Time and frequency resolved dynamics of ArBr2

Journal of Chemical Physics

Volumn 127, Issue 16, 2007, Pages

  Cabrera, Jose ^a,c   Bieler, Craig R ^a,d   McKinney, Natalie ^a,d   Van Der Veer, Wytze E ^a   Pio, Jordan M ^a   Janda, Kenneth ^a   Roncero, Octavio ^b  

^a UNIVERSITY OF CALIFORNIA   (United States)

^b INSTITUTO DE MATEMÁTICAS Y FÍSICA FUNDAMENTAL   (Spain)

^c STANFORD UNIVERSITY   (United States)

^d ALBION COLLEGE   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

BROMINE COMPOUNDS; FOURIER ANALYSIS; ISOMERS; QUANTUM THEORY; VIBRATIONAL SPECTRA;

BOND ENERGY; FREQUENCY RESOLUTION; QUANTUM NUMBERS; VIBRATIONAL RELAXATION;

ARGON;

EID: 36048965481     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.2794332     Document Type: Article

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36. As pointed out by the reviewer, we are reporting "product appearance times" for the excitation to a particular level. More precisely, what we refer to as a lifetime is 1/k for a single exponential fit to the product appearance. Given the frequency width of our laser and the uncertainty width of the individual rotational levels, it is not possible to directly measure state-to-state dynamics. We therefore follow the traditional practice of referring to the inverse product appearance rate constants as life-times.