Rotor modulations and recoupling strategies in 13C solid-state magic-angle-spinning NMR spectroscopy: Probing molecular orientation and dynamics

ChemPhysChem

Volumn 5, Issue 6, 2004, Pages 895-908

  Fischbach, Ingrid ^a   Ebert, Florian ^a,b   Spiess, Hans Wolfgang ^a   Schnell, Ingo ^a  

^a MAX PLANCK INSTITUTE FOR POLYMER RESEARCH   (Germany)

^b UNIVERSITY OF KONSTANZ   (Germany)

Author keywords

Liquid crystals; Magic angle spinning; Molecular orientation; Polymers; Solid state NMR spectroscopy

Indexed keywords

ANISOTROPY; CHEMICAL SHIFT; CRYSTAL ORIENTATION; DYNAMICS; LIGHT POLARIZATION; LIQUID CRYSTALS; MOLECULAR ORIENTATION; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; POLYMERS; X RAY SCATTERING;

CHEMICAL SHIFT ANISOTROPY; DIPOLE-DIPOLE COUPLINGS; ORIENTATION DEPENDENCIES; ORIENTATIONAL ORDER PARAMETERS; SELECTIVE DETERMINATION; SITE-SPECIFIC INFORMATION; SOLID STATE MAGIC ANGLE SPINNING NMR; SOLID-STATE NMR SPECTROSCOPY;

MAGIC ANGLE SPINNING;

ANALYTIC METHOD; ANISOTROPY; ARTICLE; CARBON NUCLEAR MAGNETIC RESONANCE; CHEMICAL STRUCTURE; ELECTRON SPIN RESONANCE; MAGIC ANGLE SPINNING NUCLEAR MAGNETIC RESONANCE; MOLECULAR DYNAMICS; MOTION; NUCLEAR MAGNETIC RESONANCE; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; PARAMETER; RADIATION SCATTERING; SENSITIVITY AND SPECIFICITY; SOLID STATE;

EID: 3142685112     PISSN: 14394235     EISSN: None     Source Type: Journal    
DOI: 10.1002/cphc.200301053     Document Type: Article

References (60)

1. Nuclear Magnetic Resonance of Liquid Crystals, NATO ASI Series, C 141, D. Reidel Publishing Company, Dordrecht, 1985.
2. K. Schmidt-Rohr, H. W. Spiess, Multidimensional Solid-State NMR and Polymers, Academic Press, London, 1994.
3. T. Gullion, Magn. Reson. Rev. 1997, 17, 83.
4. A. Brinkmann, M. Eden, M. H. Levitt, J. Chem. Phys. 2000, 112, 8539.
5. T. Gullion, Concepts Magn. Reson. 1998, 10, 277.
6. K. Saalwächter, I. Schnell, Solid State Nucl. Magn. Reson. 2002, 22, 154.
7. S. P. Brown, I. Schnell, J. D. Brand, K. Müllen, H. W. Spiess, J. Am. Chem. Soc. 1999, 121, 6712.
8. E. R. deAzevedo, W.-G. Hu, T. J. Bonagamba, K. Schmidt-Rohr, J. Am. Chem. Soc. 1999, 121, 8411.
9. a) A. Fechtenkötter, K. Saalwächter, M. A. Harbison, K. Müllen, H. W. Spiess, Angew. Chem. 1999, 111, 3224; Angew. Chem. Int. Ed. 1999, 38, 3039.
10. a) A. Fechtenkötter, K. Saalwächter, M. A. Harbison, K. Müllen, H. W. Spiess, Angew. Chem. 1999, 111, 3224; Angew. Chem. Int. Ed. 1999, 38, 3039.
11. S. P. Brown, H. W. Spiess, Chem. Rev. 2001, 101, 4125.
12. A. Rapp, I. Schnell, D. Sebastiani, S. P. Brown, V. Percec, H. W. Spiess, J. Am. Chem. Soc. 2003, 125, 13 284.
13. S. Dusold, A. Sebald, Annu. Rep. NMR Spectrosc. 2000, 41, 185.
14. A. E. Bennett, D. P. Weliky, R. Tycko, J. Am. Chem. Soc. 1998, 120, 4897.
15. J. Schmedt auf der Günne, J. Magn. Reson. 2003, 165, 18.
16. S. M. De Paul, K. Saalwächter, R. Graf, H. W. Spiess, J. Magn. Reson. 2000, 146, 140.
17. R. Hentschel, J. Schlitter, H. Sillescu, H. W. Spiess, J. Chem. Phys. 1978, 68, 56.
18. D. McElheny, J. Grinshstein, V. Frydman, L. Frydman, Macromolecules 2002, 35, 3544.
19. J. J. Titman, S. Feaux de Lacroix, H. W. Spiess, J. Chem. Phys. 1993, 98, 3816.
20. K. Schmidt-Rohr, M. Hehn, D. Schaefer, H. W. Spiess, J. Chem. Phys. 1992, 97, 2247.
21. A. Ramamoorthy, S.J. Opella, Solid State Nucl. Magn. Reson. 1995, 4, 387.
22. J. K. Denny, J. F. Wang, T. A. Cross, J. R. Quine, J. Magn. Reson. 2001, 152, 217.
23. G. S. Harbison, H. W. Spiess, Chem. Phys. Lett. 1986, 124, 128.
24. G. S. Harbison, V.-D. Vogt, H. W. Spiess, J. Chem. Phys. 1987, 86, 1206.
25. A. Hagemeyer, K. Schmidt-Rohr, H. W. Spiess, Adv. Magn. Reson. 1989, 13, 85.
26. J. Cortieu, J. P. Bayle, B. M. Fung, Prog. Nucl. Magn. Reson. Spectrosc. 1994, 26, 141.
27. C. Glaubitz, A. Watts, J. Magn. Reson. 1998, 130, 305.
28. Z. Ahmed, D. Middleton, C, Glaubitz, A. Watts, Biochem. Soc. Trans. 1998, 26, S194.
29. C. Glaubitz, I. J. Burnett, G. Grobner, A. J. Mason, A. Watts, J. Am. Chem. Soc. 1999, 121, 5787.
30. G. Grobner, I. J. Burnett, C. Glaubitz, G. Choi, A. J. Mason, A. Watts, Nature 2000, 405, 810.
31. C. Sizun, B. Bechinger, J. Am. Chem. Soc. 2002, 124, 1146.
32. D. A. Middleton, Z. Ahmed, C. Glaubitz, A. Watts, J. Magn. Reson. 2000, 147, 366.
33. C. Glaubitz, M. Carravetta, M. Eden, M. H. Levitt, in Perspectives on Solid state NMR in Biology (Eds.: S. R. Kühne, H. J. M. deGroot), Kluwer Academic Publishers, Dordrecht, 2001, pp. 71-81.
34. A. Tracz, J. K. Jeszka, M. D. Watson, W. Pisula, K. Müllen, T. Pakula, J. Am. Chem. Soc. 2003, 125, 1682.
35. T. Gullion, J. Schaefer, Adv. Magn. Reson. 1989, 13, 57.
36. T. Gullion, J. Schaefer, J. Magn. Reson. 1989, 81, 196.
37. M. Hong, J. Am. Chem. Soc. 2000, 122, 3762.
38. E. R. deAzevedo, W.-G. Hu, T. J. Bonagamba, K. Schmidt-Rohr, J. Chem. Phys. 2000, 112, 8988.
39. A. W. Hing, S. Vega, J. Schaefer, J. Magn. Reson. 1992, 96, 205.
40. K. Saalwächter, H. W. Spiess, J. Chem. Phys. 2001, 114, 5707.
41. M. Feike, D. E. Demco, R. Graf, J. Gottwald, S. Hafner, H. W. Spiess, J. Magn. Reson. Ser. A 1996, 122, 214.
42. U. Friedrich, I. Schnell, S. P. Brown, A. Lupulescu, D. E. Demco, H. W. Spiess, Mol. Phys. 1998, 95, 1209.
43. I. Fischbach, Ph.D. thesis, University of Mainz, 2004, available online at http://archimed.uni-mainz.de/pub/2004/0009.
44. M. Wind, K. Saalwächter, U.-M. Wiesler, K. Müllen, H. W. Spiess, Macromolecules 2002, 35, 10071.
45. K. Saalwächter, Macromol. Rapid Commun. 2002, 23, 286.
46. S. J. Opella, J. S. Waugh, J. Chem. Phys. 1977, 66, 4919.
47. R. Graf, D. E. Demco, J. Gottwald, S. Hafner, H. W. Spiess, J. Chem. Phys. 1997, 106, 885.
48. I. Schnell, A. Watts, H. W. Spiess, J. Magn. Reson. 2001, 149, 90.
49. K. Schmidt-Rohr, H. W. Spiess, Macromolecules 1991, 24, 5288.
50. C. Zannoni, in The Molecular Dynamics of Liquid Crystals, NATO ASI Series, C 431, Kluwer Academic Publishers, Dordrecht, 1994, pp. 11-36.
51. R. Hentschel, J. Schlitter, H. Sillescu, H. W. Spiess, J. Chem. Phys. 1978, 68, 56.
52. A. M. van de Craats, J. M. Warman, A. Fechtenkötter, J. D. Brand, M. Harbison, K. Müllen, Adv. Mater. 1999, 11, 1469.
53. L. Schmidt-Mende, A. Fechtenkötter, K. Müllen, E. Moons, R. H, Friend, J. D. MacKenzie, Science 2001, 293, 1119.
54. A. M. van de Craats, N. Stutzmann, O. Bunk, M. M. Nielsen, M. Watson, K. Müllen, H. D. Chanzy, H. Sirringhaus, R. H. Friend, Adv. Mater. 2003, 15, 495.
55. The extruder was constructed by Prof. T. Pakula, Max Planck Institute for Polymer Research, Mainz (Germany).
56. I. Fischbach, K. Saalwächter, T. Pakula, P. Minkin, A. Fechtenkötter, K. Müllen, H. W. Spiess, J. Phys. Chem. B 2002, 106, 6408.
57. F. Ebert, T. Thurn-Albrecht, Macromolecules 2003, 36, 8685.
58. J. Gauss, C. Ochsenfeld, unpublished results.
59. A. E. Bennett, C. M. Rienstra, M. Auger, K. V. Lakshmi, R. G. Griffin, J. Chem. Phys. 1995, 103, 6951.
60. G. Metz, X. Wu, S. O. Smith, J. Magn. Reson. Ser. A 1994, 110, 219.