Deuteron NMR spectra of ammonium ion isotopomers at low temperatures

Solid State Nuclear Magnetic Resonance

Volumn 28, Issue 2-4, 2005, Pages 142-159

  Birczynski A ^a   Lalowicz, Z T ^a   Olejniczak, Z ^a   Stoch, G ^a,b   Petelenz, B ^a  

^a INSTITUTE OF NUCLEAR PHYSICS   (Poland)

^b UNIVERSITY OF NEW BRUNSWICK   (Canada)

Author keywords

Ammonium compounds; Ammonium ion isotopomers; Coherent tunnelling; Deuteron NMR; Incoherent tunnelling; Molecular dynamics

Indexed keywords

MOLECULAR DYNAMICS; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; PROTONS;

AMMONIUM ION ISOTOPOMERS; COHERENT TUNNELING; DEUTERON NMR;

AMMONIUM COMPOUNDS;

EID: 29144498205     PISSN: 09262040     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.ssnmr.2005.07.003     Document Type: Article

References (41)

1. W. Press Single-Particle Rotations in Molecular Crystals Springer Tracts in Modern Physics vol. 92 1981 Springer Berlin
2. A. Birczyński, Z.T. Lalowicz, and Z. Łodziana Rotational barriers in ammonium hexachlorometallates as studied by NMR, tunnelling spectroscopy and ab initio calculations Chem. Phys. 299 2004 113 122
3. M. Prager, and A. Heidemann Rotational tunneling and neutron spectroscopy: a compilation Chem. Rev. 97 1997 2933 2966
4. 2H-NMR spectroscopy of tunneling ammonium ion: general site symmetry Z. Naturforsch. 43a 1988 895 907
5. 2H-NMR spectra of polycrystalline (ND 4 ) 2 SnCl 6, J. Chem. Phys. 88 (1988) 58-67.
6. H.G. Büttner, G.J. Kearley, and B. Frick Tunnelling of the one-dimensional rotor NH 3 D + in the NH 4 ClO 4 and NH 4 PF 6 lattices Chem. Phys. 214 1997 425 429
7. M. Prager, and W. Press Rotational tunneling in NH 4 ClO 4 : reanalysis of neutron spectra J. Chem. Phys. 75 1981 494 495
8. E.E. Ylinen, P. Filipek, M. Punkkinen, and Z.T. Lalowicz NH 3 D + dominated proton spin-lattice relaxation in partly deuterated ammonium compounds Physica B 357 2005 456 471
9. Z.T. Lalowicz, M. Johnson, ILL Experimental Report No 7-07-46, 1997.
10. M. Prager, P. Schiebel, M. Johnson, H. Grimm, H. Hagdorn, J. Ihringer, W. Prandl, and Z.T. Lalowicz The isotope effect and phase transitions in ammonium hexachloropalladate studied by neutron tunnelling spectroscopy J. Phys.: Condens. Matter 11 1999 5483 5495
11. M. Prager, P. Schiebel, H. Grimm, Dipolar interaction in (NH 3.6 D 0.4 ) 2 PtCl 6, Appl. Phys. A 74 (Suppl.) (2002) S1363-S1365.
12. M. Prager, P. Schiebel, and H. Grimm Rotational tunneling of NH 4 and NH 3 D and dipolar interaction in (NH 3.6 D 0.4 ) 2 PtCl 6 J. Chem. Phys. 116 2002 10338 10342
13. T. Schmidt, H. Schmitt, H. Zimmermann, U. Haeberlen, Z.T. Lalowicz, Z. Olejniczak, and T. Oeser Location of the H atoms in ammonium persulphate by deuteron NMR. Verification by X-ray diffraction Acta Crystallogr. B 58 2002 760 769
14. A. Birczyński, Z.T. Lalowicz, and Z. Olejniczak Deuteron NMR spectra of NH 3 D + ions Appl. Magn. Reson. 27 2004 171 181
15. Y. Kume, Y. Miyazaki, T. Matsuo, H. Suga, W.I.F. David, and R.M. Ibberson A strong isotope effect in the low-temperature property of ammonium hexachlorotellurate Europhys. Lett. 16 1991 265 270
16. Y. Kume, H. Muraoka, T. Matsuo, and H. Suga Low-temperature heat capacities of ammonium hexachloroselenate and of its deuterated analogue J. Chem. Thermodyn. 26 1994 211 222
17. Y. Kume, H. Muraoka, O. Yamamuro, and T. Matsuo Deuteron-induced phase transition in ammonium hexachloroplumbate J. Chem. Phys. 108 1998 4090 4097
18. Z.T. Lalowicz, M. Punkkinen, Z. Olejniczak, A. Birczyński, and U. Haeberlen Deuteron NMR study of the diverse mobility of the ammonium ions in the ordered phase of (ND 4 ) 2 PtCl 4 Solid State Nucl. Magn. Reson. 22 2002 373 393
19. A. Birczyński, Z.T. Lalowicz, Z. Olejniczak, G. Stoch, and B. Petelenz Low temperature domain structure in (ND 4 ) 2 TeCl 6 detected by deuteron NMR spectroscopy Chem. Phys. Lett. 339 2001 229 236
20. P. Filipek, Z.T. Lalowicz, Z. Olejniczak, and A. Birczyński Deuteron NMR study of ammonium ion mobility near the order-disorder phase transition in (ND 4 ) 2 PbCl 6 Chem. Phys. Lett. 367 2003 55 61
21. K. Vogt, and W. Prandl Calculation of the molecular rotational potential from Bragg scattering data: the method and an application to (NH 4 ) 2 SnCl 6 J. Phys. C: Solid State Phys. 16 1983 4753 4768
22. Th. Brückel, W. Prandl, K. Vogt, and C.M.E. Zeyen Quantum disorder in (NH 4 ) 2 SnCl 6 : a quantum mechanical single-particle model interpretation of neutron diffraction data J. Phys. C: Solid State Phys. 17 1984 4071 4088
23. J.A. Lerbscher, and J. Trotter Potassium Hexachlorostannate (IV) and Ammonium Hexachlorostannate (IV) Acta Crystallogr. B 32 1976 2671
24. O. Yamamuro, H. Muraoka, T. Ohta, T. Matsuo, Y. Kume, N. Onoda-Yamamuro, K. Oikawa, and T. Kamiyama Neutron diffraction study on orientational disorder of ND 4 + ions in (ND 4 ) 2 SeCl 6 crystal J. Phys. Soc. Jpn. 64 1995 2722 2725
25. O. Yamamuro, K. Okishiro, T. Matsuo, N. Onoda-Yamamuro, K. Oikawa, T. Kamiyama, Y. Kume, and F. Izumi Neutron diffraction study of (ND 4 ) 2 SeCl 6, (ND 4 ) 2 PtCl 6, and (ND 4 ) 2 PtBr 6 crystals: the origin of the strong deuterium substitution effect on the phase transitions J. Chem. Phys. 107 1997 8004 8011
26. L.P. Ingman, E. Koivula, M. Punkkinen, E.E. Ylinen, and Z.T. Lalowicz Deuteron spin-lattice relaxation in (ND 4 ) 2 SnCl 6 below 60 K Physica B 162 1990 281 292
27. 35Cl nuclear-quadrupole-resonance study of ammonium-ion motion and phase transitions in natural and deuterated (NH 4 ) 2 TeCl 6 Phys. Rev. B 41 1990 3914 3919
28. J. Pelzl, and C. Dimitropoulos Effect of deuteration on the phase transitions and on the critical dynamics in ammonium hexachlorometallates Z. Naturforsch. 49a 1994 232 246
29. C. Dimitropoulos, and Z.T. Lalowicz NMR and NQR spin-lattice relaxation in partially deuterated (NH 4 ) 2 SnCl 6 Phys. Rev. B 49 1994 644 646
30. Z.T. Lalowicz, U. Werner, and W. Müller-Warmuth Rotational tunnelling of CD 3 groups in molecular crystals as studied by NMR spectra Z. Naturforsch. 43a 1988 219 227
31. A. Detken, P. Focke, H. Zimmermann, U. Haeberlen, Z. Olejniczak, and Z.T. Lalowicz Deuteron NMR spectra of metyl groups in the tunnelling regime. A single crystal study of aspirin- CD 3 Z. Naturforsch. 50a 1995 95 116
32. 2H-NMR spectroscopy Z. Naturforsch. 46a 1991 829 840
33. Z. Olejniczak, Z.T. Lalowicz, T. Schmidt, H. Zimmermann, U. Haeberlen, and H. Schmitt The dynamics of ND 4 + and NH 3 D + groups in ammonium persulphate studied by deuteron nuclear magnetic resonance. I. Tunneling and stochastic reorientations at low temperatures J. Chem. Phys. 116 2002 10343 10355
34. T. Schmidt, H. Schmitt, U. Haeberlen, Z. Olejniczak, and Z.T. Lalowicz ND 4 + and NH 3 D + dynamics in ammonium persulphate. II. Transition from low-to-high-temperature regime J. Chem. Phys. 117 2002 9818 9827
35. 17O NMR spectra J. Magn. Reson. 72 1987 493 501
36. A. Heuer, and U. Haeberlen A new method for suppressing baseline distortions in FT NMR J. Magn. Reson. 85 1989 79
37. G. Stoch, and Z. Olejniczak Missing first points and phase artifact mutually entangled in FT NMR data-noniterative solution J. Magn. Reson. 140 2005 140 152
38. 2H NMR spectra applied to partially deuterated (NH 4 ) 2 SnCl 6 compounds Mol. Phys. Rep. 33 2001 127 131
39. E.E. Ylinen, Z.T. Lalowicz, S.F. Sagnowski, M. Punkkinen, E. Koivula, and L.P. Ingman Deuteron NMR spectrum of ND 4 VO 3 and some other ammonium salts Chem. Phys. Lett. 192 1992 590 594
40. I. Svare, D.R. Torgeson, and F. Borsa Tunneling and spin-lattice relaxation of hydrogen dissolved in scandium metal Phys. Rev. B 43 1991 7448 7457
41. S. Estalji, O. Kanert, J. Steinert, H. Jain, and K.L. Ngai Uncommon nuclear-spin relaxation in fluorozirconate glasses at low temperatures Phys. Rev. B 43 1991 7481 7486