Radiolytic modelling intercomparison exercise: Influence of alpha radiation on spent fuel alteration process

Proceedings of the International Conference on Radioactive Waste Management and Environmental Remediation, ICEM

Volumn 3, Issue , 2003, Pages 1617-1623

  Quiñones, Javier ^a   Merino, Juan ^b   Cera, Esther ^b   Bruno, Jordi ^b   Cobos, Joaquin ^a   Martínez Esparza, Aurora ^b  

^a CIEMAT   (Spain)

^b ENVIROS ^*  (Spain)

Author keywords

[No Author keywords available]

Indexed keywords

ALPHA RADIATION; RADIOLYTIC MODELING;

CORROSION; IRRADIATION; MATHEMATICAL MODELS; MIXED OXIDE FUELS; OXIDATION; RADIOACTIVITY; REDOX REACTIONS; SCINTILLATION; URANIUM;

RADIOACTIVE WASTES;

EID: 16544367961     PISSN: None     EISSN: None     Source Type: Conference Proceeding    
DOI: 10.1115/ICEM2003-4574     Document Type: Conference Paper

References (13)

1. M. Bickel, D. Feinauer, K. Mayer, S. Möbius, and H. Wedemeyer, "Uranium Dioxide: Chemical behavior," in Gmelin Handbook of inorganic and organometallic Chemistry, vol. 5, Suppl. C6, D. Fischer, W. Huisi, and F. Stein, Eds.: Springer-Verlag, 1996.
2. V.M. Oversby, Uranium dioxide, SIMFUEL, and spent fuel dissolution rates - a review of published data, vol. TR-99-22, 1999.
3. V.V. Rondinella, J. Cobos, H. j. Matzke, T. Wiss, P. Carbol, and D. Solatie, Mat. Res. Soc. Symp. Proc., vol. 663, pp. 392-399, 2001.
4. A. Martínez-Esparza, J. A. Esteban, J. Quiñones, J. de Pablo, I. Casas, J. Giménez, F. Clarens, M. Rovira, J. Merino, E. Cera, and J. Bruno, "Modelling Spent Fuel and HLW Behaviour in Repository Conditions. A review of the stat of the art," in Publicaciones técnicas, vol. 08/2002, Publicaciones técnicas. Madrid: ENRESA, 2002.
5. P. Kirkegaard and E. Bjergbakke, CHEMSIMUL: A Simulator for Chemical Kinetics. Roskilde, Denmark: Riso National Laboratory, 1999.
6. M.B. Carver, D.V. Hanley, and K.R. Chaplin, "Maksima Chemist. A program for mass action kinetics simulation by automatic chemical equation manipulation and integration by using Stiff techniques," AECL, Chalk River, Ontario AECL-6413, 1979.
7. J. Cobos, H. Matzke, V.V. Rondinella, A. Martínez Esparza, and T. Wiss, presented at Proc. GLOBAL '99 Int. Conf. on Future Nuclear Systems, Jackson Hole, USA, A.N.S, 1999.
8. J. Quiñones, J. A. Serrano, P. Díaz, J.L. Rodríguez, J. Bruno, E. Cera, J. Merino, A. Martínez Esparza, and J.A. Esteban, "Cálculo de la generación de productos radiolíticos en agua por radiación alfa. Determinación de la velocidad de alteración de la matriz del combustible gastado.," in Publicación técnica ENRESA, vol. 2/2000: ENRESA, 2000.
9. M.E. Torrrero, E. Baraj, J. de Pablo, J. Giménez, and I. Casas, "Kinetics of corrosion and dissolution of uranium dioxide as a function of pH," Int. J. Chem. Kinet., vol. 29, pp. 261-267, 1997.
10. A.B. Ross, W.G. Mallard, W.P. Helman, G.V. Buxton, R. E. Huie, and P. Neta, NDRL/NIST Solution Kinetics Database: Ver. 3.0. Gaithersburg, MD 20899: Notre Dame Radiation Laboratory, Notre Dame, IN and National Institute of Standars and Technology, 1998.
11. 2 containing alpha-emitters.," Radiochimca Acta, vol. 90, pp. 597-602, 2002.
12. J.A. Serrano, J. Quiñones, J. Cobos, P. Díaz, V.V. Rondinella, J.P. Glatz, H. Matzke, A. Martínez Esparza, and J.A. Esteban, "Leaching study of the behaviour of spent fuel and SIMFUEL under simulated granitic repository conditions," Radioactive Waste Management and Environmental Remediation - ASME, 2001.
13. J. de Pablo, I. Casas, F. Clarens, J. Giménez, and M. Rovira, "Contribución experimental y modelización de procesos básicos para el desarrollo del modelo de alteración de la matriz del combustible irradiado," in Publicaciones técnicas, vol. 01/2003. Madrid, SPAIN: ENRESA, 2003.