Characterization of water-soluble organic matter isolated from atmospheric fine aerosol

Journal of Geophysical Research Atmospheres

Volumn 107, Issue 21, 2002, Pages

  Kiss, Gyula ^a   Varga, Bálint ^b   Galambos, István ^b   Ganszky, Ildikó ^b  

^a INSTITUTE OF EXPERIMENTAL MEDICINE   (Hungary)

^b UNIVERSITY OF PANNONIA   (Hungary)

Author keywords

Atmospheric aerosol; Elemental composition; Mass conversion factor; Water soluble organic compounds

Indexed keywords

ATMOSPHERIC AEROSOLS; ATMOSPHERIC CHEMISTRY; CLIMATE CHANGE; COMPOSITION; CONCENTRATION (PROCESS); COPOLYMERS; SOLUBILITY;

AEROSOL; AIR SAMPLING; HYDROGEN; ORGANIC CARBON; ORGANIC MATTER; RURAL ATMOSPHERE;

CENTRAL EUROPE; EURASIA; EUROPE; HUNGARY;

EID: 33751267974     PISSN: 01480227     EISSN: None     Source Type: Journal    
DOI: 10.1029/2001JD000603     Document Type: Article

References (33)

1. Artaxo, P., and H.-C. Hansson, Size distribution of biogenic aerosol particles from the Amazon basin, Atmos. Environ., 29, 393-402, 1995.
2. Artaxo, P., W. Maenhaut, H. Storms, and R. Van Grieken, Aerosol characteristics and sources for the Amazon basin during the wet season, J. Geophys. Res., 95, 16,971-16,985, 1990.
3. Decesari, S., M. C. Facchini, S. Fuzzi, and E. Tagliavini, Characterization of water-soluble organic compounds in atmospheric aerosol: A new approach, J. Geophys. Res., 105, 1481-1489, 2000.
4. Ellis, E. C., T. Novakov, and M. D. Zeldin, Thermal characterization of organic aerosols, Sci. Total Environ., 36, 261-270, 1984.
5. Facchini, M. C., et al., Partitioning of the organic aerosol component between fog droplets and interstitial air, J. Geophys. Res., 104, 26,821-26,832, 1999.
6. Gelencsér, A., A. Hoffer, A. Molnár, Z. Krivácsy, G. Kiss, and E. Mészáros, Thermal behaviour of carbonaceous aerosol from a continental background site, Atmos. Environ., 34, 823-831, 2000a.
7. Gelencsér, A., M. Sallai, Z. Krivácsy, G. Kiss, and E. Mészáros, Voltammetric evidence for the presence of humic-like substances in fog water, Atmos. Res., 54, 157-165, 2000b.
8. Gelencsér, A., T. Mészáros, M. Blazsó, G. Kiss, Z. Krivácsy, A. Molnár, and E. Mészáros, Structural characterisation of organic matter in fine tropospheric aerosol by pyrolysis-gas chromatography-mass spectrometry, J. Atmos. Chem., 37, 173-183, 2000c.
9. Gelencsér, A., A. Hoffer, Z. Krivácsy, G. Kiss, A. Molnar, and E. Mészáros, On the possible origin of humic matter in fine continental aerosol, J. Geophys. Res., 107(D21), 4137, doi:10.1029/2001JD001299, 2002.
10. Graham, B., O. L. Mayol-Bracero, P. Guyon, G. C. Roberts, S. Decesari, M. C. Facchini, P. Artaxo, W. Maenhaut, P. Köll, and M. O. Andreae, Water-soluble organic compounds in Biomass burning aerosols over Amazonia, 1, Characterization by NMR and GC/MS, J. Geophys. Res., 107(D20), 8047, doi:10.1029/2001JD000336, 2002.
11. Gray, H. A., G. R. Cass, J. J. Huntzicker, E. K. Heyerdahl, and J. A. Rau, Characteristics of atmospheric organic and elemental carbon particle concentration in Los Angeles, Environ. Sci. Technol., 20, 580-589, 1986.
12. Havers, N., P. Burba, J. Lambert, and D. Klockow, Spectroscopic characterization of humic-like substances in airborne particulate matter, J. Atmos. Chem., 29, 45-54, 1998a.
13. Havers, N., P. Burba, D. Klockow, and A. Klockow-Beck, Characterization of humic-like substances in airborne particulate matter by capillary electrophoresis, Chromatographia, 47, 619-624, 1998b.
14. Heintzenberg, J., Fine particles in the global troposphere: A review, Tellus, 41B, 149-160, 1989.
15. Hlavay, J., K. Polyák, I. Bódog, A. Molnár, and E. Mészáros, Distribution of trace elements in filler-collected aerosol samples, Fresenius J. Anal. Chem., 354, 227-232, 1996.
16. Kiss, G., B. Varga, A. Gelencsér, Z. Krivácsy, Á. Molnár, T. Alsberg, L. Persson, H.-C. Hansson, and M. C. Facchini, Characterisation of polar organic compounds in fog water, Atmos. Environ., 35, 2193-2200, 2001.
17. Krivácsy, Z., et al., Study of humic-like substances in fog and interstitial aerosol by size-exclusion chromatography and capillary electrophoresis, Atmos. Environ., 34, 4273-4281, 2000.
18. Krivácsy, Z., et al., Study on the chemical character of water soluble organic compounds in fine atmospheric aerosol at the Jungfraujoch, J. Atmos. Chem., 39, 235-259, 2001.
19. Kunit, M., and H. Puxbaum, Enzymatic determination of the cellulose content of atmospheric aerosols, Atmos. Environ., 30, 1233-1236, 1996.
20. Mayol-Bracero, O. L., P. Guyon, B. Graham, G. Roberts, M. O. Andreae, S. Decesari, M. C Facchini, S. Fuzzi, and P. Artaxo, Water-soluble organic compounds in biomass burning aerosols over Amazonia, 2, Apportionment of the chemical composition and importance of the polyacidic fraction, J. Geophys. Res., 10.1029/2001JD000522, in press, 2002.
21. Molnár, A., E. Mészáros, K. Polyák, I. Borbély-Kiss, E. Koltay, G. Szabó, and Z. Horváth, Atmospheric budget of different elements in aerosol particles over Hungary, Atmos. Environ., 29, 1821-1828, 1995.
22. Molnár, A., E. Mészáros, H.-C. Hansson, H. Karlsson, A. Gelencsér, G. Kiss, and Z. Krivácsy, The importance of organic and elemental carbon in the fine atmospheric aerosol particles, Atmos. Environ., 33, 2745-2750, 1999.
23. Penner, J. E., C. C. Chuang, and C. Liousse, The contribution of carbonaceous aerosols to climate change, in Proceedings of the Fourteenth International Conference on Nucleation and Atmospheric Aerosols, pp. 759-769, Elsevier, New York, 1996.
24. Pettersson, C., J. Ephraim, and B. Allard, On the composition and properties of humic substances isolated from deep groundwaters and surface waters, Org. Geochem., 21, 443-451, 1994.
25. Puxbaum, H., Application of two thermo-gas analyzers for atmospheric aerosol characterization, Int. J. Environ. Anal. Chem., 10, 1-6, 1981.
26. Rogge, W. F., M. A. Mazurek, L. M. Hildemann, and G. R. Cass, Quantification of urban organic aerosols at a molecular level: Identification, abundance and seasonal variation, Atmos. Environ., 27A, 1309-1330, 1993.
27. Saxena, P., and L. Hildemann, Water-soluble organics in atmospheric particles: A critical review of the literature and application of thermodynamics to identify candidate compounds, J. Atmos. Chem., 24, 57-109, 1996.
28. Sempere, R., and K. Kawamura, Comparative distributions of dicarboxylic acids and related polar compounds in snow, rain and aerosols from urban atmosphere, Atmos. Environ., 28, 449-459, 1994.
29. Simoneit, B. R. T., J. J. Schauer, C. G. Nolte, D. R. Oros, V. O. Elias, M. P. Fraser, W. F. Rogge, and G. R. Cass, Levoglucosan, a tracer for cellulose in biomass burning and atmospheric particles, Atmos. Environ., 33, 173-182, 1999.
30. Turpin, B. J., J. J. Huntzicker, and S. V. Hering, Investigation of organic aerosol sampling artifacts in the Los Angeles basin, Atmos. Environ., 28, 3061-3071, 1994.
31. Turpin, B. J., P. Saxena, and E. Andrews, Measuring and simulating particulate organics in the atmosphere: Problems and prospects, Atmos. Environ., 34, 2983-3013, 2000.
32. Varga, B., G. Kiss, I. Ganszky, A. Gelencsér, and Z. Krivácsy, Isolation of water-soluble organic matter from atmospheric aerosol, Talanta, 55(3), 561-572, 2001.
33. Zappoli, S., et al., Inorganic, organic and macromolecular components of fine aerosol in different areas of Europe in relation to their water solubility, Atmos. Environ., 33, 2733-2743, 1999.