The aerosol-climate model ECHAM5-HAM

Atmospheric Chemistry and Physics

Volumn 5, Issue 4, 2005, Pages 1125-1156

  Stier, P ^a   Feichter, J ^a   Kinne, S ^a   Kloster, S ^a   Vignati, E ^b   Wilson, J ^b   Ganzeveld, L ^c   Tegen, I ^d   Werner, M ^d   Balkanski, Y ^e   Schulz, M ^e   Boucher, O ^f   Minikin, A ^g   Petzold, A ^g  

^a MAX PLANCK INSTITUTE FOR METEOROLOGY   (Germany)

^b JOINT RESEARCH CENTRE   (Italy)

^c MAX PLANCK INSTITUTE FOR CHEMISTRY   (Germany)

^d MAX PLANCK INSTITUTE FOR BIOGEOCHEMISTRY   (Germany)

^e LABORATOIRE DES SCIENCES DU CLIMAT ET DE L ENVIRONNEMENT   (France)

^f CNRS   (France)

^g GERMAN AEROSPACE CENTER DLR   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 17744381356     PISSN: 16807316     EISSN: None     Source Type: Journal    
DOI: 10.5194/acp-5-1125-2005     Document Type: Review

References (125)

1. Adams, P. J. and Seinfeld, J. H.: Predicting global aerosol size distributions in general circulation models, J. Geophys. Res., 107, 4370, doi:10.1029/2001JD001010, 2002.
2. Albrecht, B. A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227-1230, 1989.
3. Andreae, M. and Crutzen, P.: Atmospheric aerosols: biogeochemical sources and role in atmospheric chemistry, Science, 276, 1052-1058, 1997.
4. Andreae, M. O., Rosenfeld, D., Artaxo, P., Costa, A. A., Frank, G. P., Longo, K. M., and Silva-Diass, M. A. F.: Smoking rain clouds over the Amazon, Science, 303, 1337-1342, 2004.
5. Andres, R. J. and Kasgnoc, A. D.: A time-averaged inventory of subaerial volcanic sulfur emissions, J. Geophys. Res., 103, 25 251-25 261, 1998.
6. Ångström, A.: Atmospheric turbidity, global illumination and planetary albedo of the earth, Tellus, 14, 435-450, 1962.
7. Balkanski, Y., Schulz, M., Claquin, T., Moulin, C., and Ginoux, P.: Emission Of Atmospheric Trace Compounds, chap. Global emissions of mineral aerosol: formulation and validation using satellite imagery, pp. 239-267, Ed. Kluwer, 2004.
8. Bates, T. S., Huebert, B. J., Gras, J. L., Griffiths, F. B., and Durkee, P. A.: International Global Atmospheric Chemistry (IGAC) project's first Aerosol Characterisation Experiment (ACE 1): overview., J. Geophys. Res., 103, 16 297-16 318, 1998.
9. Bond, T. C., Streets, D. G., Yarber, K. F., Nelson, S. M., Woo, J.-H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res., 109, D14 203, doi:10.1029/2003JD003 697, 2004.
10. Chin, M., Jacob, D. J., Gardner, G. M., Foreman-Fowler, M. S., Spiro, P. A., and Savoie, D. L.: A global three-dimensional model of tropospheric sulfate, J. Geophys. Res., 101, 18 667-18 690, 1996.
11. Chin, M., Ginoux, P., Kinne, S., Torres, O., Holben, B. N., Duncan, B. N., Martin, R. V., Logan, J. A., Higurashi, A., and Nakajima, T.: Tropospheric aerosol optical thickness from the GOCART model and comparisons with satellite and Sun photometer measurements, J. Atmos. Sci., 59, 461-483, 2002.
12. Chu, D. A., Kaufman, Y. J., Ichoku, C., Remer, L. A., Tanré, D., and Holben, B. N.: Validation of MODIS aerosol optical depth retrieval over land, Geophys. Res. Lett., 29, 8007, doi:10.1029/2001GL013 205, 2002.
13. Chung, S. H. and Seinfeld, J. H.: Global distribution and climate forcing of carbonaceous aerosols, J. Geophys. Res., 107, 4407, doi:10.1029/2001JD001 397, 2002.
14. Claquin, T.: Modeling of the mineralogy and the radiative forcing of desert dust, Ph.D. thesis, Paris University, Paris, France, 1999.
15. Cofala, J., Amann, M., and Mechler, R.: Scenarios of world anthropogenic emissions of air pollutants and methane up to 2030, Tech. rep., International Institute for Applied Systems Analysis (IIASA), Laxenburg, Austria, available from: http://www.iiasa.ac.at/rains/global_emiss/ global_emiss.html, 2005.
16. Crutzen, P.: Nucleation of atmospheric aerosols, chap. The role of particulate matter in ozone photochemistry, pp. 268-270, Elsevier, 1996.
17. 3, and OH, J. Geophys. Res., 98, 7149-7163, 1993.
18. Downing, H. D. and Williams, D.: Optical-constants of water in infrared, J. Geophys. Res., 80, 1656-1661, 1975.
19. Dubovik, O. and King, M. D.: A flexible inversion algorithm for retrieval of aerosol optical properties from sun and sky radiance measurements, J. Geophys. Res., 105, 20 673-20 696, 2000.
20. Feichter, J., Kjellström, E., Rodhe, H., Dentener, F., Lelieveld, J., and Roelofs, G.-J.: Simulation of the tropospheric sulfur cycle in a global climate model, Atmos. Environ., 30, 1693-1707, 1996.
21. Feichter, J., Roeckner, E., Lohmann, U., and Liepert, B.: Nonlinear aspects of the climate response to greenhouse gas and aerosol forcing, J. Clim., 17, 2384-2398, 2004.
22. Fouquart, Y. and Bonnel, B.: Computations of solar heating of the earth's atmosphere: A new parameterization, Beitr. Phys. Atmos., 53, 35-62, 1980.
23. Fuchs, N. A.: Evaporation and droplet growth in gaseous media, Pergamon, Tarrytown, New York, 72 pp., 1959.
24. Fuchs, N. A.: The mechanics of aerosols, Pergamon Press, Oxford, 1964.
25. Gallagher, M. W., Nemitz, E., Dorsey, J. R., Fowler, D., Sutton, M. A., and and J. Duyzer, M. F.: Measurements and parameterizations of small aerosol deposition velocities to grassland, arable crops, and forest: Influence of surface roughness length on deposition, J. Geophys. Res., 107, 4154, doi:10.1029/2001JD000 817, 2002.
26. Ganzeveld, L. and Lelieveld, J.: Dry deposition parameterization in a chemistry general circulation model and its influence on the distribution of reactive trace gases, J. Geophys. Res., 100, 20 999-21 012, 1995.
27. Ganzeveld, L., Lelieveld, J., and Roelofs, G.-J.: Dry deposition parameterization of sulfur oxides in a chemistry and general circulation model, J. Geophys. Res., 103, 5679-5694, 1998.
28. Ghan, S., Laulainen, N., Easter, R., Wagener, R., Nemesure, S., Chapman, E., and Leung, Y. Z. R.: Evaluation of aerosol direct radiative forcing in MIRAGE, J. Geophys. Res., 106, 5295-5316, 2001a.
29. Ghan, S. J., Easter, R. C., Hudson, J., and Brèon, F.-M.: Evaluation of aerosol indirect radiative forcing in MIRAGE, J. Geophys. Res., 106, 5317-5334, 2001b.
30. Gong, S. L., Barrie, L. A., and Lazare, M.: Canadian Aerosol Module (CAM): A size-segregated simulation of atmospheric aerosol processes for climate and air quality models 2. Global sea-salt aerosol and its budgets, J. Geophys. Res., 107, 4779, doi:10.1029/2001JD002 004, 2002.
31. Gong, S. L., Barrie, L. A., Blanchet, J. P., K. von Salzen, U. L., Lesins, G., Spacek, L., Zhang, L. M., Girard, E., Lin, H., Leaitch, R., Leighton, H., Chylek, P., and Huang, R: Canadian Aerosol Module: A size-segregated simulation of atmospheric aerosol processes for climate and air quality models - 1. Module development, J. Geophys. Res., 108, 4007, doi:10.1029/2002JD002 633, 2003.
32. Graßl, H.: Albedo reduction and radiative heating of clouds by absorbing aerosol particles, Contributions Atmospheric Physics, 48, 199-210, 1975.
33. Guelle, W., Schulz, M., Balkanski, Y., and Dentener, F.: Influence of the source formulation on modeling the atmospheric global distribution of sea salt aerosol, J. Geophys. Res., 106, 27 509-27 524, 2001.
34. Guenther, A., Hewitt, C. N., Erickson, D., Fall. R., Geron, C., Graedel, T., Harley, P., Klinger, L., Lerdau, M., McKay, W. A., Pierce, T., Scholes, B., Steinbrecher, R., Tallamraju, R., Taylor, J., and Zimmerman, P: A global model of natural volatile organic compound emissions, J. Geophys. Res., 100, 8873-8892, 1995.
35. Gutman, G., Tarpley, D., Ignatov, A., and Olson, S.: The enhanced NOAA global land dataset from Advanced Very High Resolution Radiometer, Bull. Am. Meteorol. Soc., 76, 1141-1156, 1995.
36. Halmer, M. M., Schmincke, H.-U., and Graf, H.-F.: The annual volcanic gas input into the atmosphere, in particular into the stratosphere: a global data set for the past 100 years, Journal of Volcanology and Geothermal Research, 115, 511-528, 2002.
37. Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, J. Geophys. Res., 102, 6831-6864, 1997.
38. Haywood, J. M., Ramaswamy, V., and Donner, L. J.: A limited-area-model case study of the effects of sub-grid scale variations in relative humidity and cloud upon the direct radiative forcing of sulfate aerosol, Geophys. Res. Lett., 24, 143-146, 1997a.
39. Haywood, J. M., Roberts, D. L., Slingo, A., Edwards, J. M., and Shine, K. P.: General circulation model calculations of the direct radiative forcing by anthropogenic sulfate and fossil-fuel soot aerosol, J. Clim., 10, 1562-1577, 1997b.
40. Heintzenberg, J., Raes, F., Schwartz. S., Ackermann, I., Artaxo, P., Bates, T., Benkovitz, C., Bigg, K., Bond, T., Brenguier, J., Eisele, F., Feichter, J., Flossmann, A., Fuzzi, S., Graf, H., Hales, J., Herrmann, H., Hoffmann, T., Huebert, B., Husar, R., Jaenicke, R., Kärcher, B., Kaufman, Y., Kent, G., Kulmala, M., Leck, C., Liousse, C., Lohmann, U., Marticorena, B., Mcmurry, P., Noone, K., Dowd, C., Penner, J., Pszenny, A., Putaud, J., Quinn, P., Schurath, U., Seinfeld, J., Sievering, H., Snider, J., Sokolik, I., Stratmann, F., Dingenen, R. V., Westphal, D., Wexler, A., Wiedensohler, A., Winkler, D., and Wilson, J.: Atmospheric Chemistry in a Changing World, An Integration and Synthesis of a Decade of Tropospheric Chemistry Research, chap. Tropospheric Aerosols, pp. 125-156, Global Change - The IGBP Series, Springer, Berlin Heidelberg New York, 2003.
41. Henning, S., Bojinski, S., Diehl, K., Ghan, S., Nyeki, S., Weingartner, E., Wurzler, S., and Baltensperger, U.: Aerosol partitioning in natural mixed-phase clouds, Geophys. Res. Lett., 31, L06 101, doi:10.1029/2003GL019 025, 2004.
42. Hess, M., Koepke, P., and Schult, I.: Optical properties of aerosols and clouds: The software package OPAC, Bull. Am. Meteorol. Soc., 79, 831-844, 1998.
43. Holben, B. N., Tanré, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N., Newcomb, W. W., Schafer, J. S., Chatenet, B., Lavenu, F., Kaufman, Y. J., Castle, J. V., Setzer, A., Markham, B., Frouin, D. C. R., Halthore, R., Karneli, A., O'Neill, N. T., Pietras, C., Pinker, R. T., Voss, K., and Zibordi, G.: An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET, J. Geophys. Res., 106, 12 067-12 098, 2001.
44. Horowitz, L. W., Walters, S., Mauzerall, D. L., Emmons, L. K., Rasch, P. J., Granier, C., Tie, X., Lamarque, J.-F., Schultz, M. G., Tyndall, G. S., Orlando, J. J., and Brasseur, G. P.: A global simulation of tropospheric ozone and related tracers: Description and evaluation of MOZART, version 22, J. Geophys. Res., 108, 4784, doi:10.1029/2002JD002 853, 2003.
45. Hsu, N. C., Herman, J. R., Torres, O., Holben, B. N., Tanre, D., Eck, T. F., Smirnov, A., Chatenet, B., and Lavenu, F.: Comparisons of the TOMS aerosol index with Sun-photometer aerosol optical thickness: Results and applications, J. Geophys. Res., 104, 6269-6280, 1999.
46. Hummelshøj, P., Jensen, N. O., and Larsen, S. E.: Particle dry deposition to a sea surface, pp. 829-840, Precipitation scavenging and atmosphere-surface exchange, Hemisphere Publishing Corporation, Washington, 1992.
47. Jacobson, M. Z.: GATOR-GCMM: A global-through urban-scale air pollution and weather forecast model, 1. Model design and treatment of subgrid soil, vegetation, roads, rooftops, water, sea ice, and snow, J. Geophys. Res., 106, 5385-5402, 2001.
48. Jacobson, M. Z., Tabazadeh, A., and Turco, R. P.: Simulating equilibrium within aerosols and nonequilibrium between gases and aerosols, J. Geophys. Res., 101, 9079-9091, 1996.
49. Johnson, K., Gordon, R., and Coale, K.: What controls dissolved iron concentrations in the world ocean?, Marine Chemistry, 57, 137-161, 1997.
50. Kaufman, Y. J., Tanré, D., Remer, L. A., Vermote, E. F., Chu, A., and Holben, B. N.: Operational remote sensing of tropospheric aerosol over land from EOS moderate resolution imaging spectroradiometer, J. Geophys. Res., 102, 17 051-17 068, 1997.
51. Kettle, A. and Andreae, M.: Flux of the dimethylsulfide from the oceans: A comparison of updated data sets and flux models, J. Geophys. Res., 105, 26 793-26 808, 2000.
52. Kinne, S., Lohmann, U., Feichter, J., Schulz, M., Timmreck, C., Ghan, S., Easter, R., Chin, M., Ginoux, P., Takemura, T., Tegen, I., Koch, D., Herzog, M., Penner, J., Pitari, G., Holben, B., Eck, T., Smirnov, A., Dubovik, O., Slutsker, I., Tanre, D., Torres, O., Mishchenko, M., Geogdzhayev, I., Chu, D. A., and Kaufman, Y.: Monthly averages of aerosol properties: A global comparison among models, satellite data, and AERONET ground data, J. Geophys. Res., 108, 4634, doi:10.1029/ 2001JD001 253, 2003.
53. Kirchstetter, T., Novakov, T., and Hobbs, P.: Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon, J. Geophys. Res., 109, D21 208, doi:10.1029/2004JD004999, 2004. 09, D21 208, doi: 10. 1029/2004JD004 999, 2004.
54. Koepke, P., Hess, M., Schutt, I., and Shettle, E.: Global Aerosol Data Set, Report 243, Max Planck Institute for Meteorology, Hamburg, ISSN 0937-1060, 1997.
55. Kulmala, M., Laaksonen, A., and Pirjola, L.: Parameterizations for sulfuric acid/water nucleation rates, J. Geophys. Res., 103, 8301-8307, 1998.
56. Langner, J. and Rhode, H.: A global three-dimensional model of the global sulfur cycle, J. Atmos. Chem., 13, 225-263, 1991.
57. Lelieveld, J., Berresheim, H., Borrmann, S., Crutzen, P. J., Dentener, F. J., Fischer, H., Feichter, J., Flatau, P. J., Heland, J., Holzinger, R., Korrmann, R., Lawrence, M. G., Levin, Z., Markowicz, K. M., Mihalopoulos, N., Minikin, A., Ramanathan, V., de Reus, M., Roelofs, G. J., Scheeren, H. A., Sciare, J., Schlager, H., Schultz, M., Siegmund, P., Steil, B., Stephanou, E. G., Stier, P., Traub, M., Warneke, C., Williams, J., and Ziereis, H.: Global air pollution crossroads over the mediterranean, Science, 298, 794-799, doi: 10.1126/science. 1075457, 2002.
58. Lesins, G., Chylek, P., and Lohmann, U.: A study of internal and external mixing scenarios and its effect on aerosol optical properties and direct radiative forcing, J. Geophys. Res., 107, 4094, doi:10.1029/ 2001JD000 973, 2002.
59. Liepert, B. G., Feichter, J., Lohmann, U., and Roeckner, E.: Can aerosols spin down the water cycle in a warmer and moister world?, Geophys. Res. Lett., 31, L06 207, doi:10.1029/2003GL019 060, 2004.
60. Lin, S. J. and Rood, R. B.: Multidimensional flux form semi-Lagrangian transport, Mon. Wea. Rev., 124, 2046-2068, 1996.
61. Lohmann, U.: A glaciation indirect aerosol effect caused by soot aerosols, Geophys. Res. Lett., 29, 1052, doi:10.1029/2001GL014 357, 2002.
62. Lohmann, U. and Feichter, J.: Impact of sulfate aerosols on albedo and lifetime of clouds: A sensitivity study with the ECHAM4 GCM, J. Geophys. Res., 102, 13 685-13 700, 1997.
63. Lohmann, U. and Kärcher, B.: First interactive simulations of cirrus clouds formed by homogeneous freezing in the ECHAM general circulation model, J. Geophys. Res., 107, 4105, doi:10.1029/2001JD000 767, 2002.
64. Lohmann, U. and Roeckner, E.: Design and performance of a new cloud microphysics scheme developed for the ECHAM4 general circulation model, Clim. Dyn., 12, 557-572, 1996.
65. Lohmann, U., Feichter, J., Chuang, C. C., and Penner, J. E.: Predicting the number of cloud droplets in the ECHAM-GCM, J. Geophys. Res., 104, 9169-9198, 1999a.
66. Lohmann, U., von Salzen, K., McFarlane, N., Leighton, H. G., and Feichter, J.: Tropospheric sulfur cycle in the Canadian general circulation model, J. Geophys. Res., 104, 26 833-26 858, 1999b.
67. Marticorena, B. and Bergametti, G.: Modeling the atmospheric dust cycle: 1. Design of a soil-derived dust emission scheme, J. Geophys. Res., 100, 16 415-16 430, 1995.
68. Martonchik, J., Diner, D., Crean, K., and Bull, M.: Regional aerosol retrieval results from MISR, IEEE Trans. Geosci. Remote Sens., 40, 1520-1531, 2002.
69. Martonchik, J., Diner, D., Kahn, R., Gaitley, B., and Holben, B.: Comparison of MISR and AERONET aerosol optical depths over desert sites, Geophys. Res. Lett., 31, L16 102, doi:10.1029/2004GL019 807, 2004.
70. Mayol-Bracero, M.-O., Guyon, P., Graham, B., Roberts, G., Andreae, M., Decesari, S., Facchini, M., Fuzzi, S., and Artaxo, P.: Water-soluble organic compounds in biomass burning aerosols over Amazonia - 2. Apportionment of the chemical composition and importance of the polyacidic fraction, J. Geophys. Res.-Atmos., 107, 8091, doi:10.1029/ 2001JD000 522, 2002.
71. McCormic, R. A. and Ludwig, J. H.: Climate modifications by atmospheric aerosols, Science, 156, 1358-1359, 1967.
72. Metzger, S., Dentener, F., Pandis, S., and Lelieveld, J.: Gas/aerosol partitioning, 1, A computationally efficient model, J. Geophys. Res., 107, 4312, doi:10.1029/2001JD001 102, 2002.
73. Minikin, A., Petzold, A., Strom, J., Krejci, R., Seifert, M., van Velthoven, v. P., Schlager, H., and Schumann, U.: Aircraft observations of the upper tropospheric fine particle aerosol in the Northern and Southern Hemispheres at midlatitudes, Geophys. Res. Lett., 30, 1503, doi:10.1029/2002GL016 458, 2003.
74. Mishchenko, M. I., Geogdzhayev, I. V., Cairns, B., Rossow, W. B., and Lacis, A. A.: Aerosol retrievals over the ocean by use of channels 1 and 2 AVHRR data: sensitivity analysis and preliminary results, Appl. Opt., 38, 7325-7341, 1999.
75. Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S. A.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated correlated-k model for the longwave, J. Geophys. Res., 102, 16 663-16 682, 1997.
76. Monahan, E., Spiel, D., and Davidson, K.: Oceanic whitecaps and their role in air-sea exchange, chap. A model of marine aerosol generation via whitecaps and wave disruption, pp. 167-174, D. Reidel, Norwell, Massachusetts, 1986.
77. Morcrette, J.-J., Clough, S. A., Mlawer, E. J., and Iacono, M. J.: Impact of a validated radiative transfer scheme, RRTM, on the ECMWF model climate and 10-day forecasts, ECMWF, Reading, UK, technical memorandum 252 edn., 1998.
78. Moulin, C., Dulac, F., Lambert, C. E., Chazette, P., Janowiak. I., Chatenet, B., and Lavenu, F.: Long-term daily monitoring of Saharan dust load over ocean using Meteosat ISCCP-B2 data, 2, Accuracy of the method and validation using Sun photometer measurements, J. Geophys. Res., 102, 16 959-16 969, 1997.
79. Murphy, D. M., Thomson, D. S., Middlebrook, A. M., and Schein, M. E.: In situ single-particle characterization at Cape Grim, J. Geophys. Res., 103, 16 485-16 491, 1998.
80. Nightingale, P., Malin, G., Law, C., Watson, A., Liss, P., Liddicoat, M., Boutin, J., and Upstill-Goddard, R.: In situ evaluation of airsea gas exchange parameterizations using novel conservative and volatile tracers, Global Biogeochem. Cycles, 14, 373-387, 2000.
81. Nordeng, T. E.: Extended versions of the convective parameterization scheme at ECMWF and their impact on the mean and transient activity of the model in the tropics, ECMWF, Reading, UK, technical memorandum edn., 1994.
82. Olson, J.: World ecosystems (WE1.4): Digital raster data on a 10 minute geographic 1080 (2160 grid square), Global Ecosystem Database, Version 1.0: DISC A, edited by NOAA National Geophysical Data Center, Boulder, CO, 1992.
83. Penner, J. E., Andreae, M., Annegarn, H., Barrie, L., Feichter, J., Hegg, D., Jayaraman, A., Leaitch, R., Murphy, D., Nganga, J., and Pitari, G.: Climate change 2001: the scientific basis, chap. Aerosols, their direct and indirect effects, pp. 298-248, Cambridge University Press, 2001.
84. Pham, M., J.-F.Muller, Brasseur, G., Granier, C., and Megie, G.: A three-dimensional study of the tropospheric sulfur cycle, J. Geophys. Res., 100, 26 061-26 092, 1995.
85. Putaud, J., van Dingenen, R., Baltensperger, U., Bruggemann, E., Charron, A., Facchini, M., Decesari, S., Fuzzi, S., Gehrig, R., H. H.-C., Harrison, R. M., Jones, A. M., Laj, P., Lorbeer, G., Maenhaut, W., Mihalopoulos, N., Müller, K., Palmgren, F., Querol, X., Rodriguez, S., Schneider, J., Spindler, G., ten Brink, H., Tunved, P., Torseth, K., Welmer, B., Weingartner, E., Wiedensohler, A., Wahlin, P., and Raes, F.: A european aerosol phenomenology, Report EUR 20411 EN, European Comission Joint Research Centre, Ispra, Italy, available from: http://carbodat.ei.jrc.it/ccu/, 2003.
86. Ramanathan, V., Crutzen, P. J., Kiehl, J. T., and Rosenfeld, D.: Aerosols, climate, and the hydrological cycle, Science, 294, 2119-2124, 2001.
87. Rasch, P. J., Barth, M. C., Kiehl, J. T., Schwartz, S. E., and Benkovitz, C. M.: A description of the global sulfur cycle and its controlling processes in the National Center for Atmospheric Research Community Climate Model, J. Geophys. Res., 105, 1367-1386, 2000.
88. Ravishankara, A. R.: Heterogeneous and multiphase chemistry in the troposphere, Science, 276, 1058-1066, 1997.
89. Remer. L. A., Tanré, D., Kaufman, Y. J., Ichoku, C., Mattoo, S., Levy, R., Chu, D. A., Holben, B., Dubovik, O., Smirnov, A., Martins, J. V., Li, R. R., and Ahmad, Z.: Validation of MODIS aerosol retrieval over ocean, Geophys. Res. Lett., 29, 8008, doi:10.1029/2001GL013 204, 2002.
90. Roeckner, E., Baeuml, G., Bonventura, L., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kirchner, I., Kornblueh, L., Manzini, E., Rhodin, A., Schlese, U., Schulzweida, U., and Tompkins, A.: The atmospheric general circulation model ECHAM5. PART I: Model description, Report 349, Max Planck Institute for Meteorology, Hamburg, Germany, available from http://www.mpimet.mpg.de, 2003.
91. Roelofs, G.-J., Lelieveld, J., and Ganzeveld, L.: Simulation of global sulfate distribution and the influence on effective cloud drop radii with a coupled photochemistry sulfur cycle model, Tellus B, 50, 224-242, 1998.
92. Schaap, M., Gon, H. A. C. D. V. D., Dentener, F. J., Visschedijk, A. J. H., Loon, M. V., ten Brink, H. M., Putaud, J.-P., Guillaume, B., Liousse, C., and Builtjeses, P. J. H.: Anthropogenic black carbon and fine aerosol distribution over Europe, J. Geophys. Res., 109, D18 207, doi:10.1029/2003JD004 330, 2004.
93. Schulz, M., Balkanski, Y. J., Guelle, W., and Dulac, F.: Role of aerosol size distribution and source location in a three dimensional simulation of a Saharan dust episode tested against satellite-derived optical thickness, J. Geophys. Res., 103, 10 579-10 592, 1998.
94. Schulz, M., de Leeuw, G., and Balkanski, Y.: Emission Of Atmospheric Trace Compounds, chap. Sea-salt aerosol source functions and emissions, pp. 333-359, Ed. Kluwer, 2004.
95. Seinfeld, J. H. and Pandis, S. N.: Atmospheric chemistry and physics: from air pollution to climate change, Wiley-Interscience, 1998.
96. Seinfeld, J. H., Carmichael, G. R., Arimoto, R., Conant, W. C., Brechtel, F. J., Bates, T. S., Cahill, T. A., Clarke, A. D., Doherty, S. J., Flatau, P. J., Huebert, B. J., Kim, J., Markowicz, K. M., Quinn, P. K., Russell, L. M., Russell, P. B., Shimizu, A., Shinozuka, Y., Song, C. H., Tang, Y. H., Uno, I., Vogelmann, A. M., Weber, R. J., Woo, J. H., and Zhang, X. Y.: ACE-ASIA - Regional climatic and atmospheric chemical effects of Asian dust and pollution, Bull. Am. Meteorol. Soc., 85, 367-380, 2004.
97. Shettle, E. P. and Fenn, R. W.: Models of the aerosols of the lower atmosphere and the effects of humidity variations on their optical properties, Tech. rep., Air Force Geoph. Lab., Massachusetts, project 7670, 1979.
98. Simmons, A. J. and Gibson, J. K.: The ERA-40 project plan, ERA-40 Project Report Series 1, ECMWF, Shinfield Park, Reading, UK, 2000.
99. Slinn, S. A. and Slinn, W. G. N.: Predictions for particle deposition on natural waters, Atmos. Environ., 14, 1013-1016, 1980.
100. Slinn, W. G. N.: Atmosphere-surface exchange of particulate and gaseous pollutants, chap. Dry deposition and resuspension of aerosol particles - a new look at some old problems, pp. 1-40, U.S. DOE Tech. Info. Center, Oak Ridge, TN, USA, 1976.
101. Slinn, W. G. N.: Predictions for particle deposition to vegetative canopies, Atmos. Environ., 16, 1785-1794, 1982.
102. Smith, M. and Harrison, N.: The sea spray generation function, J. Aerosol Sci., 29, 189-190, 1998.
103. Stokes, R. H. and Robinson, R. A.: Interactions in aqueous non-electolyte solutions. I. Solute-solvent equilibria, J. Phys. Chem., 70, 2126-2130, 1966.
104. Takemura, T., Okamoto, H., Maruyama, Y., Numaguti, A., Higurashi, A., and Nakajima, T.: Tropospheric global three-dimensional simulation of aerosol optical thickness distribution of various origins, J. Geophys. Res., 105, 17 853-17 873, 2000.
105. Tang, I. N.: Thermodynamic and optical properties of mixed-salt aerosols of atmospheric importance, J. Geophys. Res., 102, 1883-1893, 1997.
106. Tanré, D., Kaufman, Y. J., Herman, M., and Mattoo, S.: Remote sensing of aerosol properties over oceans using the MODIS/EOS spectral radiances, J. Geophys. Res., 102, 16 971-16 988, 1997.
107. Tegen, I. and Lacis, A. A.: Modelling the particle size distribution and its influence on the radiative properties of mineral dust aerosol, J. Geophys. Res., 101, 19 237-19 244, 1997.
108. Tegen, I., Hollrig, P., Chin, M., Fung, I., Jacob, D., and Penner, J.: Contribution of different aerosol species to the global aerosol extinction optical thickness: Estimates from model results, J. Geophys. Res., 102, 23 895-23 915, 1997.
109. Tegen, I., Harrison, S. P., Kohfeld, K., Prentice, I. C., Coe, M., and Heimann, M.: Impact of vegetation and preferential source areas on global dust aerosol: Results from a model study, J. Geophys. Res., 107, 4576-4597, 2002.
110. Tiedtke, M.: A comprehensive mass flux scheme for cumulus parameterization in large scale models, Mon. Wea. Rev., 117, 1779-1800, 1989.
111. Timmreck, C. and Schulz, M.: Significant dust simulation differences in nudged and climatological operation mode of the AGCM ECHAM, J. Geophys. Res., 109, D13 202, doi:10.1029/2003JD004 381, 2004.
112. Tompkins, A.: A prognostic parameterization for the subgrid-scale variability of water vapor and clouds in large-scale models and its use to diagnose cloud cover, J. Atmos. Sci., 59, 1917-1942, 2002.
113. Toon, O. B. and Ackerman, T. P.: Algorithms for the calculation of scattering by stratified spheres, Appl. Opt., 20, 3657-3660, 1981.
114. Torres, O., Bhartia, P., Herman, J., Sinyuk, A., and Holben, B.: A long term record of aerosol optical thickness from TOMS observations and comparisons to AERONET measurements, J. Atmos. Sci., 59, 398-413, 2002.
115. Tsigardis, K. and Kanakidou, M.: Global modelling of secondary organic aerosol in the troposphere: a sensitivity analysis, Atmos. Chem. Phys., 3, 1849-1869, 2003.
116. Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251-1256, 1974.
117. Twomey, S.: The Influence of Pollution on the Shortwave Albedo of Clouds, J. Atmos. Sci., 34, 1149-1152, 1977.
118. Unsworth, J., Wauchope, R., Klein, A., Dorn, E., Zeeh, B., Yeh, S., Akerblom, M., Racke, K., and Rubin, B.: Significance of long-range transport of pesticides in the atmosphere, Pure Appl. Chem., 71, 1359-1383, 1999.
119. van der Werf, G. R., Randerson, J. T., Collatz, G. J., and Giglio, L.: Carbon emissions from fires in tropical and subtropical ecosystems, Global Change Biology, 9, 547-562, 2003.
120. van Pul, W., de Leeuw, F., van Jaarsveld, J., van der Gaag, M., and Sliggers, C.: The potential for long-range transboundary atmospheric transport, Chemosphere, 37, 113-141, 1998.
121. Vehkamäki, H., Kulmala, M., Napari, I., Lehtinen, K. E. J., Timmreck, C., Noppel, M., and Laaksonen, A.: An improved parameterization for sulfuric acid water nucleation rates for tropospheric and stratospheric conditions, J. Geophys. Res., 107, 4622-4632, 2002.
122. Vignati, E., Wilson, J., and Stier, P.: M7: a size resolved aerosol mixture module for the use in global aerosol models, J. Geophys. Res., 109, D22 202, doi:10.1029/2003JD004 485, 2004.
123. Vink, S. and Measures, C.: The role of dust deposition in determining surface water distributions of Al and Fe in the South West Atlantic, Deep See Res., 48, 2782-2809, 2001.
124. Wilson, J., Cuvelier, C., and Raes, F.: A modelling study of global mixed aerosol fields, J. Geophys. Res., 106, 34 081-34 108, 2001.
125. Zadanovskii, A. B.: New methods for calculating solubilities of electrolytes in multicomponent systems, Zhur. Fiz. Kim., 22, 1475-1485, 1948.