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33750427707
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note
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Note that in a recent work Win and Menon (preprint cond-mat/ 0508648) claim that the dynamics in glycerol are quantitatively more sensitive to fractional changes in density (volume) than temperature. This finding, which seems completely orthogonal to what found earlier [2,8], is due to the fact that the authors do not properly evaluate the relative contributions of density and temperature effects along an isobar. As a result they miss a large effect due to the isobaric coefficient of expansivity.
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8
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0037426222
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Paluch M., Roland C.M., Casalini R., Meier G., and Patkowski A. J. Chem. Phys 118 (2003) 4578
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Tokuyama M., and Oppenheim I. (Eds), ACS Books, Washington, DC
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Tarjus G., Alba-Simionesco C., Ferrer M.L., Sakai H., and Kivelson D. In: Tokuyama M., and Oppenheim I. (Eds). Slow Dynamics in Complex Systems (1999), ACS Books, Washington, DC 406
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Tarjus, G.1
Alba-Simionesco, C.2
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4043147409
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Dreyfus C., Aouadi A., Gapinski G., Matos-Lopez M., Steffen W., Patkowski A., and Pick R.M. Phys. Rev. E 68 (2003) 011204
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Papadopoulos P., Peristeraki D., Floudas G., Koutalas G., and Hadjichristidis N. Macromolecules 37 (2004) 8116
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33750490637
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note
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P decreases as one approaches the glass transition whether along an isobar or an isotherm.
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15
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A. Chauty-Cailliau, PhD thesis, Université de Paris-Sud, 11 July, 2003.
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33750432708
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note
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τ{divides}, exceptionally high at the glass transition, behaves in the opposite direction over the first hundreds of MPa, and tends to increases along an isochrone as T increases [8]; the isobaric fragility behaves accordingly. This could be related to the strength of the H-bond network, whose contribution decreases as T increases.
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25
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58149319544
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Kivelson D., Kivelson S.A., Zhao X.-L., Nussinov Z., and Tarjus G. Physica A 219 (1995) 27
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33750451806
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note
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∞(ρ) is small for the binary Lennard-Jones model, large for the H-bonded liquid Glycerol and intermediate for the organic liquid o-terphenyl (see Refs. [3,12]).
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