Femtosecond time-resolved geometry relaxation and ultrafast intramolecular energy redistribution in Ag2Au

ChemPhysChem

Volumn 6, Issue 2, 2005, Pages 243-253

  Bernhardt, Thorsten M ^a   Hagen, Jan ^a   Socaciu, Liana D ^a   Mitrić, Roland ^b   Heidenreich, Andreas ^c   Le Roux, Jérôme ^a   Popolan, Denisia ^a   Vaida, Mihai ^a   Wöste, Ludger ^a   Bonaĉić Koutecký, Vlasta ^b   Jortner, Joshua ^c  

^a FREIE UNIVERSITÄT BERLIN   (Germany)

^b HUMBOLDT UNIVERSITY   (Germany)

^c TEL AVIV UNIVERSITY   (Israel)

Author keywords

Femtochemistry; Gold; Mass spectrometry; Metal clusters; Silver

Indexed keywords

BINARY ALLOYS; GOLD; GOLD ALLOYS; KINETIC ENERGY; KINETICS; MASS SPECTROMETRY; NEGATIVE IONS; PHOTOIONIZATION; POLONIUM COMPOUNDS; POSITIVE IONS; PROBES; SILVER;

FEMTOCHEMISTRY; FEMTOSECOND TIME-RESOLVED; INTRAMOLECULAR VIBRATIONAL ENERGY REDISTRIBUTIONS; IONIZATION PROBABILITIES; METAL CLUSTER; THEORETICAL SIMULATION; TWO PHOTON IONIZATION; ZERO ELECTRON KINETIC ENERGIES;

SILVER ALLOYS;

GOLD DERIVATIVE; SILVER DERIVATIVE;

ACCURACY; ARTICLE; CALCULATION; CHEMICAL STRUCTURE; CONFORMATIONAL TRANSITION; ELECTRIC POTENTIAL; ENERGY TRANSFER; FEMTOSECOND TIME RESOLVED SPECTROSCOPY; GEOMETRY; HYPOTHESIS; MEASUREMENT; MOLECULAR DYNAMICS; MOLECULAR WEIGHT; PARAMETER; SIMULATION; SPECTROSCOPY; STRUCTURE ANALYSIS; SURFACE PROPERTY; TECHNIQUE; TEMPERATURE DEPENDENCE; VIBRATION;

EID: 20144376076     PISSN: 14394235     EISSN: None     Source Type: Journal    
DOI: 10.1002/cphc.200400454     Document Type: Article

References (47)

1. a) A. H. Zewail, Femtochemistry: Ultrafast Dynamics of the Chemical Bond, World Scientific, Singapore, 1994;
2. b) J. Manz, L. Wöste, Femtosecond Chemistry, VCH, Weinheim, 1995;
3. c) M. Chergui, Femtochemistry: Ultrafast Chemical and Physical Processes in Molecular Systems, World Scientific, Singapore, 1996.
4. V. Sundström, in Nobel Symposium, Vol. 101, Imperial College Press, London, 1997.
5. a) A. H. Zewail, Faraday Discuss. Chem. Soc. 1991, 91, 207;
6. b) A. Mokhtari, P. Cong, J. L. Herek, A. H. Zewail, Nature 1990, 348, 225;
7. c) M. Dantus, R. M. Bowman, M. Gruebele, A. H. Zewail, J. Chem. Phys. 1989, 91, 7437;
8. d) A. Weaver, R. B. Metz, S. E. Bradforth, D. M. Neumark, J. Chem. Phys. 1990, 93, 5352;
9. e) R. B. Metz, D. M. Neumark, J. Chem. Phys. 1992, 97, 962;
10. f) D. M. Neumark, Acc. Chem. Res. 1993, 26, 33;
11. g) S. M. Burnett, A. E. Stevens, C. S. Feigerle, W. C. Lineberger, Chem. Phys. Lett. 1983, 100, 124;
12. h) K. M. Ervin, J. Ho, W. C. Lineberger, J. Chem. Phys. 1989, 91, 5974;
13. i) P. G. Wenthold, D. Hrovat, W. T. Borden, W. C. Lineberger, Science 1996, 272, 1456.
14. S. Wolf, G. Sommerer, S. Rutz, E. Schreiber, T. Leisner, L. Wöste, R. S. Berry, Phys. Rev. Lett. 1995, 74, 4177.
15. R. S. Berry, V. Bonačić-Koutecký, J. Gaus, T. Leisner, J. Manz, B. Reischl-Lenz, H. Ruppe, S. Rutz, E. Schreiber, S. Vajda, R. de Vivie-Riedle, S. Wolf, L. Wöste, Adv. Chem. Phys. 1997, 101, 101.
16. O. Rubner, C. Meier, V. Engel, J. Chem. Phys. 1997, 107, 1066.
17. M. Hartmann, J. Pittner, V. Bonačić-Koutecký, A. Heidenreich, J. Jortner, J. Chem. Phys. 1998, 108, 3096.
18. M. Hartmann, J. Pittner, V. Bonačić-Koutecký, A. Heidenreich, J. Jortner, J. Phys. Chem. A 1998, 102, 4069.
19. a) L. Wöste, Z. Phys. Chem. (Muenchen Ger.) 1996, 196, 1;
20. b) H. Hess, K. R. Asmis, T. Leisner, L. Wöste, Eur. J. Phys. 2001, 16, 145.
21. D. H. Paik, D.-S. Yang, I.-R. Lee, A. H. Zewail, Angew. Chem. 2004, 116, 2890; Angew. Chem. Int. Ed. 2004, 43, 2830.
22. D. H. Paik, D.-S. Yang, I.-R. Lee, A. H. Zewail, Angew. Chem. 2004, 116, 2890; Angew. Chem. Int. Ed. 2004, 43, 2830.
23. a) H. O. Jeschke, M. E. Garcia, K. H. Bennemann, Phys. Rev. A 1996, 54, R4601;
24. b) H. O. Jeschke, M. E. Garcia, K. H. Bennemann, J. Phys. B At Mol Opt Phys 1996, 29, L545.
25. W. D. Boo, Y. Ozaki, L. H. Andersen, W. C. Lineberger, J. Phys. Chem. A 1997, 101, 6688.
26. I. Adrianov, V. Bonačić-Koutecký, M. Hartmann, J. Manz, J. Pittner, K. Sundermann, Chem. Phys. Lett. 2000, 318, 256.
27. a) J. Manz, C. S. Parmenter, Mode Selectivity in Unimolecular Reactions, Chem. Phys. 1989, 139 (special issue);
28. b) J. Jortner, R. D. Levine, R. B. Pullman, Mode Selective Chemistry, Kluwer, Dordrecht, 1991.
29. a) C. N. Hinshelwood, Proc. R. Soc. Lond. A 1926, 113, 230;
30. b) C. N. Hinshelwood, C. J. M. Fletcher, Nature 1933, 24, 131.
31. A. Amirav, C. Horowitz, J. Jortner, J. Chem. Phys. 1988, 88, 3092.
32. P. M. Felker, A. H. Zewail, J. Chem. Phys. 1985, 83, 2975.
33. T. Leisner, S. Vajda, S. Wolf, L. Wöste, R. S. Berry, J. Chem. Phys. 1999, 111, 1017.
34. H. Hess, S. Kwiet, L. Socaciu, S. Wolf, T. Leisner, L. Wöste, Appl. Phys. B 2000, 71, 337.
35. R. Keller, F. Nöhmeier, P. Spädtke, M. H. Schönenberg, Vacuum 1984, 34, 31.
36. C.-P. Huang, M. T. Asaki, S. Backus, M. M. Murnane, H. C. Kapteyn, Opt. Lett. 1992, 17, 1289.
37. a) M. Hartmann, J. Pittner, H. van Dam, V. Bonačić- Koutecký, Eur. Phys. J. D 1999, 9, 393;
38. b) M. Hartmann, J. Pittner, V. Bonačić-Koutecký, J. Chem. Phys. 2001, 114, 2106;
39. S. Vajda, C. Lupulescu, A. Merli, F. Budzyn, L. Wöste, M. Hartmann, J. Pittner, V. Bonačić-Koutecký, Phys. Rev. Lett. 2002, 89, 213 404.
40. M. Hartmann, R. Mitrić, B. Stanca, V. Bonačić- Koutecký, Eur. Phys. J. D 2001, 16, 151.
41. M. Hartmann, J. Pittner, V. Bonačić-Koutecký, J. Chem. Phys. 2001, 114, 2132.
42. R. Mitrić, M. Hartmann, B. Stanca, V. Bonačić- Koutecký, P. Fantucci, J. Phys. Chem. A 2001, 105, 8892.
43. a) D. Reichardt, V. Bonačić-Koutecký, P. Fantucci, J. Jellinek, Chem. Phys. Lett. 1997, 279, 129;
44. b) V. Bonačić-Koutecký, M. Hartmann, D. Reichardt, P. Fantucci in Recent Advances in Density Functional Methods, Part III (Eds.: V. Barone, A. Bencini, P. Fantucci), World Scientific, Singapore, 2000.
45. R. Mitrić, M, Hartmann, B. Stanca, V. Bonačić- Koutecký, P. Fantucci, J. Phys. Chem. A 2001, 105, 8892.
46. Y. Negeshi, Y. Nakamura, A. Nakajima, K. Kaya, J. Chem. Phys. 2001, 115, 36S7.
47. J. Hagen, PhD thesis, Freie Universität Berlin (Berlin), 2004.