Direct observation of an isopolyhalomethane O-H insertion reaction with water: Picosecond time-resolved resonance Raman (ps-TR3) study of the isobromoform reaction with water to produce a CHBr2OH product

Journal of Chemical Physics

Volumn 120, Issue 7, 2004, Pages 3323-3332

  Kwok, Wai Ming ^a   Zhao, Cunyuan ^a,b   Li, Yun Liang ^a   Guan, Xiangguo ^a   Phillips, David Lee ^a  

^a UNIVERSITY OF HONG KONG   (Hong Kong)

^b NORTHWEST NORMAL UNIVERSITY   (China)

Author keywords

[No Author keywords available]

Indexed keywords

ACETONITRILE; CHEMICAL BONDS; HYDROGEN; LIGHT ABSORPTION; LIGHT SCATTERING; OXYGEN; PHOTOLYSIS; PHOTONS; RAMAN SPECTROSCOPY; RESONANCE; SOLUTIONS;

INSERTION REACTIONS; REACTION PRODUCTS;

METHANE;

EID: 1642377192     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1640997     Document Type: Article

References (79)

1. Th. Class and K. Ballschmiter, J. Atmos. Chem. 6, 35 (1988).
2. S. Klick and K. Abrahamsson, J. Geophys. Res., [Oceans] 97, 12683 (1992).
3. K. G. Heumann, Anal. Chim. Acta 283, 230 (1993).
4. R. M. Moore, M. Webb, R. Tokarczyk, and R. Wever, J. Geophys. Res., [Oceans] 101, 20899 (1996).
5. C. T. McElroy, C. A. McLinden, and J. C. McConnell, Nature (London) 397, 338 (1997).
6. J. C. Mössigner, D. E. Shallcross, and R. A. Cox, J. Chem. Soc., Faraday Trans. 94, 1391 (1998).
7. L. J. Carpenter, W. T. Sturges, S. A. Penkett, and P. S. Liss, J. Geophys. Res., [Atmos.] 104, 1679 (1999).
8. B. Alicke, K. Hebstreit, J. Stutz, and U. Platt, Nature (London) 397, 572 (1999).
9. R. P. Wayne, Chemistry of Atmospheres, 3rd ed. (Oxford University Press, Oxford, U.K., 2000).
10. S.-F. Fan and D. J. Jacob, Nature (London) 359, 522 (1992).
11. M. Mozurkewich, J. Geophys. Res., [Atmos.l 100, 14199 (1995).
12. R. Vogt, P. J. Crutzen, and S. Sander, Nature (London) 383, 327 (1996).
13. R. Sander and P. J. Crutzen, J. Geophys. Res., [Atmos.] 101, 9121 (1996).
14. K. W. Oum, M. J. Lakin, D. O. DeHaan, T. Brauers, and B. J. Finalyson-Pitts, Science 279, 74 (1998).
15. C. T. McElroy, C. A. McLinden, and J. C. McConnell, Nature (London) 397, 338 (1999).
16. R. Vogi, R. Sander, R. V. Glasow, and P. J. Crutzen, J. Atmos. Chem. 32, 375 (1999).
17. W. Behnke, M. Elend, U. Krüger, and C. Zetzsch, J. Atmos. Chem. 34, 87 (1999).
18. E. M. Knipping, M. J. Lakin, K. L. Foster, P. Jungwirth, D. J. Tobias, R. B. Gerber, D. Dabdub, and B. J. Finalyson-Pitts, Science 288, 301 (2000).
19. B. J. Finalyson-Pitts and J. C. Hemminger, J. Phys. Chem. A 104, 11463 (2000).
20. K. L. Foster, R. A. Plastridge, J. W. Bottenheim, P. B. Shepson, B. J. Finalyson-Pitts, and C. W. Spicer, Science 291, 471 (2001).
21. X.-Y. Yu and J. R. Barker, J. Phys. Chem. A 107, 1313 (2003).
22. C. D. O'Dowd, J. L. Jimenez, R. Bahreini, R. C. Plagan, J. H. Seinfeld, K. Hamerl, L. Pirjola, M. Kulmala, S. G. Jennings, and T. Hoffmann, Nature (London) 417, 632 (2002).
23. G. Maier and H. P. Reisenauer, Angew. Chem., Int. Ed. Engl. 25, 819 (1986).
24. G. Maier, H. P. Reisenauer, J. Lu, L. J. Scaad, and B. A. Hess, Jr., J. Am. Chem. Soc. 112, 5117 (1990).
25. A. N. Tarnovsky, J.-L. Alvarez, A. P. Yartsev, V. Sündstrom, and E. Åkesson, Chem. Phys. Lett. 312, 121 (1999).
26. A. N. Tarnovsky, M. Wall, M. Gustafsson, N. Lascoux, V. Sundström, and E. Åkesson, J. Phys. Chem. A 106, 5999 (2002).
27. M. Wall, A. N. Tarnovsky, T. Pascher, V. Sundstr̈m, and E. Åkesson, J. Phys. Chem. A 107, 211 (2003).
28. W. M. Kwok, C. Ma, A. W. Parker, D. Phillips, M. Towrie, P. Matousek, and D. L. Phillips, J. Chem. Phys. 113, 7471 (2000).
29. W. M. Kwok, C. Ma, A. W. Parker, D. Phillips, M. Towrie, P. Matousek, X. Zheng, and D. L. Phillips, J. Chem. Phys. 114, 7536 (2001).
30. W. M. Kwok, C. Ma, A. W. Parker, D. Phillips, M. Towrie, P. Matousek, and D. L. Phillips, Chem. Phys. Lett. 341, 292 (2001).
31. X. Zheng, W.-H. Fang, and D. L. Phillips, J. Chem. Phys. 113, 10934 (2000).
32. X. Zheng, C. W. Lee, Y.-L. Li, W.-H. Fang, and D. L. Phillips, J. Chem. Phys. 114, 8347 (2001).
33. D. L. Phillips, W.-H. Fang, and X. Zheng, J. Am. Chem. Soc. 123, 4197 (2001).
34. D. L. Phillips and W.-H. Fang, J. Org. Chem. 66, 5890 (2001).
35. Y.-L. Li, K. H. Leung, and D. L. Phillips, J. Phys. Chem. A 105, 10621 (2001).
36. W.-H. Fang, D. L. Phillips, D. Wang, and Y.-L. Li, J. Org. Chem. 67, 154 (2002).
37. Y.-L. Li, D. M. Chen, D. Wang, and D. L. Phillips, J. Org. Chem. 67, 4228 (2002).
38. Y.-L. Li, D. Wang, and D. L. Phillips, J. Chem. Phys. 117, 7931 (2002).
39. B. Zurawski and W. Kutzelnigg, J. Am. Chem. Soc. 100, 2654 (1978).
40. S. Sakai, Int. J. Quantum Chem. 70, 291 (1998).
41. L. B. Harding, H. B. Schlegel, R. Krishnan, and J. A. Pople, J. Phys. Chem. 84, 3394 (1980).
42. J. A. Pople, K. Raghavachari, M. J. Frisch, J. B. Blinkley, and P. V. R. Schleyer, J. Am. Chem. Soc. 105, 6389 (1983).
43. C. Wesdemiotis, R. Feng, P. O. Danis, E. R. Williams, and F. W. Lafferty, J. Am. Chem. Soc. 108, 5847 (1986).
44. B. F. Yates, W. J. Bouma, and L. Radom, J. Am. Chem. Soc. 109, 2250 (1987).
45. W. Kirmse, T. Meinert, D. A. Moderelli, and M. S. Platz, J. Am. Chem. Soc. 115, 8918 (1993).
46. S. P. Walch, J. Chem. Phys. 98, 3163 (1993).
47. C. Gonzalez, A. Restrepo-Cossio, M. Márquez, and K. B. Wiberg, J. Am. Chem. Soc. 118, 5408 (1996).
48. C. J. Moody and G. H. Whitman, in Reactive Intermediates, edited by S. G. Davies (Oxford University Press, New York, 1992).
49. J. R. Pliego, Jr. and W. B. De Almeida, J. Phys. Chem. 100, 12410 (1996).
50. J. R. Pliego, Jr. and W. B. De Almeida, J. Phys. Chem. A 103, 3904 (1999).
51. W. M. Kwok, C. Ma, A. W. Parker, D. Phillips, M. Towrie, P. Matousek, and D. L. Phillips, J. Phys. Chem. A 107, 2624 (2003).
52. Y.-L. Li, C. Y. Zhao, W. M. Kwok, X. G. Guan, P. Zuo, and D. L. Phillips, J. Chem. Phys. 119, 4671 (2003).
53. M. J. Frisch, G. W. Trucks, H. B. Schlegel et al., GAUSSIAN 98, Revision A.7, Gaussian, Inc., Pittsburgh PA, 1998.
54. C. Gonzalez and H. B. Schlegel, J. Chem. Phys. 90, 2154 (1989); J. Phys. Chem. 94, 5523 (1990).
55. C. Gonzalez and H. B. Schlegel, J. Chem. Phys. 90, 2154 (1989); J. Phys. Chem. 94, 5523 (1990).
56. See EPAPS Document No. E-JCPSA6-120-507407 for supporting information on the Cartesian coordinates, total energies and vibrational zero-point energies for selected stationary structures shown in Fig. 4. A direct link to this document may be found in the online article's HTML reference section. The document may also be reached via the EPAPS homepage (http://www.aip.org/pubservs/epaps.html) or from ftp.aip.org in the directory/epaps/. See the EPAPS homepage for more information.
57. S. Q. Man, W. M. Kwok, and D. L. Phillips, J. Phys. Chem. 99, 15705 (1995).
58. W. M. Kwok and D. L. Phillips, J. Chem. Phys. 104, 2529 (1996).
59. W. M. Kwok and D. L. Phillips, J. Chem. Phys. 104, 9816 (1996).
60. S. Q. Man, W. M. Kwok, A. E. Johnson, and D. L. Phillips, J. Chem. Phys. 105, 5842 (1996).
61. Y.-L. Li, P. Zuo, and D. L. Phillips, Chem. Phys. Lett. 364, 573 (2002).
62. C. Conley and F.-M. Tao, Chem. Phys. Lett. 301, 29 (1999).
63. B. J. Gertner, G. H. Peslherbe, and J. T. Hynes, Isr. J. Chem. 39, 273 (1999).
64. E. M. Cabaleiro-Lago, J. M. Hermida-Ramón, and J. Rodríguez-Otero, J. Chem. Phys. 117, 3160 (2002).
65. S. M. Hurley, T. E. Dermota, D. P. Hydutsky, and A. W. Castleman, Jr., Science 298, 202 (2002).
66. H. M. Lee and K. S. Kim, J. Chem. Phys. 114, 4461 (2001).
67. M. Kowal, R. W. Gora, S. Roszak, and J. Lexzczynski, J. Chem. Phys. 115, 9260 (2001).
68. M. Kawasaki, S. J. Lee, and R. Bersohn, J. Chem. Phys. 63, 809 (1975).
69. G. Schmitt and F. J. Comes, J. Photochem. 14, 107 (1980).
70. P. M. Kroger, P. C. Demou, and S. J. Riley, J. Chem. Phys. 65, 1823 (1976).
71. J. B. Koffend and S. R. Leone, Chem. Phys. Lett. 81, 136 (1981).
72. S. R. Cain, R. Hoffman, and R. Grant, J. Phys. Chem. 85, 4046 (1981).
73. S. J. Lee and R. Bersohn, J. Phys. Chem. 86, 728 (1982).
74. L. J. Butler, E. J. Hintsa, and Y. T. Lee, J. Chem. Phys. 84, 4104 (1986).
75. L. J. Butler, E. J. Hintsa, and Y. T. Lee, J. Chem. Phys. 86, 2051 (1987).
76. Q. Zhang, U. Marvet, and M. Dantus, J. Chem. Phys. 109, 4428 (1998).
77. K.-W. Jung, T. S. Ahmadi, and M. A. El-Sayed, Bull. Korean Chem. Soc. 18, 1274 (1997).
78. K. Kavita and P. K. Das, J. Chem. Phys. 112, 8426 (2000).
79. I. Nocole, J. de Laat, M. Dore, J. P. Duguet, and H. Suty, Environ. Sci. Technol. 12, 21 (1991).