Rejuvenation of moisture-exposed Pd/δ-Al2O3 catalysts for isoprene-selective hydrogenation: Correlation between Pd dispersion and catalytic properties

Industrial and Engineering Chemistry Research

Volumn 44, Issue 6, 2005, Pages 1677-1687

  Su, Wei Bin ^a   Tang, Mau Tsu ^b   Chang, Jen Ray ^a  

^a NATIONAL CHUNG CHENG UNIVERSITY   (Taiwan)

^b NATIONAL SYNCHROTRON RADIATION RESEARCH CENTER   (Taiwan)

Author keywords

[No Author keywords available]

Indexed keywords

CATALYSTS; CHEMISORPTION; COKE; DEPOSITION; DISPERSIONS; PALLADIUM COMPOUNDS; SPECTROSCOPIC ANALYSIS;

ISOPRENES; REJUVENATION PROCEDURE; STEADY STATE; TERMINAL SITE;

HYDROGENATION;

2 METHYL 2 BUTENE; HYDROCARBON; ISOPRENE; PALLADIUM; UNCLASSIFIED DRUG;

HYDROGENATION;

ABSORPTION; ADSORPTION; ARTICLE; CATALYSIS; CATALYST; CHEMICAL STRUCTURE; DESORPTION; DIFFERENTIAL SCANNING CALORIMETRY; DISPERSION; HYDROGENATION; INFRARED SPECTROSCOPY; MOISTURE; TEMPERATURE; X RAY SPECTROMETRY;

EID: 14844339008     PISSN: 08885885     EISSN: None     Source Type: Journal    
DOI: 10.1021/ie049054y     Document Type: Article

References (35)

1. Griffiths, D. J.; Luntz, D. M.; James, J. L. Making the Most out of Pyrolysis Gasoline. Oil Gas J. 1968, 27, 613.
2. Lepage, J. F.; Courty, P.; Freund, E.; Franck, J. P.; Jacquin, Y.; Juguin, B.; Marcilly, C.; Marino, G.; Miguel, J.; Montarnal, R.; Sugier, A.; Landeghem, H. V. Applied Heterogeneous Catalysis Design Manufacture Use of Solid Catalysts; Institut Franaâis du Pètrole, Gulf Publishing Co.: Houston, TX, 1987; p 329.
3. Boitiaux, J.-P.; Cosyns, J.; Derrien, M.; Leger, G. Newest Hydrogenation Catalysts. Hydrocarbon Process. 1985, Mar, 51.
4. Zieliński, J. Morphology of Nickel/Alumina Catalysts. J. Catal. 1982, 76, 157.
5. 3. Appl. Catal., A 1994, 110, 217.
6. Koningsberger, D. C.; Prins, R. X-ray Absorption: Principles, Applications, Techniques of EXAFS, SEXAFS, and XANES; John Wiley & Sons: New York, 1988.
7. Jong, P. S.; Wang, C. Y.; Leu, S. H. The Operation Manual of Hydrogenation of Pyrolysis Gasoline on No. 4 Naphtha Cracker Plant; Chinese Petroleum Corp.: Taiwan, 1984; Vol. 134.
8. Lin, T.-B.; Chou, T.-C. Selective Hydrogenation of Isoprene on Egg-shell and Uniform Palladium Profile Catalyst. Appl. Catal., A 1994, 108, 7.
9. Jones, A.; McNicol, B. Temperature-Programmed Reduction for Solid Materials Characterization; Marcel Dekker: New York, 1986; p 70.
10. Satterfield, C. N. Trickled Bed Reactors (Review). AIChE J. 1975, 21, 209.
11. Cheng, Y.-M.; Chang, J.-R.; Wu, J. C. Kinetic Study of Pyrolysis Gasoline Hydrogenation over Supported Palladium Catalyst. Appl. Catal. 1986, 24, 273.
12. 3 in Selective Hydrogenation of Pyrolysis Gasoline. Ind. Eng. Chem. Res. 2000, 39, 4063.
13. Furlong, B. K.; Hightower, J. W.; Chan, T. Y.-L.; Sarkany, A.; Guczi, L. 1,3-Butadiene Selective Hydrogenation Over Pd/Alumina and CuPd/Alumina Catalysts. Appl. Catal., A 1994, 117, 41.
14. Chang, J.-C.; Chou, T.-C. Selective Hydrogenation of Isoprene over δ-Alumina-Supported Eggshell Pd Catalysts: Particle Size Effects. Appl. Catal., A 1997, 156, 193.
15. Little, L. H. Infrared Spectra of Adsorbed Species; Academic Press: London, 1966.
16. van Zon, J. B. A. D. Ph.D. Dissertation, Eindhoven University of Technology, The Netherlands, 1988.
17. Asakura, K. In Iwasawa, Y., Ed.; X-ray Absorption Fine Structure for Catalysts and Surface; World Scientific: Singapore, 1995; p 52.
18. Koningsberger, D. C.; Gates, B. C. Nature of the Metal-Support Interface in Supported Metal Catalysts: Results from X-ray Absorption Spectroscopy. Catal. Lett. 1992, 13, 271.
19. Vaarkam, M.; Linders, J. C.; Koningsberger, D. C. XDAP User's Guide; XAFS Service International, 1996.
20. Lee, P. A.; Beni, G. New Method for the Calculation of Atomic Phase Shifts: Application to Extended X-ray Absorption Fine structure (EXAFS) in Molecules and Crystals. Phys. Rev. B 1977, 15, 2862.
21. Kampers, F. W. H. EXAFS in Catalysis Instrmentation and Applications. Ph.D. Dissertation, Eindhoven University of Techonology, The Netherlands, 1988.
22. Aduriz, H. R.; Bodnariuk, P.; Coq, B.; Figueras, F. Alumina-Supported Bimetallics of Palladium Alloyed with Germanium, Tin, Lead, or Antimony from Organometallic Precursors. J. Catal. 1991, 129, 47.
23. Horsley, J. A. Stability of Supported Catalysts: Sintering and Redispersion. Catal. Stud. Div. 1991, 11-91.
24. Wanke, S. E.; Szymura, J. A.; Yu, T.-T. The Sintering of Supported Metal Catalysts. In Catalyst Deactivation; Petersen, E. E., Bell, A. T., Eds.; Marcel Dekker: New York, 1987.
25. Geus, J. W. Preparation and Thermal Stability of Supported Metal Catalysts. in Sintering and Catalysis; Kuczynski, G. C., Ed. Mater. Sci. Res., 10; Plenum Press: New York, 1975.
26. Germain, J. E. Catalytic Conversion of Hydrocarbons; Academic Press: London, 1969.
27. Lin, T.-B.; Chou, T.-C. Pd Migration. 1. A Possible Reason for the Deactivation of Pyrolysis Gasoline Partial Hydrogenation Catalysts. Ind. Eng. Chem. Res. 1995, 34, 128.
28. Sze, M. C.; Bauer, W. V. Petrochem Show Issue: Hydrorefining Pyrolysis Gasoline. Chem. Eng. Prog. 1969, 65, 59.
29. Trimm, D. L. Catalyst Design for Reduced Coking: Review. Appl. Catal. 1983, 5, 263.
30. Moyes, R. B.; Wells, P. B.; Grant, J.; Salman, N. Y. Electronic Effects in Butadiene Hydrogenation Catalyzed by the Transition Metals. Appl. Catal. 2002, 229, 251.
31. Ryndin, Yu. A.; Nosova, L. V.; Boronin, A. I.; Chuvilin, A. L. Effect of Dispersion of Supported Palladium on its Electronic and Catalytic Properties in the Hydrogenation of Vinylacetylene. Appl. Catal. 1988, 42, 131.
32. Ryndin, Yu. A.; Stenin, M. V.; Boronin, A. I.; Bukhtiyarov, V. I.; Zaikovskii, V. I. Effect of Pd/C Dispersion on its Catalytic Properties in Acetylene and Vinylacetylene Hydrogenation. Appl. Catal. 1989, 54, 277.
33. Bazin, D.; Sayers, D.; Rher, J. Comparison between X-ray Absorption Spectroscopy, Anomalous Wide-Angle X-ray scattering, Anomalous Small-Angle X-ray Scattering, and Diffraction Anomalous Fine Structure Techniques Applied to Nanometer-Scale Metallic Clusters. J. Phys. Chem. B 1997, 101, 11040.
34. Mojet, B. L.; Miller, J. T.; Ramaker, D. E.; Koningsberger, D. C. A New Model Describing the Metal-Support Interaction in Nobel Metal Catalysts. J. Catal. 1999, 186, 373.
35. Cotton, F. A.; Wilkinson, G. Advanced Inorganic Chemistry; John Wiley & Sons: New York, 1988.