Growing correlation length on cooling below the onset of caging in a simulated glass-forming liquid

Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics

Volumn 66, Issue 3, 2002, Pages

  Lacevic N ^a,b,c   Starr, F W ^b   Schroder T B ^b,d   Novikov, V N ^b   Glotzer, S C ^a,b  

^a UNIVERSITY OF MICHIGAN   (United States)

^b NATIONAL INSTITUTE OF STANDARDS AND TECHNOLOGY   (United States)

^c JOHNS HOPKINS UNIVERSITY   (United States)

^d ROSKILDE UNIVERSITY   (Denmark)

Author keywords

[No Author keywords available]

Indexed keywords

CORRELATION LENGTHS; DENSITY CORRELATION FUNCTIONS; GLASS-FORMING LIQUIDS; LENNARD-JONES LIQUIDS;

COMPUTER SIMULATION; COOLING SYSTEMS; CORRELATION METHODS; GLASS TRANSITION; LIQUIDS; MOLECULAR DYNAMICS; RELAXATION PROCESSES; THERMAL EFFECTS;

DENSITY OF LIQUIDS;

ARTICLE;

EID: 41349105662     PISSN: 1063651X     EISSN: None     Source Type: Journal    
DOI: 10.1103/PhysRevE.66.030101     Document Type: Article

References (48)

1. H. Sillescu, J. Non-Cryst. Solids 243, 81 (1999).
2. M.D. Ediger, Annu. Rev. Phys. Chem. 51, 99 (2000).
3. S.C. Glotzer, J. Non-Cryst. Solids 274, 342 (2000).
4. W. Götze and L. Sjögren, Rep. Prog. Phys. 55, 241 (1992).
5. M.R. Ernst, Phys. Rev. B 43, 8070 (1991).
6. R.L. Leheny, J. Chem. Phys. 105, 7783 (1996);
7. A. van Blaaderen and P. Wiltzius, Science 270, 1177 (1995).
8. W. Kob, C. Donati, P.H. Poole, S.J. Plimpton, and S.C. Glotzer, Phys. Rev. Lett. 79, 2827 (1997);
9. Phys. Rev. Lett.C. Donati, S.C. Glotzer, and P.H. Poole, 82, 5064 (1999);
10. C. Donati, Phys. Rev. E 60, 3107 (1999);
11. C. Bennemann, C. Donati, J. Baschnagel, and S.C. Glotzer, Nature (London) 399, 246 (1999);
12. Y. Gebremichael, T.B. Schrøder, F.W. Starr, and S.C. Glotzer, Phys. Rev. E 64, 051503 (2001).
13. See e.g., B. Doliwa and A. Heuer, Phys. Rev. E 61, 6898 (2000);
14. R. Yamamoto and A. Onuki, Phys. Rev. Lett. 81, 4915 (1998);
15. R. YamamotoA. OnukiPhys. Rev. E 58, 3515 (1998);
16. Phys. Rev. ET. Muranaka and Y. Hiwatari, 51, R2735 (1995);
17. Phys. Rev. EM. Hurley and P. Harrowell, 52, 1694 (1995);
18. J. Qian, R. Hentschke, and A. Heuer, J. Chem. Phys. 111, 10177 (1999);
19. A.I. Mel’cuk, Phys. Rev. Lett. 75, 2522 (1995);
20. G. Johnson, Phys. Rev. E 57, 5707 (1998);
21. N.E. Moe and M.D. Ediger, Polymer 37, 1787 (1996);
22. J.P. Garrahan and D. Chandler, Phys. Rev. Lett. 89, 035704 (2002).
23. W.K. Kegel and A. van Blaaderen, Science 287, 290 (2000);
24. ScienceE.R. Weeks, 287, 627 (2000);
25. S.C. Glotzer, Phys. World 13, 22 (2000).
26. C. Dasgupta, A.V. Indrani, S. Ramaswamy, and M.K. Phani, Europhys. Lett. 15, 307 (1991);
27. Europhys. Lett.C. DasguptaA.V. IndraniS. RamaswamyM.K. Phani15, 467 (1991).
28. C. Donati, S. Franz, G. Parisi, S.C. Glotzer, and G. Parisi, J. Non-Cryst. Solids (to be published).
29. S.C. Glotzer, V.N. Novikov, and T.B. Schrøder, J. Chem. Phys. 112, 509 (2000).
30. J. P. Hansen and I. R. McDonald, Theory of Simple Liquids (Academic Press, New York, 1986).
31. S. Franz, Philos. Mag. B 79, 1827 (1999);
32. S. Franz and G. Parisi, J. Phys.: Condens. Matter 12, 6335 (2000).
33. S. Franz and G. Parisi, Phys. Rev. Lett. 79, 2486 (1997);
34. Phys. Rev. Lett.G. Parisi, 50, 1946 (1983);
35. S.F. Edwards and P.W. Anderson, J. Phys. F: Met. Phys. 5, 965 (1975).
36. N. Lačević et al. (unpublished).
37. H. E. Stanley, Introduction to Phase Transitions and Critical Phenomena (Oxford University Press, New York, 1971).
38. J. Colmenero, Phys. Rev. Lett. 69, 478 (1992);
39. Phys. Rev. Lett.A. Arbe, 81, 590 (1998).
40. U. Tracht, Phys. Rev. Lett. 81, 2727 (1998);
41. H.W. Spiess, Macromol. Symp. 117, 257 (1997);
42. K. Schmidt-Rohr and H.W. Spiess, Phys. Rev. Lett. 66, 3020 (1991).
43. The LJ interaction parameters (Formula presented) and (Formula presented) are given by (Formula presented) (Formula presented) (Formula presented) (Formula presented) Lengths are defined in units of (Formula presented) temperature T in units of (Formula presented) and time in units of (Formula presented)
44. T.B. Schrøder, et al., J. Chem. Phys. 112, 9834 (2000).
45. Strictly speaking, a simulation in the grand canonical ensemble would instead yield a small but nonzero (Formula presented) value at early times.
46. R.D. Mountain, ACS Symp. Ser. 676, 122 (1997);
47. R.D. Mountain, J. Chem. Phys. 102, 5408 (1995);
48. R. Ahluwalia and S.P. Das, Phys. Rev. E 57, 5771 (1997).