Ethanol and acetaldehyde adsorption on a carbon-supported Pt catalyst: A comparative DEMS study

Fuel Cells

Volumn 4, Issue 1-2, 2004, Pages 113-125

  Wang, H ^a,b   Jusys, Z ^a   Behm, R J ^a  

^a UNIVERSITY OF ULM   (Germany)

^b BEIJING NORMAL UNIVERSITY   (China)

Author keywords

Acetaldehyde; Adsorption; Adsorption kinetics; C2h6 formation; Ch4 formation; Co oxidation; DEMS; Dissociation; Ethanol; Pt vulcan catalyst; Supported catalyst

Indexed keywords

ADSORPTION; ALDEHYDES; CATALYST ACTIVITY; DISSOCIATION; ELECTROCHEMISTRY; ETHANOL; MASS SPECTROMETRY; OXIDATION; PLATINUM; REACTION KINETICS;

ACETALDEHYDE; ADSORPTION KINETICS; CH4 FORMATION; CO OXIDATION; DIFFERENTIAL ELECTROCHEMICAL MASS SPECTROMETRY (DEMS); PT/VULCAN CATALYSTS; SUPPORTED CATALYSTS;

FUEL CELLS;

EID: 2442612123     PISSN: 16156846     EISSN: None     Source Type: Journal    
DOI: 10.1002/fuce.200400014     Document Type: Conference Paper

References (35)

1. J. Wang, S. Wasmus, R.F. Savinell, J. Electrochem. Soc. 1995, 142, 4218.
2. V.M. Schmidt, R. Ianniello, E. Pastor, S. Gonzalez, J. Phys. Chem., 100, 17901.
3. S.-G. Sun, in Electrocatalysis, J. Lipkowski and P. N. Ross Jr., eds., Wiley-VCH, 1998.
4. N. Fujiwara, K.A. Friedrich, U. Stimming, J. Electroanal. Chem. 1999, 472, 120.
5. J.L. Rodríguez, E. Pastor, X.H. Xia, T. Iwasita, Langmuir 2000, 16, 5479.
6. C. Lamy, E.M. Belgsir, J.-M. Léger, J. Appl. Electrochem. 2001, 31, 799.
7. J.P.I. de Souza, S.L. Queiroz, K. Bergamaski, E.R. Gonzalez, F.C. Nart, J. Phys. Chem. B 2002, 106, 9825.
8. H. Hitmi, E.M. Belgsir, J.M. Leger, C. Lamy, R.O. Lezna, Electrochim. Acta 1994, 39, 407.
9. V.S. Bagotzky, Y. B. Vassilyev, Electrochim. Acta 1967, 12, 1323.
10. B. Bittins-Cattaneo, S. Wilhelm, E. Cattaneo, H.W. Buschmann, W. Vielstich, Ber. Bunsenges. Phys. Chem. 1988, 92, 1210.
11. B. Beden, M.C. Morin, F. Hahn, C. Lamy, J. Electroanal. Chem. 1987, 229, 353.
12. F. Cases, M. Lopez-Atalaya, J.L. Vazquez, A. Aldaz, J. Clavilier, J. Electroanal. Chem. 1990, 278, 433.
13. J. Shin, W.J. Tornquist, C. Korzeniewski, C.S. Hoaglurvd, Surf. Sci. 1996, 364, 122.
14. T. Iwasita, E. Pastor, Electrochim. Acta, 1994, 39, 531.
15. R. Ianniello, V.M. Schmidt, J.L. Rodriguez, E. Pastor, J. Electroanal. Chem. 1999, 471, 167.
16. J. Silva-Chong, E. Méndez, J.L. Rodriguez, M.C. Aréva- lo, E. Pastor, Electrochim. Acta 2003, 47, 1441.
17. E. Mendéz, J.L. Rodriguez, M.C. Arévalo, E. Pastor, Langmuir 2002, 18, 763.
18. J. Willsau, J. Heitbaum, J. Electroanal. Chem. 1985, 194, 27.
19. U. Schmiemann, U. Müller, H. Baltruschat, Electrochim. Acta 1994, 40, 99.
20. J.F.E. Gootzen, W. Visscher, J.A.R. Van Veen, Langmuir 1996, 12, 5076.
21. Z. Jusys, J. Kaiser, R.J. Behm, Langmuir 2003, 19, 6759.
22. Z. Jusys, R.J. Behm, J. Phys. Chem. B 2001, 105, 10874.
23. Z. Jusys, J. Kaiser, R.J. Behm, Chem. Phys. 2001, 3, 4650.
24. T.J. Schmidt, H.A. Gasteiger, G.D. Stäb, P.M. Urban, D.M. Kolb, R.J. Behm, J. Electrochem. Soc. 1998, 145, 2354.
25. Z. Jusys, H. Massong, H. Baltruschat, J. Electrochem. Soc. 1999, 146, 1093.
26. L.-W.H. Leung, S.-C. Chang, M.J. Weaver, J. Electroanal. Chem. 1989, 266, 317.
27. th Electrochemical Society Meeting, S. Naraya-nan, T. Zawodzinski, S. Gottesfeld (eds.), (Electrochemical Society, Pennington, 2001), p. 50.
28. B.I. Podlovchenko, O.A. Petry, A.N. Frumkin, H. Lal, J. Electroanal. Chem. 1966, 11, 12.
29. H. Wang, Z. Jusys, R.J. Behm, to be publ.
30. M.E. Gamboa-Aldeo, E. Herrero, P.S. Zelenay, A. Wieckowski, J. Electroanal. Chem. 1993, 348, 451.
31. F. Cases, J.L. Vazquez, J.M. Perez, A. Aldaz, J. Clavilier, J. Electroanal. Chem. 1990, 281, 283.
32. H. Baltruschat, in Interfacial Electrochemistry - Theory, Experiment and Applications, A. Wieckowski (ed.), Marcel Dekker Inc., New York, 1999.
33. J. Willsau, J. Heitbaum, Electrochim. Acta 1986, 31, 943.
34. H. Zhao, J. Kim, B.E. Koel, Surf. Sci. 2003, 538, 147.
35. Atlas of mass spectral data, E. Stenhagen, S. Abrahamsson, F.W. McLafferty (eds.) Interscience, New York, 1969.