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Volumn 111, Issue 47, 2007, Pages 13404-13409

Molecular motion of a nickel-bis(dithiolato) complex in solution

(12) Kowert, Bruce A a Broeker, Gregory K a Gentemann, Steven J a Stemmler, Timothy L a Fehr, Michael J a Stemmler, Ann Joern a Thurman Keup, Eva M a McCoo, Penelope Whittington a Everett, Theodoro B a Lupo, Darret J a Fitzsimmons, Patricia K a Cordero, Ana Barros a

a Saint Louis University (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ALCOHOLS; DIFFUSION; MOLECULAR STRUCTURE; NEGATIVE IONS; PARAMAGNETIC RESONANCE; SOLVENTS;

DIFFUSION CONSTANTS; MOLECULAR MOTION; POLAR SOLVENTS;

NICKEL COMPOUNDS;

EID: 36949035770 PISSN: 15206106 EISSN: None Source Type: Journal
DOI: 10.1021/jp077072y Document Type: Article

Times cited : (3)

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- Consider the case when only gx (associated with the low field feature) is temperature-dependent. In the spectrum calculated using the glassy gi in Figure 4, the central feature, as noted previously, is up field from the experimental value. The separations between it and the low and high field features are greater than and less than the observed values, respectively. The only way to bring these separations into agreement with experiment is to decrease both gx and D ⊥. The decrease in gx is unacceptable and also causes the absolute positions of the three features to be slightly upfield from their experimental values. If gz (associated with the high field feature) is temperature-dependent, one matches the experimental separations by decreasing it and increasing D⊥, which again is unacceptable. As for gxT, the calculated positions of th
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- ⊥).

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