103/PhysRevB.78.161101     Document Type: Article
Times cited : (7)

References (26)
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    • The largest γ value of C50 is actually 34× 10-32 esu and is located at around 17300 cm-1. This γ value is, however, anomalously enhanced compared with the simulated result. The disagreement is accounted for the effect of the experimental artifact, which has been marked in the phase spectra (Ref.). For this reason, we consider that the experimental γmax of C50 is located at 18550 cm-1 (31× 10-32 esu), at which the simulated γ spectrum also has its maximum.
    • The largest γ value of C50 is actually 34× 10-32 esu and is located at around 17300 cm-1. This γ value is, however, anomalously enhanced compared with the simulated result. The disagreement is accounted for the effect of the experimental artifact, which has been marked in the phase spectra (Ref.). For this reason, we consider that the experimental γmax of C50 is located at 18550 cm-1 (31× 10-32 esu), at which the simulated γ spectrum also has its maximum.
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    • In the phase spectra, an experimental artifact is observed at the same energy region in every homologue. The origin of this artifact is not clear. However, we believe that it is an artifact because at the energy at which it is located the homologues do not have any absorption and so the phase angle would be expected to be zero.
    • In the phase spectra, an experimental artifact is observed at the same energy region in every homologue. The origin of this artifact is not clear. However, we believe that it is an artifact because at the energy at which it is located the homologues do not have any absorption and so the phase angle would be expected to be zero.
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    • There exists a one-photon forbidden state, S1, between S0 and S2. It does not actually contribute to the THG process. Note that the S2 and Sm states in the present study are denoted S1 and S2, respectively, in Ref..
    • There exists a one-photon forbidden state, S1, between S0 and S2. It does not actually contribute to the THG process. Note that the S2 and Sm states in the present study are denoted S1 and S2, respectively, in Ref..
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* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.