메뉴 건너뛰기




Volumn 110, Issue 16, 1988, Pages 5471-5479

Catalytic Photochemical Oxidation of Organic Substrates by Polyoxometalates. Picosecond Spectroscopy, Photochemistry, and Structural Properties of Charge-Transfer Complexes between Heteropolytungstic Acids and Dipolar Organic Compounds

Author keywords

[No Author keywords available]

Indexed keywords


EID: 33845278638     PISSN: 00027863     EISSN: 15205126     Source Type: Journal    
DOI: 10.1021/ja00224a035     Document Type: Article
Times cited : (159)

References (51)
  • 1
    • 0004275283 scopus 로고
    • Heteropoly and Isopoly Oxometalates
    • Springer-Verlag: Berlin
    • Pope, M. T. Heteropoly and Isopoly Oxometalates; Springer-Verlag: Berlin, 1983.
    • (1983)
    • Pope, M.T.1
  • 2
    • 13844278943 scopus 로고
    • Washington, D.C.
    • Day, V. W.; Klemperer, W. G. Science (Washington, D.C.) 1985, 228, 533.
    • (1985) Science , vol.228 , pp. 533
    • Day, V.W.1    Klemperer, W.G.2
  • 3
    • 11544301429 scopus 로고
    • Reviews (b) Kozhevnikov, I. V.; Matveev, K. I. Appl. Catal. 1983, 5, 135.
    • Reviews: (a) Kozhevnikov, I. V.; Matveev, K. I. Russ. Chem. Rev. (Engl. Transl.) 1982, 51, 1075. (b) Kozhevnikov, I. V.; Matveev, K. I. Appl. Catal. 1983, 5, 135.
    • (1982) Russ. Chem. Rev. (Engl. Transl.) , vol.51 , pp. 1075
    • Kozhevnikov, I.V.1    Matveev, K.I.2
  • 4
    • 33748733221 scopus 로고
    • A large number of papers addressing the use of polyoxometalates in heterogeneous catalysis exist. Recent representative examples (b) Moffat, J. B. J. Mol. Catal. 1984, 26, 385. (c) Akimoto, M.; Ikeda, H.; Oka be, A.; Echigoya, E. J. Catal. 1984, 89, 196. (d) Hayashi, H.; Moffat, J. B. Chem. Rev. (Engl. Transl.). 1983, 83, 192; 81, 61. (e) Konshi, Y.; Sakata, K.; Misono, M.; Yoneda, Y. Chem. Rev. (Engl. Transl.). 1982, 77, 169.
    • A large number of papers addressing the use of polyoxometalates in heterogeneous catalysis exist. Recent representative examples: (a) McMonagle, J. B.; Moffat, J. B. J. Catal. 1985, 91, 132. (b) Moffat, J. B. J. Mol. Catal. 1984, 26, 385. (c) Akimoto, M.; Ikeda, H.; Oka be, A.; Echigoya, E. J. Catal. 1984, 89, 196. (d) Hayashi, H.; Moffat, J. B. Chem. Rev. (Engl. Transl.). 1983, 83, 192; 81, 61. (e) Konshi, Y.; Sakata, K.; Misono, M.; Yoneda, Y. Chem. Rev. (Engl. Transl.). 1982, 77, 169.
    • (1985) J. Catal. , vol.91 , pp. 132
    • McMonagle, J.B.1    Moffat, J.B.2
  • 5
    • 85022753033 scopus 로고
    • (b) Besecker, C. J.; Day, V. W.; Klemperer, W. G.; Thompson, M. R. J. Am. Chem. Soc. 1984, 106, 4125. (c) Besecker, C. J.; Day, V. W.; Klemperer, W. G.; Thompson, M. R. Inorg. Chem. 1985, 24, 44. (d) Day, V. W.; Klemperer, W. G.; Maltbie, D. J. Organometallics 1985, 4, 104. (e) Besecker, C. J.; Klemperer, W. G.; Maltbie, D. J.; Wright, D. A. Inorg. Chem. 1985, 24, 1027. (f) Che, T. M.; Day, V. W.; Francesconi, L. C.; Fredrich, M. F.; Klemperer, W. G. Chem. Rev. (Engl. Transl.). 1985, 24, 4055. (g) Day, V. W.; Earley, C. W.; Klemperer, W. G.; Maltbie, D. J. J. Am. Chem. Soc. 1985, 107, 8261 and references cited in each.
    • Besecker, C. J.; Klemperer, W. G. J. Organomet. Chem. 1981, 205, C31. (b) Besecker, C. J.; Day, V. W.; Klemperer, W. G.; Thompson, M. R. J. Am. Chem. Soc. 1984, 106, 4125. (c) Besecker, C. J.; Day, V. W.; Klemperer, W. G.; Thompson, M. R. Inorg. Chem. 1985, 24, 44. (d) Day, V. W.; Klemperer, W. G.; Maltbie, D. J. Organometallics 1985, 4, 104. (e) Besecker, C. J.; Klemperer, W. G.; Maltbie, D. J.; Wright, D. A. Inorg. Chem. 1985, 24, 1027. (f) Che, T. M.; Day, V. W.; Francesconi, L. C.; Fredrich, M. F.; Klemperer, W. G. Chem. Rev. (Engl. Transl.). 1985, 24, 4055. (g) Day, V. W.; Earley, C. W.; Klemperer, W. G.; Maltbie, D. J. J. Am. Chem. Soc. 1985, 107, 8261 and references cited in each.
    • (1981) J. Organomet. Chem. , vol.C31 , pp. 205
    • Besecker, C.J.1    Klemperer, W.G.2
  • 6
    • 0000512482 scopus 로고
    • (b) Finke, R. G.; Droege, M. W. Chem. Rev. (Engl. Transl.). 1984, 106, 7274. (c) Finke, R. G.; Droege, M. W.; Cook, J. C.; Suslick, K. S. Chem. Rev. (Engl. Transl.). 1984, 106, 5750 and references in each.
    • Finke, R. G.; Droege, M.; Hutchinson, J. R.; Gansow, O. J. Am. Chem. Soc. 1981, 103, 1587. (b) Finke, R. G.; Droege, M. W. Chem. Rev. (Engl. Transl.). 1984, 106, 7274. (c) Finke, R. G.; Droege, M. W.; Cook, J. C.; Suslick, K. S. Chem. Rev. (Engl. Transl.). 1984, 106, 5750 and references in each.
    • (1981) J. Am. Chem. Soc. , vol.103 , pp. 1587
    • Finke, R.G.1    Droege, M.2    Hutchinson, J.R.3    Gansow, O.4
  • 8
    • 0000811423 scopus 로고
    • (b) Knoth, W. H. J. Am. Chem. Soc. 1979, 101, 2211. (c) Domaille, P. J.; Knoth, W. H. Inorg. Chem. 1983, 22, 818. (d) Knoth, W. H.; Domaille, P. J.; Farlee, R. D. Organometallics 1985, 4, 62.
    • Knoth, W. H. J. Am. Chem. Soc. 1979, 101, 759. (b) Knoth, W. H. J. Am. Chem. Soc. 1979, 101, 2211. (c) Domaille, P. J.; Knoth, W. H. Inorg. Chem. 1983, 22, 818. (d) Knoth, W. H.; Domaille, P. J.; Farlee, R. D. Organometallics 1985, 4, 62.
    • (1979) J. Am. Chem. Soc. , vol.101 , pp. 759
    • Knoth, W.H.1
  • 9
    • 0002566110 scopus 로고
    • Chem. Lett
    • (b) Yamase, T.; Hayashi, H.; Ikawa, T. J. Am. Chem. Soc. 1974, 1055. (c) Yamase, T.; Ikawa, T. Bull. Chem. Soc. Jpn. 1977, 50, 746. (d) Yamase, T. J. Chem. Soc., Dalton Trans. 1978, 238. (e) Yamase, T.; Ikawa, T. Inorg. Chim. Acta 1979, 37, L529. (f) Yamase, T.; Ikawa, T. J. Am. Chem. Soc. 1980, 45, L55. (g) Yamase, T. J. Am. Chem. Soc. 1981, 54, L165. (h) Yamase, T.; Sasaki, R.; Ikawa, T. J. Chem. Soc., Dalton Trans. 1981, 628. (i) Yamase, T. Inorg. Chim. Acta 1981, 54, L207. (j) Yamase, T. J. Am. Chem. Soc. 1982, 64, L155. (k) Yamase, T. J. Chem. Soc., Dalton Trans. 1982, 1987. (l) Yamase, T.; Kurozumi, T. J. Am. Chem. Soc. 1983, 2205. (m) Yamase, T. Inorg. Chim. Acta 1983, 76, L25. (n) Yamase, T.; Kurozumi, T. J. Am. Chem. Soc. 1984, 83, L25. (o) Yamase, T. J. Chem. Soc., Dalton Trans. 1985, 2586.
    • Yamase, T. Chem. Lett. 1973, 615. (b) Yamase, T.; Hayashi, H.; Ikawa, T. J. Am. Chem. Soc. 1974, 1055. (c) Yamase, T.; Ikawa, T. Bull. Chem. Soc. Jpn. 1977, 50, 746. (d) Yamase, T. J. Chem. Soc., Dalton Trans. 1978, 238. (e) Yamase, T.; Ikawa, T. Inorg. Chim. Acta 1979, 37, L529. (f) Yamase, T.; Ikawa, T. J. Am. Chem. Soc. 1980, 45, L55. (g) Yamase, T. J. Am. Chem. Soc. 1981, 54, L165. (h) Yamase, T.; Sasaki, R.; Ikawa, T. J. Chem. Soc., Dalton Trans. 1981, 628. (i) Yamase, T. Inorg. Chim. Acta 1981, 54, L207. (j) Yamase, T. J. Am. Chem. Soc. 1982, 64, L155. (k) Yamase, T. J. Chem. Soc., Dalton Trans. 1982, 1987. (l) Yamase, T.; Kurozumi, T. J. Am. Chem. Soc. 1983, 2205. (m) Yamase, T. Inorg. Chim. Acta 1983, 76, L25. (n) Yamase, T.; Kurozumi, T. J. Am. Chem. Soc. 1984, 83, L25. (o) Yamase, T. J. Chem. Soc., Dalton Trans. 1985, 2586.
    • (1973) , pp. 615
    • Yamase, T.1
  • 10
    • 37049109818 scopus 로고
    • (b) Yamase, T.; Watanabe, R. J. Chem. Soc., Dalton Trans. 1986, 1669.
    • Yamase, T.; Takabayashi, N.; Kaji, M. J. Chem. Soc., Dalton Trans. 1984, 793. (b) Yamase, T.; Watanabe, R. J. Chem. Soc., Dalton Trans. 1986, 1669.
    • (1984) J. Chem. Soc., Dalton Trans. , vol.793
    • Yamase, T.1    Takabayashi, N.2    Kaji, M.3
  • 11
    • 0000386379 scopus 로고
    • Inorg. Chim. Acta
    • (b) Papaconstantinou, E.; Ioannidis, A. J. Am. Chem. Soc. 1983, 75, 235. (c) Dimotikali, D.; Papaconstantinou, E. J. Am. Chem. Soc. 1984, 87, 177. (d) Ioannidis, A.; Papaconstantinou, E. Inorg. Chem. 1985, 24, 439. (e) Argitis, P.; Papaconstantinou, E. J. Am. Chem. Soc. 1986, 25, 4386.
    • Papaconstantinou, E.; Dimotikali, D.; Politou, A. Inorg. Chim. Acta 1980, 46, 155. (b) Papaconstantinou, E.; Ioannidis, A. J. Am. Chem. Soc. 1983, 75, 235. (c) Dimotikali, D.; Papaconstantinou, E. J. Am. Chem. Soc. 1984, 87, 177. (d) Ioannidis, A.; Papaconstantinou, E. Inorg. Chem. 1985, 24, 439. (e) Argitis, P.; Papaconstantinou, E. J. Am. Chem. Soc. 1986, 25, 4386.
    • (1980) , vol.46 , pp. 155
    • Papaconstantinou, E.1    Dimotikali, D.2    Politou, A.3
  • 13
    • 37049100704 scopus 로고
    • (b) Akid, R.; Darwent, J. R. J. Chem. Soc., Dalton Trans. 1985, 395.
    • Darwent, J. R. J. Chem. Soc., Chem. Commun. 1982, 798. (b) Akid, R.; Darwent, J. R. J. Chem. Soc., Dalton Trans. 1985, 395.
    • (1982) J. Chem. Soc., Chem. Commun. , pp. 798
    • Darwent, J.R.1
  • 16
    • 0011295044 scopus 로고
    • Polyhedron
    • (b) Nomiya, K.; Miyazaki, T.; Maeda, K.; Miwa, M. Inorg. Chim. Acta 1987, 127, 65.
    • Nomiya, K.; Sugie, Y.; Miyazaki, T.; Miwa, M. Polyhedron 1986, 5, 1267. (b) Nomiya, K.; Miyazaki, T.; Maeda, K.; Miwa, M. Inorg. Chim. Acta 1987, 127, 65.
    • (1986) , vol.5 , pp. 1267
    • Nomiya, K.1    Sugie, Y.2    Miyazaki, T.3    Miwa, M.4
  • 18
    • 33845375145 scopus 로고
    • (b) Renneke, R. F.; Hill, C. L. J. Am. Chem. Soc., preceding paper in this issue.
    • Renneke, R. F.; Hill, C. L. J. Am. Chem. Soc. 1986, 108, 3528. (b) Renneke, R. F.; Hill, C. L. J. Am. Chem. Soc., preceding paper in this issue.
    • (1986) J. Am. Chem. Soc. , vol.108 , pp. 3528
    • Renneke, R.F.1    Hill, C.L.2
  • 22
    • 34250528065 scopus 로고
    • Colored solutions of heteropoly compounds in organic solvents have been noted before. See work cited in ref 1 and
    • Colored solutions of heteropoly compounds in organic solvents have been noted before. See work cited in ref 1 and: Umland, F.; Wuensch, G. Z. Anal. Chem. 1967, 225, 362.
    • (1967) Z. Anal. Chem. , vol.225 , pp. 362
    • Umland, F.1    Wuensch, G.2
  • 24
    • 0000040711 scopus 로고
    • 3- has yet to be well characterized, we have evidence that it exists and can be present as a minor impurity in the α isomer.
    • 3- has yet to be well characterized, we have evidence that it exists and can be present as a minor impurity in the α isomer.
    • (1920) J. Biol. Chem. , vol.43 , pp. 189
    • Wu, H.1
  • 28
    • 84980089549 scopus 로고
    • Acta Crystallogr., Sect. A: Cryst. Phys., Diffr. Theor. Gen. Crystallogr
    • North, A. C. T.; Phillips, D. C. Mathews, F. C. Acta Crystallogr., Sect. A: Cryst. Phys., Diffr. Theor. Gen. Crystallogr. 1968, A24, 351.
    • (1968) , vol.A24 , pp. 351
    • North, A.C.T.1    Phillips, D.C.2    Mathews, F.C.3
  • 29
    • 0000409196 scopus 로고
    • Acta Crystallogr
    • Larsen, A. C. Acta Crystallogr. 1967, 23, 664.
    • (1967) , vol.23 , pp. 664
    • Larsen, A.C.1
  • 30
    • 0003872738 scopus 로고
    • International Tables of X-ray Crystallogrphy
    • Kynoch: Birmingham, England Table 2.2B.
    • Cromer, D. T.; Waber, J. T. International Tables of X-ray Crystallogrphy; Kynoch: Birmingham, England, 1974; Vol. 4, Table 2.2B.
    • (1974) , vol.4
    • Cromer, D.T.1    Waber, J.T.2
  • 31
    • 0001222418 scopus 로고
    • (b) Bent, H. E.; French, C. L. J. Am. Chem. Soc. 1941, 63, 568. (c) Benesi, H. A. Hildebrand, J. H. J. Am. Chem. Soc. 1949, 71, 2703.
    • Benesi, H. A.; Hildebrand, J. H. J. Am. Chem. Soc. 1948, 70, 3978. (b) Bent, H. E.; French, C. L. J. Am. Chem. Soc. 1941, 63, 568. (c) Benesi, H. A. Hildebrand, J. H. J. Am. Chem. Soc. 1949, 71, 2703.
    • (1948) J. Am. Chem. Soc. , vol.70 , pp. 3978
    • Benesi, H.A.1    Hildebrand, J.H.2
  • 34
    • 0042553279 scopus 로고
    • Anal. Chem
    • Savitzky, A.; Golay, M. J. E. Anal. Chem. 1964, 36, 1627.
    • (1964) , vol.36 , pp. 1627
    • Savitzky, A.1    Golay, M.J.E.2
  • 35
    • 33845469139 scopus 로고
    • Inorg. Chem
    • For a reasonable description of this symmetry problem see
    • For a reasonable description of this symmetry problem see: Evans, H. T., Jr.; Pope, M. T. Inorg. Chem. 1984, 23, 501.
    • (1984) , vol.23 , pp. 501
    • Evans, H.T.1    Pope, M.T.2
  • 37
    • 0039720524 scopus 로고
    • (b) Rao, Ch. P.; Rao, A. M.; Rao, C. N. R. Inorg. Chem. 1984, 23, 2080 and references cited in each.
    • Hill, C. L.; Williamson, M. M. Inorg. Chem. 1985, 24, 2836. (b) Rao, Ch. P.; Rao, A. M.; Rao, C. N. R. Inorg. Chem. 1984, 23, 2080 and references cited in each.
    • (1985) Inorg. Chem. , vol.24 , pp. 2836
    • Hill, C.L.1    Williamson, M.M.2
  • 38
    • 0002934882 scopus 로고
    • Perspect. Struct. Chem
    • Review of early polyoxometalate structural investigations
    • Review of early polyoxometalate structural investigations: Evans, H. T. Perspect. Struct. Chem. 1971, 4, 1.
    • (1971) , vol.4 , pp. 1
    • Evans, H.T.1
  • 39
    • 0002429423 scopus 로고
    • Proc. R. Soc. London, Ser. A
    • Keggin, J. F. Proc. R. Soc. London, Ser. A 1934, A144, 75.
    • (1934) , vol.A144 , pp. 75
    • Keggin, J.F.1
  • 43
    • 0004274056 scopus 로고
    • Molecular Complexes
    • Wiley-Interscience: New York many references cited therein.
    • Mulliken, R. S.; Person, W. B. Molecular Complexes; Wiley-Interscience: New York, 1969; many references cited therein.
    • (1969)
    • Mulliken, R.S.1    Person, W.B.2
  • 44
    • 0003450560 scopus 로고
    • Organic Charge-Transfer Complexes
    • Reviews of organic electron donor-acceptor complexes Academic: New York (b) Molecular Complexes; Foster, R., Ed.; Crane, Russak and Co.; New York; 1973, Vol. 1; 1974, Vol. 2. (c) Molecular Association; Foster, R., Ed.; Academic: New York: 1975, Vol. 1; 1979, Vol. 2. (d) Kosower, E. Prog. Phys. Org. Chem. 1965, 3, 81. (e) Kosower, E. Physical Organic Chemistry; Wiley: New York, 1968; pp 179–195.
    • Reviews of organic electron donor-acceptor complexes: (a) Foster, R. Organic Charge-Transfer Complexes; Academic: New York, 1969. (b) Molecular Complexes; Foster, R., Ed.; Crane, Russak and Co.; New York; 1973, Vol. 1; 1974, Vol. 2. (c) Molecular Association; Foster, R., Ed.; Academic: New York: 1975, Vol. 1; 1979, Vol. 2. (d) Kosower, E. Prog. Phys. Org. Chem. 1965, 3, 81. (e) Kosower, E. Physical Organic Chemistry; Wiley: New York, 1968; pp 179–195.
    • (1969)
    • Foster, R.1
  • 45
    • 4243160964 scopus 로고
    • (b) Masnovi, J. M.; Kochi, J. K.; Hilinski, E. F.; Rentzepis, P. M. J. Am. Chem. Soc. 1986, 108, 1126.
    • Masnovi, J. M.; Huffman, J. C.; Kochi, J. K.; Hilinski, E. F.; Rentzepis, P. M. Chem. Phys. Lett. 1984, 106, 20. (b) Masnovi, J. M.; Kochi, J. K.; Hilinski, E. F.; Rentzepis, P. M. J. Am. Chem. Soc. 1986, 108, 1126.
    • (1984) Chem. Phys. Lett. , vol.106 , pp. 20
    • Masnovi, J.M.1    Huffman, J.C.2    Kochi, J.K.3    Hilinski, E.F.4    Rentzepis, P.M.5
  • 47
    • 0004190075 scopus 로고
    • Organometallic Mechanisms and Catalysis
    • Academic: New York Part 3, and references cited therein.
    • Kochi, J. K. Organometallic Mechanisms and Catalysis; Academic: New York, 1978; Part 3, and references cited therein.
    • (1978)
    • Kochi, J.K.1
  • 49
    • 0000199048 scopus 로고
    • (b) Hilinski, E. F.; Masnovi, J. M.; Kochi, J. K.; Rentzepis, P. M. J. Am. Chem. Soc. 1984, 106, 8071.
    • Hilinski, E. F.; Masnovi, J. M.; Amatore, C. Kochi, J. K.; Rentzepis, P. M. J. Am. Chem. Soc. 1983, 105, 6167. (b) Hilinski, E. F.; Masnovi, J. M.; Kochi, J. K.; Rentzepis, P. M. J. Am. Chem. Soc. 1984, 106, 8071.
    • (1983) J. Am. Chem. Soc. , vol.105 , pp. 6167
    • Hilinski, E.F.1    Masnovi, J.M.2    Amatore, C.3    Kochi, J.K.4    Rentzepis, P.M.5
  • 50
    • 0003975627 scopus 로고
    • Mixed Valence Compounds
    • Review on heteropoly blues Brown, D. B., Ed.; D. Reidel: Boston (b) Papaconstantinou, E.; Hoffman, M. Z. Inorg. Chem. 1982, 21, 2087. (c) Flynn, G. M.; Pope, M. T. Inorg. Chem. 1973, 12, 1626. (d) Fruchart, J. M.; Herve, G.; Launay, J. P.; Massart, R. J. Inorg. Nucl. Chem. 1976, 38, 1627. (e) Papaconstantinou, E.; Pope, M. T. Inorg. Chem. 1970, 9, 667.
    • Review on heteropoly blues: Pope, M. T. In Mixed Valence Compounds; Brown, D. B., Ed.; D. Reidel: Boston, 1980; pp 365–386. (b) Papaconstantinou, E.; Hoffman, M. Z. Inorg. Chem. 1982, 21, 2087. (c) Flynn, G. M.; Pope, M. T. Inorg. Chem. 1973, 12, 1626. (d) Fruchart, J. M.; Herve, G.; Launay, J. P.; Massart, R. J. Inorg. Nucl. Chem. 1976, 38, 1627. (e) Papaconstantinou, E.; Pope, M. T. Inorg. Chem. 1970, 9, 667.
    • (1980) , pp. 365-386
    • Pope, M.T.1


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.