Radionuclide migration at the Koongarra uranium deposit, Northern Australia - Lessons from the Alligator Rivers analogue project

Physics and Chemistry of the Earth

Volumn 31, Issue 10-14, 2006, Pages 572-586

  Payne, Timothy E ^a   Airey, Peter L ^a  

^a AUSTRALIAN NUCLEAR SCIENCE AND TECHNOLOGY ORGANISATION   (Australia)

Author keywords

Koongarra; Natural analogue; Radionuclide transport; Repository; Sorption; Uranium

Indexed keywords

CHARACTERIZATION; GEOCHEMISTRY; GEOLOGICAL REPOSITORIES; GEOLOGY; HYDROLOGY; RADIOACTIVE WASTE DISPOSAL; SORPTION; URANIUM DEPOSITS;

NATURAL ANALOGUE; RADIONUCLIDE MIGRATION;

RADIOISOTOPES;

GROUNDWATER POLLUTION; RADIOACTIVE WASTE; RADIONUCLIDE MIGRATION; URANIUM; WASTE DISPOSAL;

AUSTRALASIA; AUSTRALIA; KOONGARRA; NORTHERN TERRITORY;

ALLIGATOR;

EID: 33746341471     PISSN: 14747065     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.pce.2006.04.008     Document Type: Article

References (81)

1. Airey P.L. Radionuclide migration around uranium ore bodies in the Alligator Rivers Region of the Northern Territory of Australia - analogue of radioactive waste repositories - a review. Chem. Geol. 55 (1986) 255-268
2. Banfield J.F., and Murakami T. Atomic-resolution transmission electron microscope evidence for the mechanism by which chlorite weathers to 1:1 semi-regular chlorite-vermiculite. Am. Mineral. 83 (1998) 348-357
3. Birchard G.F. International Alligator Rivers Analogue Project. Radioact. Waste Manag. Nuc. Fuel Cycle 13 (1989) 325-337
4. Birgersson, L., Larsson, A., Skagius, K., 1996. The International INTRAVAL Project, Phase 2. The Analyses of the Alligator Rivers Natural Analogue. OECD Nuclear Energy Agency.
5. Borovec Z. The adsorption of uranyl species by fine clay. Chem. Geol. 32 (1981) 45-58
6. Bottomley D.J. The Geochemical Immobilisation of Uranium in a Spent Fuel Repository in the Canadian Shield: Evidence from Natural Analogue Investigations (1996), Atomic Energy Control Board, Canada
7. Buddemeier R.W., and Hunt J.R. Transport of colloidal contaminants in groundwater: radionuclide migration at the Nevada Test Site. Appl. Geochem. 3 (1988) 535-548
8. Cruikshank B.I., and Pyke J.G. Biogeochemistry and soil geochemistry of the Ranger One, number 3 orebody, Australia. Uranium 3 (1986) 1-26
9. Curtis D.B., Fabryka-Martin J., Dixon P., Aguilar R., Rokop D., and Cramer J. Radionuclide release rates from natural analogues of spent nuclear fuel. Radiochim. Acta 66/67 (1994) 551-557
10. Curtis D., Fabryka-Martin J., Dixon P., and Cramer J. Nature's uncommon elements: plutonium and technetium. Geochim. Cosmochim. Acta 63 (1999) 275-285
11. Davis, J.A., 2001. Surface complexation modeling of uranium(VI) adsorption on natural mineral assemblages. Report NUREG/CR-6708. United States Nuclear Regulatory Commission, Washington, 214pp.
12. Davis J.A., and Kent D.B. Surface complexation modeling in aqueous geochemistry. In: Hochella M.F., and White A.F. (Eds). Mineral-Water Interface Geochemistry. Rev. Mineral. vol. 23 (1990), Mineralogical Society of America, Washington 177-260
13. 2 dependence of uranium(VI) adsorption by a weathered schist with surface complexation models. In: Zhang P.C., and Brady P.V. (Eds). Geochemistry of Soil Radionuclides (2002), Soil Science Society of America, Madison 61-86
14. Dodson, R.G., Needham, R.S., Wilkes, P.G., Page, R.W., Smart, P.G., Watchman, A.L., 1974. Uranium mineralization in the Rum Jungle - Alligator Rivers Province, Northern Territory, Australia. In: Formation of Uranium Ore Deposits. IAEA, Vienna, pp. 551-567.
15. Duerden, P., 1992a. The Alligator Rivers analogue project - Characterisation of the development of the uranium dispersion fan. In: C.G. Sombret (Ed.), Scientific Basis for Nuclear Waste Management XV. Materials Research Society Symposium Proceedings, vol. 257, pp. 529-536.
16. Duerden, P., 1992b. The International Intraval Project, Phase 1. Test Case 2: The Alligator Rivers Natural Analogue. OECD Nuclear Energy Agency.
17. Duerden, P., Lever, D.A., Sverjensky, D.A., Townley, L.R., 1992. Summary of Findings. Alligator Rivers Analogue Project, Final Report, vol. 1, Australian Nuclear Science and Technology Organisation.
18. Duerden P., and Airey P.L. ARAP - the International Alligator Rivers Analogue Project - Background and Results (1994), OECD Nuclear Energy Agency, Paris 33pp
19. Edghill R. The redistribution of uranium with weathering in the Koongarra uranium deposit. Radiochim. Acta 52/53 (1991) 381-386
20. Edis, R, Cao, L., Cashion, J., Klessa, D., Koppi, A.J., Murakami, T, Nightingale, T., Payne, T.E., Snelling, A., Yanase, N., 1992. Chemistry and Mineralogy of Rocks and Soil. Alligator Rivers Analogue Project, Final Report, Vol. 8, Australian Nuclear Science and Technology Organisation.
21. El-Ghonemy H., Watts L., and Fowler L. Treatment of uncertainty and developing conceptual models for environmental risk assessments and radioactive waste disposal safety cases. Environ. Int. 31 (2005) 89-97
22. Emerson, D.W., Mills, K.J., Miyakawa, K., Hallett, M.S. Cao, L.Q., 1992. Geophysics, Petrophysics and Structure. Alligator Rivers Analogue Project, Final Report, vol. 4, Australian Nuclear Science and Technology Organisation.
23. Emerson D.W., Mills K.J., Miyakawa K., Hallett M.S., and Cao L.Q. The petrophysics, geophysics and structure of the Koongarra site, Northern Territory. Exploration Geophysics 24 (1993) 1-71
24. 36Cl. Alligator Rivers Analogue Project, Final Report, vol. 15, Australian Nuclear Science and Technology Organisation.
25. Fabryka-Martin J., Davis S.N., Roman D., Airey P.L., Elmore D., and Kubik P.W. Iodine-129 and chlorine-36 in uranium ores 2. Discussion of AMS measurements. Chem. Geol. (Isotope Geoscience Section) 72 (1988) 7-16
26. Fenton B.R., and Waite T.D. A kinetic study of cation release from a mixed mineral assemblage: implications for determination of uranium uptake. Radiochim. Acta 74 (1996) 251-256
27. Galson D.A., Swift P.N., Anderson D.R., Bennett D.G., Crawford M.B., Hicks T.W., Wilmot R.D., and Basabilvazo G. Scenario development for the waste isolation pilot plant compliance certification application. Reliab. Eng. Syst. Safe. 69 (2000) 129-149
28. Giblin A.M. The role of clay adsorption in genesis of uranium ores. In: Ferguson J., and Goleby A.B. (Eds). Uranium in the Pine Creek Geosyncline (1980), IAEA, Vienna 521-529
29. Golian, C., Lever, D.A., 1992. Radionuclide transport. Alligator Rivers Analogue Project, Final Report, Vol. 14, Australian Nuclear Science and Technology Organisation.
30. Golian C., Nightingale T., and Airey P.L. Protactinium-231 measurement and application to a uranium series transport model. Nucl. Instrum. Methods 223 (1984) 577-581
31. Herczeg, A.L., Payne, T.E., 1992. Recharge and weathering processes in fractured rock aquifers in Northern Australia. In: Kharaka, Y., Maest, A.E. (Eds.), 7th International Conference on Water Rock Interaction, International Association for Geochemistry and Cosmochemistry. Balkema, Rotterdam, pp. 561-564.
32. Horie K., and Hidaka H. Redistribution of U, Pb and REE in association with alteration of uranium minerals from the Koongarra deposit, Northern Territory, Australia. Radiochim. Acta 92 (2004) 805-808
33. Hsi C.-K.D., and Langmuir D. Adsorption of uranyl onto ferric oxyhydroxides: application of the surface complexation site-binding model. Geochim. Cosmochim. Acta 49 (1985) 1931-1941
34. Isobe H., Murakami T., and Ewing R.C. Alteration of uranium minerals in the Koongarra deposit, Australia: unweathered zone. J. Nucl. Mater. 190 (1992) 174-187
35. 2 + on natural composite minerals. J. Radioanal. Nucl. Ch. 242 (1999) 405-412
36. Keum D.K., and Hahn P.S. A coupled reactive chemical transport model: mixing cell model with two solid phases and its application. Comput. Geosci. 29 (2003) 431-445
37. Komninou A., and Sverjensky D.A. Pre-ore hydrothermal alteration in an unconformity-type uranium deposit. Contrib. Mineral. Petr. 121 (1995) 99-114
38. Komninou A., and Sverjensky D.A. Hydrothermal alteration and the chemistry of ore-forming fluids in an unconformity-type uranium deposit. Geochim. Cosmochim. Acta 59 (1995) 2709-2723
39. Koppi A.J., Edis R., Field D.J., Geering H.R., Klessa D.A., and Cockayne D.J.H. Rare earth element trends and cerium-uranium-manganese associations in weathered rock from Koongarra, Northern Territory, Australia. Geochim. Cosmochim. Acta 60 (1996) 1695-1707
40. Leijnse A., van de Weerd H., and Hassanizadeh S.M. Modeling uranium transport in Koongarra, Australia: the effect of a moving weathering zone. Math. Geol. 33 (2001) 1-29
41. 234U activity ratios in mineral phases of a lateritic weathered zone. Geochim. Cosmochim. Acta 50 (1986) 1697-1702
42. Miller W., Alexander R., Chapman N., McKinley I., and Smellie J. Natural Analogue Studies in the Geological Disposal of Radioactive Wastes. Studies in Environmental Science vol. 57 (1994), Elsevier, Amsterdam
43. Murakami T., Isobe H., Sato T., and Ohnuki T. Weathering of chlorite in a quartz-chlorite schist: I. Mineralogical and chemical changes. Clay Clay Miner. 44 (1996) 244-256
44. Murakami T., Ohnuki T., Isobe H., and Sato T. Mobility of uranium during weathering. Am. Mineral. 82 (1997) 888-899
45. Murakami T., Sato T., Ohnuki T., and Isobe H. Field evidence for uranium nanocrystallization and its implications for uranium transport. Chem. Geol. 221 (2005) 117-126
46. Nagano T., Sato T., Williams I.S., Zaw M., Payne T.E., Airey P.L., Yanase N., Isobe H., and Ohnuki T. SHRIMP measurements of U and Pb isotopes in the Koongarra secondary ore deposit, Northern Australia. Geochem. J. 34 (2000) 349-358
47. Ohnuki T., Isobe H., Yanase N., Nagano T., Sakamoto Y., and Sekine K. Change in sorption characteristics of uranium during crystallization of amorphous iron minerals. J. Nucl. Sci. Technol. 34 (1997) 1153-1158
48. Ohnuki T., Kozai N., Samadfam M., Yasuda R., Kamiya T., Sakai T., and Murakami T. Analysis of uranium distribution in rocks by μ-PIXE. Nucl. Instrum. Meth. B 181 (2001) 586-592
49. Payne T.E., and Waite T.D. Surface complexation modelling of uranium sorption data obtained by isotope exchange techniques. Radiochim. Acta 52/53 (1991) 487-493
50. Payne, T.E., Edis, R., Herczeg, A.L., Seo, T., Waite, T.D., Yanase, N., 1992a. Groundwater Chemistry. Alligator Rivers Analogue Project, Final Report, vol. 7, Australian Nuclear Science and Technology Organisation.
51. Payne, T.E., Edis, R., Seo, T., 1992b. Radionuclide transport by groundwater colloids at the Koongarra uranium deposit. In: C.G. Sombret (Ed.), Scientific Basis for Nuclear Waste Management XV. Materials Research Society Symposium Proceedings, vol. 257, pp. 481-488.
52. Payne T.E., Davis J.A., and Waite T.D. Uranium retention by weathered schists - the role of iron minerals. Radiochim. Acta 66/67 (1994) 297-303
53. Payne T.E., Davis J.A., and Waite T.D. Uranium adsorption on ferrihydrite - effects of phosphate and humic acid. Radiochim. Acta 74 (1996) 239-243
54. VI adsorption on model minerals: controlling factors and surface complexation modeling. In: Jenne E.A. (Ed). Adsorption of Metals by Geomedia: Variables, Mechanisms and Models (1998), Academic Press, San Diego 75-97
55. Payne T.E., Edis R., Fenton B.R., and Waite T.D. Comparison of laboratory uranium sorption data with 'in-situ distribution coefficients' at the Koongarra uranium deposit, Northern Australia. J. Environ. Radioactiv. 57 (2001) 35-55
56. Payne T.E., Davis J.A., Lumpkin G.R., Chisari R., and Waite T.D. Surface complexation model of uranyl sorption on Georgia kaolinite. Appl. Clay Sci. 26 (2004) 151-162
57. Payne T.E., Davis J.A., Ochs M., Olin M., and Tweed C.J. Uranium adsorption on weathered schist - intercomparison of modelling approaches. Radiochim. Acta 92 (2004) 651-661
58. Sato T., Murakami T., Yanase N., Isobe H., Payne T.E., and Airey P.L. Iron nodules scavenging uranium from groundwater. Environ. Sci. Technol. 31 (1997) 2854-2858
59. Sato T., Yanase N., Williams I.S., Compston W., Zaw M., Payne T.E., and Airey P.L. Uranium micro-isotopic analysis of weathered rock by a sensitive high resolution ion microprobe (SHRIMP II). Radiochim. Acta 82 (1998) 335-340
60. 238U activity ratios in clay as a function of distance from primary ore. In: International Uranium Symposium on the Pine Creek Geosyncline. IAEA, Vienna, pp. 509-519.
61. 238U decay series in the vicinity of mineralised zones: 1. The Austatom Uranium Prospect, Northern Territory, Australia. Geochim. Cosmochim. Acta 47 (1983) 403-412
62. 234U activity ratios in the colloidal phases of aquifers in lateritic weathered zones. Geochim. Cosmochim. Acta 52 (1988) 2555-2563
63. Skagius, K., Wingefors, S., 1992. Application of Scenario Development Methods in Evaluation of the Koongarra Analogue. Alligator Rivers Analogue Project, Final Report, vol. 16, Australian Nuclear Science and Technology Organisation.
64. Skagius K., Wiborgh M., Strom A., and Morén L. Performance assessment of the geosphere barrier of a deep geological repository for spent fuel. The use of interaction matrices for identification, structuring and ranking of features, events and processes. Nucl. Eng. Des. 176 (1997) 155-162
65. Smellie J.A.T., and Karlsson F. The use of natural analogues to assess radionuclide transport. Eng. Geol. 52 (1999) 193-220
66. Snell, R.D., 2000. Saturated Zone Flow and Transport Process Model Report. Report TDR-NBS-HS-000001 Rev 00 ICN 02. US Department of Energy, Las Vegas.
67. Snelling, A.A., 1980. Uraninite and its alteration products, Koongarra uranium deposit. In: International Uranium Symposium on the Pine Creek Geosyncline. IAEA, Vienna, pp. 487-498.
68. Snelling A.A. Koongarra uranium deposits. In: Hughes F.E. (Ed). Geology of the Mineral Deposits of Australia and Papua New Guinea (1990), Australian Institute of Mining and Metallurgy 807-812
69. Snelling, A.A., 1992. Geologic Setting. Alligator Rivers Analogue Project, Final Report, vol. 2, Australian Nuclear Science and Technology Organisation.
70. Snelling A.A., and Dickson B.L. Uranium/daughter disequilibrium in the Koongarra uranium deposit Australia. Miner. Deposita 14 (1979) 109-118
71. Sverjensky, D.A., 1992. Geochemical modelling of present-day groundwaters. Alligator Rivers Analogue Project, Final Report, vol. 12, Australian Nuclear Science and Technology Organisation.
72. 234U in spring waters, sediments and fossils at the Pomme de Terre Valley, southwestern Missouri. Geochim. Cosmochim. Acta 46 (1982) 1675-1679
73. Townley, L.R., Barr, A.D., Braumiller, S., Kawanishi, M., Lever, D.A., Miyakawa, K., Morris, S.T., Raffensperger, J.P., Smoot, J.L., Tanaka, Y., Trefry, M.G., 1992. Hydrogeological Modelling. Alligator Rivers Analogue Project, Final Report, vol. 6, Australian Nuclear Science and Technology Organisation.
74. Waite T.D., Davis J.A., Payne T.E., Waychunas G.A., and Xu N. Uranium(VI) adsorption to ferrihydrite: application of a surface complexation model. Geochim. Cosmochim. Acta 58 (1994) 5465-5478
75. Waite T.D., Davis J.A., Fenton B.R., and Payne T.E. Approaches to modelling uranium(VI) adsorption on natural mineral assemblages. Radiochim. Acta 88 (2000) 687-693
76. Watters R.A. Biogeochemistry and soil geochemistry of the Ranger One, number 3 orebody, Australia - comments. Uranium 4 (1988) 415-418
77. Wyrwoll, K.H., 1992. Geomorphology and Paleoclimatic History. Alligator Rivers Analogue Project, Final Report, vol. 3, Australian Nuclear Science and Technology Organisation.
78. Yanase N., Nightingale T., Payne T., and Duerden P. Uranium distribution in mineral phases of rock by sequential extraction procedure. Radiochim. Acta 52/53 (1991) 387-393
79. Yanase N., Payne T.E., and Sekine K. Groundwater geochemistry in the Koongarra ore deposit, Australia (I): implications for uranium migration. Geochem. J. 29 (1995) 1-29
80. Yanase N., Payne T.E., and Sekine K. Groundwater geochemistry in the Koongarra ore deposit, Australia (II): activity ratios and migration mechanisms of uranium series radionuclides. Geochem. J. 29 (1995) 31-54
81. Yanase N., Sato T., Iida Y., and Sekine K. Distributions of uranium-series radionuclides in rock and migration rate of uranium at the Koongarra uranium deposit, Australia. Radiochim. Acta 82 (1998) 319-325