How adiabatic is activated adsorption/associative desorption?

Journal of Chemical Physics

Volumn 123, Issue 7, 2005, Pages

  Luntz, A C ^a   Persson, M ^b  

^a UNIVERSITY OF SOUTHERN DENMARK   (Denmark)

^b UNIVERSITY OF GOTHENBURG   (Sweden)

Author keywords

[No Author keywords available]

Indexed keywords

ACTIVATION ANALYSIS; ADSORPTION; DESORPTION; DISSOCIATION; ELECTRON MOBILITY; ELECTRONIC STRUCTURE; FRICTION; HOLE MOBILITY; PROBABILITY DENSITY FUNCTION; REACTION KINETICS;

ACTIVATED ADSORPTION; ASSOCIATIVE DESORPTION; ELECTRON-HOLE PAIR; NUCLEAR MOTION;

CHEMICAL ACTIVATION;

EID: 34547853977     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.2000249     Document Type: Article

References (34)

1. J. E. Lennard-Jones, Trans. Faraday Soc. 28, 333 (1932).
2. E. Müller-Hartmann, T. V. Ramakrishnan, and G. Toulouse, Phys. Rev. B 3, 1102 (1971).
3. J. W. Gadzuk and H. Metiu, Phys. Rev. B 22, 2603 (1980).
4. R. Brako and D. M. Newns, Solid State Commun. 33, 713 (1980).
5. K. Schönhammer and O. Gunnarsson, Phys. Rev. B 27, 5113 (1983).
6. R. Brako and D. M. Newns, Rep. Prog. Phys. 52, 655 (1989).
7. J. R. Schrieffer, J. Vac. Sci. Technol. 13, 335 (1976);
8. J. K. Nørskov, 18, 420 (1981).
9. B. Kasemo, E. Tornqvist, J. K. Nørskov, and B. I. Lundqvist, Surf. Sci. 89, 554 (1979).
10. G. J. Kroes, Prog. Surf. Sci. 60, 1 (1999).
11. L. Diekhöner, L. Hornekær, H. Mortensen, E. Jensen, A. Baurichter, V. Petrunin, and A. C. Luntz, J. Chem. Phys. 117, 5018 (2002).
12. D.C. Langreth and M. Persson, in Laser Spectroscopy and Photochemistry on Metal Surfaces, edited by, H.-L. Dai, and, W. Ho, (World Scientific, River Edge, New Jersey, 1995), Vol. 5, p. 498.
13. B. Hammer, M. Scheffler, K. W. Jacobsen, and J. K. Nörskov, Phys. Rev. Lett. 73, 1400 (1994).
14. M. J. Murphy, J. F. Skelly, A. Hodgson, and B. Hammer, J. Chem. Phys. 110, 6954 (1999).
15. M. Head-Gordon and J. C. Tully, J. Chem. Phys. 96, 3939 (1992);
16. M. Persson, Philos. Trans. R. Soc. London, Ser. A 362, 1173 (2004).
17. E. G. Dagliano, P. Kumar, W. Schaich, and H. Suhl, Phys. Rev. B 11, 2122 (1975).
18. J. R. Trail, D. M. Bird, M. Persson, and S. Holloway, J. Chem. Phys. 119, 4539 (2003).
19. B. N. J. Persson and M. Persson, Solid State Commun. 36, 175 (1980).
20. B. Hellsing and M. Persson, Phys. Scr. 29, 360 (1984).
21. M. Head-Gordon and J. C. Tully, J. Chem. Phys. 103, 10137 (1995).
22. G. Kresse and J. Furthmuller, Phys. Rev. B 54, 11169 (1996).
23. M. Head-Gordon and J. C. Tully, Phys. Rev. B 46, 1853 (1992).
24. N. Lorente and M. Persson, Faraday Discuss. 117, 277 (2000).
25. S. Sakong and A. Gross, Surf. Sci. 525, 107 (2003).
26. B. Hammer and J. K. Nørskov, Surf. Sci. 343, 211 (1995).
27. J. Dai and J. Z. H. Zhang, J. Chem. Phys. 102, 6280 (1995).
28. H. A. Michelsen, C. T. Rettner, D. J. Auerbach, and R. N. Zare, J. Chem. Phys. 98, 8294 (1993).
29. L. Diekhöner, H. Mortensen, A. Baurichter, E. Jensen, V. Petrunin, and A. C. Luntz, J. Chem. Phys. 115, 9028 (2001).
30. B. Hammer and J.K. Nørskov, in Advances in Catalysis (Academic, San Diego, 2000), Vol. 45, p. 71.
31. J. T. Kindt, J. C. Tully, M. Head-Gordon, and M. A. Gomez, J. Chem. Phys. 109, 3629 (1998).
32. Y. H. Huang, C. T. Rettner, D. J. Auerbach, and A. M. Wodtke, Science 290, 111 (2000).
33. B. Gergen, H. Nienhaus, W. H. Weinberg, and E. W. McFarland, Science 294, 2521 (2001).
34. H. Nienhaus, Surf. Sci. Rep. 45, 3 (2002).