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Ref. also studied the plasmonic attractive bonding forces by using electrodynamics. Our study differs from Ref. in that Ref. focuses on how the optical force affects the surface enhance Raman spectroscopy, whereas we focus on the properties of the optical force itself.
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Ref. also studied the plasmonic attractive bonding forces by using electrodynamics. Our study differs from Ref. in that Ref. focuses on how the optical force affects the surface enhance Raman spectroscopy, whereas we focus on the properties of the optical force itself.
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Throughout this paper, the angular momentum truncation orders for the MS-MST calculations are taken as 43, 75, 76, 93, 94, and 96 for nanospheres of radii 5, 30, 50, 100, 150, and 200 nm, respectively. We remark that since electrodynamics is not valid for near touching spheres, our result with smaller separation [e.g., (D-2 rs) <1 nm] is less accurate.
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Throughout this paper, the angular momentum truncation orders for the MS-MST calculations are taken as 43, 75, 76, 93, 94, and 96 for nanospheres of radii 5, 30, 50, 100, 150, and 200 nm, respectively. We remark that since electrodynamics is not valid for near touching spheres, our result with smaller separation [e.g., (D-2 rs) <1 nm] is less accurate.
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However, for extremely closely spaced particles, say when the gap between the particles is less than 1 nm, in this case, the electrons on one of the sphere can actually leak to the other sphere. In other words, classical electrodynamics, and hence the MS-MST formalism, is not accurate.
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However, for extremely closely spaced particles, say when the gap between the particles is less than 1 nm, in this case, the electrons on one of the sphere can actually leak to the other sphere. In other words, classical electrodynamics, and hence the MS-MST formalism, is not accurate.
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This is because the terms that are quadratic in incident field equally contribute to both spheres and therefore do not contribute to the binding force, and the terms that are quadratic in the resonant scattered field are too small owing to the weak coupling between the particles.
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