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Volumn 6, Issue 10, 2005, Pages 2190-2196

Microcavity-controlled single-molecule fluorescence

Author keywords

Fluorescence spectroscopy; Microcavity; Single molecule studies; Spontaneous emission enhancement; Time resolved spectroscopy

Indexed keywords

FABRY-PEROT INTERFEROMETERS; FLUORESCENCE; FLUORESCENCE SPECTROSCOPY; LASER SPECTROSCOPY; MICROCAVITIES; PARTICLE BEAMS; SPONTANEOUS EMISSION;

EID: 27144494194     PISSN: 14394235     EISSN: None     Source Type: Journal    
DOI: 10.1002/cphc.200500108     Document Type: Article
Times cited : (61)

References (42)
  • 5
    • 27144552410 scopus 로고    scopus 로고
    • note
    • All values denoted as free space in this work refer to molecular fluorescence emission in a microcavity of the same type as that reported in the Experimental Section, but without silver mirrors.
  • 7
  • 32
    • 14344280947 scopus 로고
    • The microcavity design presented in this paper has some relation to a similar resonator layout reported earlier using an air gap between two dielectric substrates with different refractive indices: R. E. Kunz, W. Lukosz, Phys. Rev. B 1980, 21, 4814.
    • (1980) Phys. Rev. B , vol.21 , pp. 4814
    • Kunz, R.E.1    Lukosz, W.2
  • 34
    • 27144463243 scopus 로고    scopus 로고
    • note
    • It should be remarked that single-molecule fluorescence was also observed for higher interference orders up to m = 3. Since the observation volume increases with the cavity length L, the ratio of single molecule to background fluorescence signal decreases for a given dye concentration and spatial addressing of single molecules becomes impossible for larger orders of interference.
  • 35
    • 27144506339 scopus 로고    scopus 로고
    • note
    • 0 of PI molecules solved in dichloromethane as well as embedded in the cured polymer was measured by applying standard methods using Rhodamin 6 G dye as a reference.
  • 36
    • 27144469649 scopus 로고    scopus 로고
    • note
    • 2 = 0.91 at λ = 532 nm calculated for the thickness of our silver films measured by AFM.
  • 37
    • 27144543327 scopus 로고    scopus 로고
    • note
    • 2 = 0.9 at λ = 532 nm calculated for the thickness of our silver films measured by AFM.
  • 39
    • 27144494354 scopus 로고    scopus 로고
    • note
    • SpE could also be modelled assuming parallel dipole orientation (θ = 0°) and emitter displacements of ± 30 nm from the z = 0 plane in the center of the microcavity.


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.