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-1) of the title complex was placed in a 2-mm quartz cuvette for Z-scan measurements. The nonlinear refraction and nonlinear absorption were measured by the Z-scan techniques with linearly polarized 8 ns pulses at 532 nm generated from a Q-switched frequency-doubled Nd:YAG laser. The spatial profiles of the optical pulses were nearly Gaussian. The laser beam was focused onto the sample cell with a 30 cm focal-length mirror. The repetition rate of the laser pulse was 1 Hz. The energies of the input and out pulses were measured simultaneously by a Laser Precision detector (Rjp-735 energy probe) that were linked to a computer by an IEEE interface, while the incident pulse energy was varied by a Newport Co. attenuator. The NLO properties of the samples were manifested by moving the samples along the axis of the incident beam (Z direction) with respect to the focal point. An aperture of 2 mm radius was placed in front of the detector to assist the measurement of self-focusing effect (closed aperture measurement).
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